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Half-Heuslers, an emerging thermoelectric material group, has complex bandstructures with multiple bands that can be aligned through band engineering approaches, giving us an opportunity to improve their power factor. In this work, going…

Materials Science · Physics 2019-06-05 Chathurangi Kumarasinghe , Neophytos Neophytou

These compounds have long been known as promising thermoelectric materials. Recently it was revealed, that they also have unconventional electronic topology. This renewed interest to the investigation of their transport properties. In order…

Mesoscale and Nanoscale Physics · Physics 2018-11-14 D. A. Pshenay-Severin , Y. V. Ivanov , A. T. Burkov

The electronic and thermoelectric (TE) transport properties of 13 n-type and p-type half-Heusler alloys are computationally examined using Boltzmann transport. The electronic scattering times resulting from all relevant phonon interactions…

Band convergence is an effective strategy to improve the thermoelectric performance of complex bandstructure thermoelectric materials. Half-Heuslers are good candidates for band convergence studies because they have multiple bands near the…

Materials Science · Physics 2020-11-10 Chathurangi Kumarasinghe , Neophytos Neophytou

We perform an ab initio computational investigation of the electronic and thermoelectric transport properties of one of the best performance half-Heusler (HH) alloys, NbFeSb. We use Boltzmann Transport equation while taking into account the…

Materials Science · Physics 2025-10-28 Bhawna Sahni , Yao Zhao , Zhen Li , Rajeev Dutt , Patrizio Graziosi , Neophytos Neophytou

Recent first-principles electron-phonon scattering calculations of heavily-doped semiconductors suggest that a simple DOS scattering model, wherein the electronic scattering rates are assumed to be proportional to the density-of-states,…

Materials Science · Physics 2020-02-26 Cameron Rudderham , Jesse Maassen

In the field of thermoelectric materials and devices, improving energy conversion efficiency remains a long-standing challenge. As a promising approach to address this issue, utilizing energy-dependent electron-scattering beyond the…

Strongly Correlated Electrons · Physics 2025-11-03 Daiki Goto , Kentaro Kuga , Kiyohisa Tanaka , Tsunehiro Takeuchi , Masaharu Matsunami

Intervalley collisions, which scatter electrons from one valley or band to another, can be detrimental to thermoelectric performance in materials with multiple valleys/bands. In this study, density functional theory is used to investigate…

Materials Science · Physics 2023-02-08 Vahid Askarpour , Jesse Maassen

We have investigated the effect on phonon energy transport in mesoscopic systems and the reduction in the thermal conductance in the quantum limit due to phonon scattering by surface roughness using full 3-dimensional elasticity theory for…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 D. H. Santamore , M. C. Cross

Considering screeening of electron scattering interactions in terms of the finite-temperature STLS theory and solving the linearized Boltzmann equation (with no appeal to a relaxation time approximation), we present a theoretical analysis…

Materials Science · Physics 2011-06-08 S. Y. Liu , X. L. Lei , Norman J. M. Horing

In this work, we employed non-equilibrium Green's function to investigate the electron transport properties in the nanowire with the presence of scatterings. The scattering mechanism is modelled by using the concept of B\"uttiker probe. The…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Jing Li , Tin Cheung Au Yeung , Chan Hin Kam

Materials with ring-shaped electronic bands are promising thermoelectric candidates, since their unusual dispersion shape is predicted to give large power factors. While previous calculations of these materials have relied on the assumption…

Mesoscale and Nanoscale Physics · Physics 2021-04-14 Cameron Rudderham , Jesse Maassen

Both the semi-classical and quantum transport properties of F-doped SnO$_2$ thick films ($\sim$1\,$\mu$m) were investigated experimentally. It is found that the resistivity caused by the thermal phonons obeys Bloch-Gr\"{u}neisen law from…

Materials Science · Physics 2014-08-06 Wen-Jing Lang , Zhi-Qing Li

Improvement of numerical methods for calculating charge transport quantities of materials from the Boltzmann transport equation (BTE) is important for prediction of material properties. In particular, techniques which allow for more…

Materials Science · Physics 2025-08-25 H. A. McDonough , Nicholas A. Mecholsky

We present systematic theoretical results on thermoelectric effects in semimetals based on the variational method of the linearized Boltzmann equation. Inelastic electron-hole scattering is known to play an important role in the unusual…

Strongly Correlated Electrons · Physics 2023-03-31 Keigo Takahashi , Hiroyasu Matsuura , Hideaki Maebashi , Masao Ogata

To increase the performance of thermoelectric materials, the electronic parameters in the figure of merit must be improved. In this paper, we use full, numerical band structures and solve the Boltzmann equation in the relaxation time…

Materials Science · Physics 2018-12-17 Evan Witkoske , Xufeng Wang , Jesse Maassen , Mark Lundstrom

Relaxor ferroelectrics are difficult to study and understand. The experiment shows that at low energy scattering there is an acoustic mode, an optic mode, dynamic quasi-elastic scattering and strictly elastic scattering as well as Bragg…

Materials Science · Physics 2008-08-29 R. A. Cowley , S. N. Gvasaliya , B. Roessli

Recent discovery of new materials for thermoelectric energy conversion is enabled by efficient prediction of materials' performance from first-principles, without empirically fitted parameters. The novel simplified approach for computing…

Materials Science · Physics 2018-05-02 Georgy Samsonidze , Boris Kozinsky

The effect of phonon scattering by surface roughness on the thermal conductance in mesoscopic systems at low temperatures is calculated using full elasticity theory. The low frequency behavior of the scattering shows novel power law…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 D. H. Santamore , M. C. Cross

Traditional thermoelectric materials rely on low thermal conductivity to enhance their efficiency but suffer from inherently limited power factors. Novel pathways to optimize electronic transport are thus crucial. Here, we achieve ultrahigh…

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