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Modern nonlinear optical materials allow light of one wavelength be efficiently converted into light at another wavelength. However, designing nonlinear optical materials to operate with ultrashort pulses is difficult, because it is…

We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…

Quantum Physics · Physics 2022-11-21 Emil J. Zak

Advances in the amplification and manipulation of ultrashort laser pulses has led to revolutions in several areas. Examples include chirped pulse amplification for generating high peak-power lasers, power-scalable amplification techniques,…

Optics · Physics 2016-08-24 C. R. Phillips , B. W. Mayer , L. Gallmann , U. Keller

Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…

Atomic and Molecular Clusters · Physics 2020-03-25 Zhao Xi , Wang Su-Ju , Yu Wei-Wei , Wei Hui , Lin C. D

Singly ionized nitrogen molecules in ambient air pumped by near-infrared femtosecond laser give rise to superradiant emission. Here we demonstrate coherent control of this superradiance by injecting a pair of resonant seeding pulses inside…

We introduce a general technique to generate compressed broadband terahertz pulses based on difference frequency generation of optical pump radiation using aperiodically poled structures. The pump pulse format and poling of the crystals…

Optics · Physics 2019-02-22 Koustuban Ravi , Franz X Kärtner

The generation of isolated attosecond pulses with high efficiency and high beam quality is essential for attosec- ond spectroscopy. We numerically investigate the supercontinuum generation in a neutral rare-gas medium driven by a two-color…

Optics · Physics 2015-05-30 Zhe Wang , Weiyi Hong , Qingbin Zhang , Shaoyi Wang , Peixiang Lu

We study optical response of a resonant medium possessing nonlinear coupling to external field driven by a few-cycle pump pulse sequence. We demonstrate the possibility to directly produce unipolar half-cycle pulses from the medium…

Lightwave pulse shaping in the picosecond regime has remained unaddressed because it resides beyond the limits of state-of-the-art techniques, either due to its inherently narrow spectral content or fundamental speed limitations in…

Optics · Physics 2025-03-10 Randy Lemons , Jack Hirschman , Hao Zhang , Charles Durfee , Sergio Carbajo

An isolated attosecond vortex $\gamma$-ray pulse is generated by using a relativistic spatiotemporal optical vortex (STOV) laser in particle-in-cell simulations. A $\sim$ 300-attosecond electron slice with transverse orbital angular…

Plasma Physics · Physics 2024-11-11 Fengyu Sun , Xinyu Xie , Wenpeng Wang , Stefan Weber , Xin Zhang , Yuxin Leng , Ruxin Li , Zhizhan Xu

Specific features of nonlinear interference processes at quantum transitions in near- and fully-resonant optically-dense Doppler-broadened medium are studied. The feasibility of overcoming of the fundamental limitation on a…

Quantum Physics · Physics 2009-11-11 A. K. Popov , S. A. Myslivets , Thomas F. George

Supercontinuum generation in all-normal-dispersion optical fibers has so far been predominantly explored under femtosecond pumping conditions. Here, we demonstrate that efficient and broadband supercontinuum generation can also be achieved…

The simultaneous laser-driven acceleration and angular manipulation of the fast electron beam is experimentally demonstrated. The bunch of multi-MeV energy charged particles is generated during the propagation of the femtosecond laser pulse…

Plasma Physics · Physics 2023-10-19 K. Ivanov , D. Gorlova , I. Tsymbalov , I. Tsygvintsev , S. Shulyapov , R. Volkov , A. Savelev

Nonlinear optical generation from a crystalline material can reveal the symmetries of both its lattice structure and underlying ordered electronic phases and can therefore be exploited as a complementary technique to diffraction based…

Strongly Correlated Electrons · Physics 2014-11-04 D. H. Torchinsky , H. Chu , T. Qi , G. Cao , D. Hsieh

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

Ultrafast laser pulses provide unique tools to manipulate magnetization dynamics at femtosecond timescales, where the interaction of the electric field -- such as excitation of spin carriers to non-equilibrium states, generation of…

We show how bright, fully coherent, hard x-ray beams can be generated through nonlinear upconversion of femtosecond laser light. By using longer-wavelength mid-infrared driving lasers of moderate peak intensity, full phase matching of the…

The interaction between relativistic electron beams and intense laser fields has been extensively studied for generating high-energy radiation. However, achieving coherent radiation from such interactions needs to precisely control the…

Plasma Physics · Physics 2025-09-01 H. Peng , T. W. Huang , C. N. Wu , K. Jiang , R. Li , C. Riconda , S. Weber , C. T. Zhou

We demonstrate experimentally a method of all-optical selective rotational control in gas mixtures. Using an optical centrifuge - an intense laser pulse whose linear polarization rotates at an accelerated rate, we simultaneously excite two…

Chemical Physics · Physics 2024-06-19 P. Amani , A. A. Milner , V. Milner

Various schemes are presented for the generation of circularly polarized molecular high-order harmonic generation (MHOHG) from molecules. In particular it is shown that combinations of counter-rotating circularly polarized pulses produce…

Optics · Physics 2015-12-15 Andre D. Bandrauk , Kai-Jun Yuan