Related papers: The exact solution for the free induction decay in…
The 19F spins in a crystal of fluorapatite have often been used to experimentally approximate a one-dimensional spin system. Under suitable multi-pulse control, the nuclear spin dynamics may be modeled to first approximation by a…
Nuclear spin-1/2 lattices where each spin has a small effective number of interacting neighbors represent a particular challenge for first-principles calculations of free induction decays (FIDs) observed by nuclear magnetic resonance (NMR).…
Strategies to protect multi-qubit states against decoherence are difficult to formulate because of their complex many-body dynamics. A better knowledge of the decay dynamics would help in the construction of decoupling control schemes. Here…
A new approach is presented that treats NMR spin-spin relaxation as kinetics in spin phase space. The approach is applied to free induction decay (FID) in solids containing equivalent nuclear spins 1/2. The description obtained does not…
We have measured the decay of NMR multiple quantum coherence intensities both under the internal dipolar Hamiltonian as well as when this interaction is effectively averaged to zero, in the cubic calcium fluoride (CaF2) spin system and the…
First-principles calculations of high-temperature spin dynamics in solids in the context of nuclear magnetic resonance (NMR) is a long-standing problem, whose conclusive solution can significantly advance the applications of NMR as a…
Multiple quantum (MQ) NMR methods \cite{Baum} are applied to the analysis of various problems of quantum information processing. It is shown that the two-spin/two-quantum Hamiltonian \cite{Baum} describing MQ NMR dynamics is related to the…
We investigate numerically the Multiple Quantum (MQ) NMR dynamics in systems of nuclear spins 1/2 coupled by the dipole-dipole interactions in the case of the pseudopure initial state. Simulations of the MQ NMR with the real molecular…
We evaluate free-induction decay for the transverse components of a localized electron spin coupled to a bath of nuclear spins via the Fermi contact hyperfine interaction. Our perturbative treatment is valid for special (narrowed) bath…
We investigate the system of a heavy impurity immersed in a degenerated Fermi gas, where the impurity's internal degree of freedom (pseudospin) is manipulated by a series of radiofrequency (RF) pulses at several different times. Applying…
Quantum correlations are investigated theoretically in a two-spin system with the dipole-dipole interactions in the NMR multiple-pulse spin-locking experiments. We consider two schemes of the multiple-pulse spin-locking. The first scheme…
We present a new experimental investigation of the NMR free induction decay (FID) in a lattice of spin-1/2 nuclei in a strong Zeeman field. Following a pi/2 pulse, evolution under the secular dipolar Hamiltonian preserves coherence number…
We investigate the limits of effectiveness of classical spin simulations for predicting free induction decays (FIDs) measured by solid-state nuclear magnetic resonance (NMR) on systems of quantum nuclear spins. The specific limits…
Quantum unitary evolution typically leads to thermalization of generic interacting many-body systems. There are very few known general methods for reversing this process, and we focus on the magic echo, a radio-frequency pulse sequence…
This letter presents a two-dimensional nuclear magnetic resonance(NMR) approach for constructing a two-logical-qubit decoherence-free subspace (DFS) based on the fact that the three protons in a CH3 spin system can not be resolved in…
NMR is the technique of election to probe the local properties of materials. Herein we present the results of density functional theory (DFT) \textit{ab initio} calculations of the NMR parameters for fluorapatite (FAp), a calcium…
Nuclear magnetic resonance (NMR) has been a widely used tool in various scientific fields and practical applications, with quantum control emerging as a promising strategy for synergistic advancements. In this paper, we propose a novel…
The free-induction decay (FID) of the transverse magnetization in a dipolar-coupled rigid lattice is a fundamental problem in magnetic resonance and in the theory of many-body systems. As it was shown earlier the FID shapes for the systems…
The space- and time-dependent response of many-body quantum systems is the most informative aspect of their emergent behaviour. The dynamical structure factor, experimentally measurable using neutron scattering, can map this response in…
The many body quantum dynamics of dipolar coupled nuclear spins I = 1/2 on an otherwise isolated cubic lattice are studied with nuclear magnetic resonance (NMR). By increasing the signal-to-noise ratio by two orders of magnitude compared…