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Confinement can significantly alter fluid properties, offering potential for specific technological applications. However, achieving precise control over the structural complexity of confined fluids and soft matter remains challenging, as…

Soft Condensed Matter · Physics 2024-11-20 Fabio Leoni , Erdal C. Oğuz , Giancarlo Franzese

Freezing of water droplets placed on the bare and superhydrophobic surfaces of polymer wedges are studied both experimentally and computationally. Two-dimensional numerical calculations of the transient temperature field in a chilled…

We investigate the structural, thermodynamic and dynamic behavior of of a two dimensional core-corona system using Langevin Dynamics simulations. The particles are modeled using a core-softened potential that exhibits waterlike anomalies…

Soft Condensed Matter · Physics 2018-02-14 José Rafael Bordin , Marcia C. Barbosa

The so-called thermodynamic anomalies of water form an integral part of the peculiar behaviour of this both important and ubiquitous molecule. In this paper our aim is to establish whether the recently proposed TIP4P/2005 model is capable…

In the present article we carry out a molecular dynamics study of the core-softened system and show that the existence of the water-like anomalies in this system depends on the trajectory in $P-\rho-T$ space along which the behavior of the…

Soft Condensed Matter · Physics 2010-10-21 Yu. D. Fomin , V. N. Ryzhov

Many of the anomalous properties of water are amplified in the deeply supercooled region. Here we present neutron scattering measurements of the density of heavy water confined in a nanoporous silica matrix MCM-41-S (\approx15 {\AA} pore…

We study the effect of confinement on glassy liquids using Random First Order Transition theory as framework. We show that the characteristic length-scale above which confinement effects become negligible is related to the point-to-set…

Disordered Systems and Neural Networks · Physics 2013-10-01 C. Cammarota , G. Gradenigo , G. Biroli

Context. The level of porosity of interstellar ices - largely comprised of amorphous solid water (ASW) - contains clues on the trapping capacity of other volatile species and determines the surface accessibility that is needed for solid…

Solar and Stellar Astrophysics · Physics 2014-12-10 S. Cazaux , J. -B. Bossa , H. Linnartz , A. G. G. M. Tielens

In this paper we present a simulation study of water-like anomalies in core-softened system introduced in our previous publications. We investigate the anomalous regions for a system with the same functional form of the potential but with…

Soft Condensed Matter · Physics 2015-05-30 Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

We use a one-dimensional (1d) core-softened potential to develop a physical picture for some of the anomalies present in liquid water. The core-softened potential mimics the effect of hydrogen bonding. The interest in the 1d system stems…

Soft Condensed Matter · Physics 2009-10-31 M. Reza Sadr-Lahijany , Antonio Scala , Sergey~V. Buldyrev , H. Eugene Stanley

We consider the phase behavior of two-dimensional ($2D$)system of particles with an isotropic core-softened potential introduced in our previous publications. As one can expect from the qualitative consideration for the three dimensional…

Soft Condensed Matter · Physics 2015-06-18 D. E. Dudalov , Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

We show that the existence of the water-like anomalies in kinetic coefficients in the core-softened systems depends on the trajectory in $\rho-T$ plane along which the kinetic coefficients are calculated. In particular, it is shown that the…

Soft Condensed Matter · Physics 2010-08-06 Yu. D. Fomin , V. N. Ryzhov

We perform molecular dynamics simulations to investigate the diffusive motion of TIP5P water in the direction perpendicular to the two hydrophobic confining walls. To calculate the diffusion coefficient, we use the concept of the…

Soft Condensed Matter · Physics 2009-11-13 Sungho Han , Pradeep Kumar , H. Eugene Stanley

In this work, molecular dynamics simulations are performed to estimate the equilibrium pressure of liquid confined in nanopores. The simulations show that the pressure is highly sensitive to the pore size and can significantly change from…

Soft Condensed Matter · Physics 2021-04-21 An Zou , Shalabh C. Maroo

The properties of water can have a strong dependence on the confinement. Here, we consider a water monolayer nanoconfined between hydrophobic parallel walls under conditions that prevent its crystallization. We investigate, by simulations…

Soft Condensed Matter · Physics 2014-03-24 Valentino Bianco , Giancarlo Franzese

The adsorption of a near-critical fluid confined in a slit pore is investigated by means of density functional theory and by Monte Carlo simulation for a Lennard-Jones fluid. Our work was stimulated by recent experiments for SF_6 adsorbed…

Statistical Mechanics · Physics 2009-10-31 A. Maciolek , R. Evans , N. B. Wilding

When water molecules are confined to nanoscale spacings, such as in the nanometer size pores of activated carbon fiber (ACF), their freezing point gets suppressed down to very low temperatures ($\sim$ 150 K), leading to a metastable liquid…

Soft Condensed Matter · Physics 2015-06-23 S. O. Diallo , L. Vlcek , E. Mamontov , J. K. Keum , Jihua Chen , J. S. Hayes , A. A. Chialvo

We study, by Monte Carlo simulations, a coarse-grained model of a water monolayer between hydrophobic walls at partial hydration, with a wall-to-wall distance of about 0.5 nm. We analyze how the diffusion constant parallel to the walls,…

Soft Condensed Matter · Physics 2011-09-14 Francisco de los Santos , Giancarlo Franzese

Water confined in nanoscale cavities plays a crucial role in everyday phenomena in geology and biology, as well as technological applications at the water-energy nexus. However, even understanding the basic properties of nano-confined water…

We explore the structural properties of anomalous fluids confined in a nanopore using Molecular Dynamics simulations. The fluid is modeled by core-softened (CS) potentials that have a repulsive shoulder and an attractive well at a further…

Soft Condensed Matter · Physics 2014-10-22 Leandro B. Krott , José Rafael Bordin , Marcia Barbosa