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To improve the computational efficiencies of the real-space orbital-free density functional theory, this work develops a new single-grid solver by directly providing the closed-form solution to the inner iteration and using an improved…

Computational Physics · Physics 2023-05-16 Ling-Ze Bu , Wei Wang

A thesis providing a pedagogical introduction to the problem of achieving self-consistency in density functional theory. Contained is an introduction to the framework of Kohn-Sham density functional theory, leading then to the…

Other Condensed Matter · Physics 2018-03-06 Nick Woods

In this work, we address the efficient computation of parameterized systems of linear equations, with possible nonlinear parameter dependence. When the matrix is highly sensitive to the parameters, mean-based preconditioning might not be…

Numerical Analysis · Mathematics 2026-05-29 Wouter Gerrit van Harten , Laura Scarabosio

We present an accurate and efficient framework for real-space Hubbard-corrected density functional theory. In particular, we obtain expressions for the energy, atomic forces, and stress tensor suitable for real-space finite-difference…

Computational Physics · Physics 2025-10-20 Sayan Bhowmik , Andrew J. Medford , Phanish Suryanarayana

Repeated computations on the same molecular system, but with different geometries, are often performed in quantum chemistry, for instance, in ab-initio molecular dynamics simulations or geometry optimizations. While many efficient…

Chemical Physics · Physics 2020-12-02 E. Polack , A. Mikhalev , Geneviève Dusson , B. Stamm , F. Lipparini

We show the power of the algebra of subspace collections developed in Chapter 7 of the book "Extending the Theory of Composites to Other Areas of Science (edited by Milton, 2016). Specifically we accelerate the Fast Fourier Transform…

Numerical Analysis · Mathematics 2020-02-21 Graeme W. Milton

We present an efficient preconditioning technique for accelerating the fixed point iteration in real-space Kohn-Sham density functional theory (DFT) calculations. The preconditioner uses a low rank approximation of the dielectric matrix…

Materials Science · Physics 2023-03-29 Sambit Das , Vikram Gavini

Iterative Fast Fourier Transform methods are useful for calculating the fields in composite materials and their macroscopic response. By iterating back and forth until convergence, the differential constraints are satisfied in Fourier…

Numerical Analysis · Mathematics 2018-01-25 Hervé Moulinec , Pierre Suquet , Graeme W. Milton

The boundary integral method is an efficient approach for solving time-harmonic obstacle scattering problems by a bounded scatterer. This paper presents the directional preconditioner for the iterative solution of linear systems of the…

Numerical Analysis · Mathematics 2014-09-17 Lexing Ying

We present an acceleration method for sequences of large-scale linear systems, such as the ones arising from the numerical solution of time-dependent partial differential equations coupled with algebraic constraints. We discuss different…

Numerical Analysis · Mathematics 2024-03-29 Margherita Guido , Daniel Kressner , Paolo Ricci

Fourier transform-based methods enable accurate, dispersion-free simulations of time-domain scattering problems by evaluating solutions to the Helmholtz equation at a discrete set of frequencies sufficient to approximate the inverse Fourier…

Numerical Analysis · Mathematics 2025-10-29 Oscar P. Bruno , Manuel A. Santana

A new framework is presented for evaluating the performance of self-consistent field methods in Kohn-Sham density functional theory. The aims of this work are two-fold. First, we explore the properties of Kohn-Sham density functional theory…

Computational Physics · Physics 2019-07-18 Nick Woods , Phil Hasnip , Mike Payne

We present preconditioning techniques to solve linear systems of equations with a block two-by-two and three-by-three structure arising from finite element discretizations of the fictitious domain method with Lagrange multipliers. In…

Numerical Analysis · Mathematics 2026-03-09 Michele Benzi , Marco Feder , Luca Heltai , Federica Mugnaioni

Although some preconditioners are available for solving dense linear systems, there are still many matrices for which preconditioners are lacking, in particular in cases where the size of the matrix $N$ becomes very large. There remains…

Numerical Analysis · Mathematics 2016-02-05 Pieter Coulier , Hadi Pouransari , Eric Darve

In this paper, we address the efficient numerical solution of linear and quadratic programming problems, often of large scale. With this aim, we devise an infeasible interior point method, blended with the proximal method of multipliers,…

Numerical Analysis · Mathematics 2021-01-18 Luca Bergamaschi , Jacek Gondzio , Ángeles Martínez , John W. Pearson , Spyridon Pougkakiotis

We present a method to filter a distribution so that it is confined within a sphere of given radius r_c and, simultaneously, whose Fourier transform is optimally confined within a sphere of radius k_c. Our procedure may have several…

Computational Physics · Physics 2009-11-11 Eduardo Anglada , Jose M. Soler

The paper introduces the sweeping preconditioner, which is highly efficient for iterative solutions of the variable coefficient Helmholtz equation including very high frequency problems. The first central idea of this novel approach is to…

Numerical Analysis · Mathematics 2010-08-04 Björn Engquist , Lexing Ying

We introduce an approximate phase-space technique to simulate the quantum dynamics of interacting bosons. With the future goal of treating Bose-Einstein condensate systems, the method is designed for systems with a natural separation into…

Quantum Physics · Physics 2009-11-13 Scott E. Hoffmann , Joel F. Corney , Peter D. Drummond

We perform and extend real-time numerical simulation of a low-dimensional scalar field theory or a quantum mechanical system using stochastic quantization. After a brief review of the quantization method and the complex Langevin dynamics,…

High Energy Physics - Phenomenology · Physics 2015-01-30 Ryoji Anzaki , Kenji Fukushima , Yoshimasa Hidaka , Takashi Oka

An effective means to approximate an analytic, nonperiodic function on a bounded interval is by using a Fourier series on a larger domain. When constructed appropriately, this so-called Fourier extension is known to converge geometrically…

Numerical Analysis · Mathematics 2013-05-14 Ben Adcock , Daan Huybrechs , Jesus Martin-Vaquero