Related papers: Robust and highly-efficient discrimination of chir…
Chiral light matter interaction enables new fundamental researches and applications of light. The interaction has traditionally faced challenges in low directionality and efficiency based on spin orbit interaction of light in microscopic…
High-dimensional encoding and hyper-entanglement are unique features that distinguish optical photons from other quantum information carriers, leading to improved system efficiency and novel quantum functions. However, the disparate…
In reaction path optimization, such as the calculation of a minimum energy path (MEP) between given reactant and product configurations of atoms, it is advantageous to start with an initial guess where close proximity of atoms is avoided…
Determination of enantiomeric excess is important and remains challenges. We theoretically propose a new spectroscopic method for this issue based on the chirality-dependent AC Stark effects in cyclic three-level models under the…
Size and shape are critical discriminators between molecular species and states. We describe a micro-chip based high-throughput imaging approach offering rapid and precise determination of molecular properties under native solution…
We present a comprehensive overview of chirality and its optical manifestation in plasmonic nanosystems and nanostructures. We discuss top-down fabricated structures that range from solid metallic nanostructures to groupings of metallic…
We explore a pure optical method for enantioselective orientation of chiral molecules by means of laser fields with twisted polarization. Several field implementations are considered, including a pair of delayed cross-polarized laser…
Chiral excited electronic states of molecules have an intrinsic sense of handedness, or twist, and are the active component in energy efficient display technologies and in new photosynthetic routes to produce pharmaceuticals. Creating…
Dynamic encircling a second-order exception point (EP) exhibit chiral state transfer, while there is few research on dynamic encircling multiple and higher-order EPs. Here, we study proximity-encirclement of the EPs in a multimode…
Enantioselective orientation of chiral molecules excited by a shaped picosecond laser pulse and a delayed femtosecond pulse is considered. Using quantum mechanical simulations, we demonstrate a strong field-free enantioselective orientation…
Enantioselective interactions of chiral molecules include distinct absorptions to opposite-handed circularly polarized light, known as chiral absorption. Traditionally, chiral absorption has been primarily attributed to electric dipole and…
We propose a gain-assisted enantioselective scheme in dye-doped chiral particles, demonstrating optical pulling and pushing forces that can be tuned using externally controllable parameters. By controlling the concentration of dye molecules…
A STIRAP-like scheme is proposed to exploit a three-photon resonance taking place in alkaline-earth-metal ions. This scheme is designed for state transfer between the two fine structure components of the metastable D-state which are two…
We propose to realize the two-mode continuous-variable entanglement of microwave photons in an electro-optic system, consisting of two superconducting microwave resonators and one or two optical cavities filled with certain electro-optic…
Stimulated Raman Adiabatic Passage (STIRAP) and its variants, such as multi-state chainwise-STIRAP allow efficiently transferring the populations in multi-state system and have been widely used to prepare ultracold deeply-bound molecules.…
Optical forces can be chiral when they exhibit opposite signs for the two enantiomeric versions of a chiral molecule or particle. Such forces could be eventually used to separate enantiomers, which could find application in numerous…
Coherent control of ultrafast molecule making from colliding reactants is crucial for realizing coherent control of binary photoreactions (CCBP). To handle diverse excitation scenarios, feasibility with both weak and strong fields is…
We consider a photonic crystal (PC) doped with four-level atoms whose intermediate transition is coupled near-resonantly with a photonic band-gap edge. We show that two photons, each coupled to a different atomic transition in such atoms,…
We predict a discriminatory interaction between a chiral molecule and an achiral molecule which is mediated by a chiral body. To achieve this, we generalize the van der Waals interaction potential between two ground-state molecules with…
Chiroptical enantioselective sensing is gaining traction across various applications. However, intrinsic molecular chiroptical responses are weak, and existing amplification approaches add synthesis, manufacturing, or operational complexity…