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Despite the growing interest in topological materials, the difficulty of experimentally synthesizing and integrating them with other materials has been one of the main barriers restricting access to their unique properties. Recent advances…

Materials Science · Physics 2020-03-25 Zhenyao Fang , Heng Gao , Jörn W. F. Venderbos , Andrew M. Rappe

The addition of dilute concentrations of bismuth (Bi) into GaAs to form GaBiAs alloys results in a large reduction of the band gap energy Eg accompanied by a significant increase of the spin-orbit-splitting energy (delta_SO), leading to an…

Materials Science · Physics 2015-06-11 Muhammad Usman , Christopher A Broderick , Eoin P. O'Reilly

Adding a few atomic percent of Bi to III--V semiconductors leads to significant changes in their electronic structure and optical properties. Bismuth substitution on the pnictogen site leads to a large increase in spin-orbit splitting…

Materials Science · Physics 2026-01-23 Abdul Saboor , Shoaib Khalid , Anderson Janotti

Gallium oxide (Ga2O3) is a wide-band-gap semiconductor promising for UV sensors and high power transistor applications, with Baliga's figure of merit that far exceeds those of GaN and SiC, second only to diamond. Engineering its band…

Materials Science · Physics 2019-06-04 Fernando P. Sabino , Xuefen Cai , Su-Huai Wei , Anderson Janotti

Incorporation of bismuth (Bi) in dilute quantities in (In)GaAs has been shown to lead to unique electronic properties that can in principle be exploited for the design of high efficiency telecomm lasers. This motivates the development of…

Materials Science · Physics 2013-09-16 Christopher A. Broderick , Muhammad Usman , Eoin P. O'Reilly

We develop an atomistic, nearest-neighbor sp3s* tight-binding Hamiltonian to investigate the electronic structure of dilute bismide alloys of GaP and GaAs. Using this model we calculate that the incorporation of dilute concentrations of Bi…

Materials Science · Physics 2011-12-12 Muhammad Usman , Christopher A. Broderick , Andrew Lindsay , Eoin P. O'Reilly

The incorporation of dilute concentrations of bismuth (Bi) into traditional III V alloys leads to significant reduction in bandgap energy, making InSbBi is a promising candidate for long wavelength infrared photodetection sensors due to its…

The LDA-1/2 method is employed in density functional theory calculations for the electronic structure of III-V dilute bismide systems. For the representative example of Ga(SbBi) with Bi concentrations below $10 \%$, it is shown that this…

Materials Science · Physics 2020-08-12 Sven C. Liebscher , Lars C. Bannow , Jörg Hader , Jerome V. Moloney , Stephan W. Koch

Anion substitution with bismuth (Bi) in III-V semiconductors is an effective method for experimental engineering of the band gap Eg at low Bi concentrations, in particular in gallium arsenide (GaAs). The inverse Bi-concentration dependence…

Using an $sp^{3}s^{*}$ tight-binding model we demonstrate how the observed strong bowing of the band gap and spin-orbit-splitting with increasing Bi composition in the dilute bismide alloy GaBi$_{x}$As$_{1-x}$ can be described in terms of a…

Materials Science · Physics 2018-11-08 Christopher A. Broderick , Muhammad Usman , Eoin P. O'Reilly

Significant efficiency droop is a major concern for light-emitting diodes and laser diodes operating at high current density. Recent study has suggested that heavily Bi-alloyed GaAs can decrease the non-radiative Auger recombination and…

Materials Science · Physics 2016-09-19 Guangfu Luo , Kamran Forghani , Thomas F. Kuech , Dane Morgan

Bi-containing III-V semiconductors constitute an exciting class of metastable compounds with wide-ranging potential optoelectronic and electronic applications. However, the growth of III-V-Bi alloys requires group-III-rich growth…

Materials Science · Physics 2019-04-16 Miriam Oliva , Guanhui Gao , Esperanza Luna , Lutz Geelhaar , Ryan B. Lewis

The incorporation of bismuth (Bi) in GaAs results in a large reduction of the band gap energy (E$_g$) accompanied with a large increase in the spin-orbit splitting energy ($\bigtriangleup_{SO}$), leading to the condition that…

Oxygen-scavenging at oxide heterointerfaces has emerged as a powerful route for stabilizing metastable phases that exhibit interesting phenomena, including high-mobility two-dimensional electron gases and high T$_{c}$ superconductivity. We…

Superconductivity · Physics 2025-12-16 Shama , Jordan T. McCourt , Merve Baksi , Gleb Finkelstein , Divine P. Kumah

Dilute nitride bismide GaNBiAs is a potential semiconductor alloy for near- and mid-infrared applications, particularly in 1.55 $\mu$m optical communication systems. Incorporating dilute amounts of Bismuth (Bi) into GaAs reduces the…

Mesoscale and Nanoscale Physics · Physics 2017-06-22 W. J. Fan , Sumanta Bose , D. H Zhang

Bulk bismuth presents outstanding optical properties, such as a giant infrared refractive index (n near 10) and a negative ultraviolet visible permittivity induced by giant interband electronic transitions. Although such properties are very…

Optics · Physics 2019-04-18 Johann Toudert , Rosalia Serna , Claire Deeb , Esther Rebollar

GaSbBi alloys have recently emerged as attractive materials for mid-infrared optoelectronics owing to strong band gap reduction enabled by Bi incorporation into the GaSb matrix. The fundamental understanding of the epitaxial process…

Applied Physics · Physics 2019-04-16 Joonas Hilska , Eero Koivusalo , Janne Puustinen , Soile Suomalainen , Mircea Guina

In this paper, the structural, electronic, mechanical and optical properties of antimonene-bismuthene Van-der Waals heterostructure (Sb-Bi HS) were calculated based on the first principle density functional theory. We explored different…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Shobair Mohammadi Mozvashi , Sahar Izadi Vishkayi , Meysam Bagheri Tagani

Highly mismatched semiconductor alloys such as GaNAs and GaBiAs have several novel electronic properties, including a rapid reduction in energy gap with increasing x and also, for GaBiAs, a strong increase in spin orbit- splitting energy…

Materials Science · Physics 2018-11-08 Christopher A. Broderick , Muhammad Usman , Stephen J. Sweeney , Eoin P. O'Reilly

Bi alloying is predicted to transform GaAs from a semiconductor to a topological insulator or semi-metal. To date, studies of the GaAs$_{1-x}$Bi$_x$ alloy band structure have been limited, and the origins of Bi-induced enhancement of the…

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