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A size-extensive, converging, black-box, ab initio coupled-cluster ($\Delta$CC) ansatz is introduced that computes the energies and wave functions of stationary states from any degenerate or nondegenerate Slater-determinant references with…

Chemical Physics · Physics 2026-05-15 So Hirata

We present an efficient implementation of the Generalized Green's function Cluster Expansion (GGCE), which is a new method for computing the ground-state properties and dynamics of polarons (single electrons coupled to lattice vibrations)…

Computational Physics · Physics 2023-10-16 Matthew R. Carbone , Stepan Fomichev , Andrew J. Millis , Mona Berciu , David R. Reichman , John Sous

We show how to use the input-output formalism compute the propagator for an open quantum system, i.e. quantum networks with a low dimensional quantum system coupled to one or more loss channels. The total propagator is expressed entirely in…

Quantum Physics · Physics 2018-11-02 Rahul Trivedi , Kevin Fischer , Shanshan Xu , Shanhui Fan , Jelena Vuckovic

In classical computational chemistry, the coupled-cluster ansatz is one of the most commonly used $ab~initio$ methods, which is critically limited by its non-unitary nature. The unitary modification as an ideal solution to the problem is,…

Quantum Physics · Physics 2017-03-01 Yangchao Shen , Xiang Zhang , Shuaining Zhang , Jing-Ning Zhang , Man-Hong Yung , Kihwan Kim

We propose a novel model-reduction methodology for large-scale dynamic networks with tightly-connected components. First, the coherent groups are identified by a spectral clustering algorithm on the graph Laplacian matrix that models the…

Systems and Control · Electrical Eng. & Systems 2022-10-04 Hancheng Min , Enrique Mallada

Dynamical quantum-cluster approaches, such as different cluster extensions of the dynamical mean-field theory (cluster DMFT) or the variational cluster approximation (VCA), combined with efficient cluster solvers, such as the quantum…

Strongly Correlated Electrons · Physics 2013-05-29 Gang Li , Werner Hanke , Alexei N. Rubtsov , Sebastian Bäse , Michael Potthoff

We present the concept, derivation, and implementation of dynamical configuration interaction, a quantum embedding theory that combines Green's function methodology with the many-body wave function. In a strongly-correlated active space, we…

Chemical Physics · Physics 2019-04-03 Marc Dvorak , Patrick Rinke

Double--folded optical $\alpha$--nucleus potentials can be used to calculate elastic scattering cross sections in a wide mass-- and energy region. Because of the systematic behavior of the potential parameters we are able to obtain reliable…

Nuclear Theory · Physics 2009-09-25 P. Mohr , H. Abele , U. Atzrott , G. Staudt , R. Bieber , K. Grün , H. Oberhummer , T. Rauscher , E. Somorjai

Embedding theories became important approaches used for accurate calculations of both molecules and solids. In these theories, a small chosen subset of orbitals is treated with an accurate method, called an impurity solver, capable of…

Chemical Physics · Physics 2023-03-20 Avijit Shee , Chia-Nan Yeh , Bo Peng , Karol Kowalski , Dominika Zgid

I introduce several simplified schemes for the approximation of the self-consistency condition of the dynamical cluster approximation. The applicability of the schemes is tested numerically using the fluctuation-exchange approximation as a…

Strongly Correlated Electrons · Physics 2012-04-25 J. P. Hague

We have developed an approach to calculate the single-particle Green function of a one-dimensional many-body system in the strongly localized limit at zero temperature. Our approach, based on the locator expansion, sums the contributions of…

Mesoscale and Nanoscale Physics · Physics 2017-05-05 A. N. Somoza , M. Ortuño , V. Gasparian , M. Pino

Coupled-cluster theory is a powerful tool for first-principles calculations of atomic nuclei, enabling accurate predictions of nuclear observables across the Segr\`e chart. While coupled-cluster computations are especially efficient at…

Nuclear Theory · Physics 2026-04-08 F. Marino , F. Bonaiti , P. Demol , S. Bacca , T. Duguet , G. Hagen , G. R. Jansen , T. Papenbrock , A. Tichai

We present and benchmark a quantum computing approach to calculate the two-dimensional coherent spectrum (2DCS) of high-spin models. Our approach is based on simulating their real-time dynamics in the presence of several magnetic field…

Quantum Physics · Physics 2024-07-02 Martin Mootz , Peter P. Orth , Chuankun Huang , Liang Luo , Jigang Wang , Yong-Xin Yao

We examine whether essence and quantitative aspects of electronic excitation spectra are correctly captured by an effective low-energy model constructed from an {\em ab initio} downfolding scheme. A global electronic structure is first…

Strongly Correlated Electrons · Physics 2009-11-13 Kazuma Nakamura , Yoshihide Yoshimoto , Ryotaro Arita , Shinji Tsuneyuki , Masatoshi Imada

This paper examines the effectiveness of the Dyson-Schwinger (DS) equations as a calculational tool in quantum field theory. The DS equations are an infinite sequence of coupled equations that are satisfied exactly by the connected Green's…

Mathematical Physics · Physics 2023-03-29 Carl M. Bender , Christos Karapoulitidis , S. P. Klevansky

We formulate an ab initio downfolding scheme for electron-phonon coupled systems. In this scheme, we calculate partially renormalized phonon frequencies and electron-phonon coupling, which include the screening effects of high-energy…

Strongly Correlated Electrons · Physics 2015-12-10 Yusuke Nomura , Ryotaro Arita

We present a real-time second-order Green's function (GF) method for computing excited states in molecules and nanostructures, with a computational scaling of $O(N_{\rm e}^3$), where $N_{\rm e}$ is the number of electrons. The cubic scaling…

Chemical Physics · Physics 2024-01-29 Leopoldo Mejía , Jia Yin , David R. Reichman , Roi Baer , Chao Yang , Eran Rabani

We present a new charge self-consistent scheme combining Density Functional and Dynamical Mean Field Theory, which uses Green's function of multiple scattering-type. In this implementation the many-body effects are incorporated into the…

Strongly Correlated Electrons · Physics 2017-10-11 A. Östlin , L. Vitos , L. Chioncel

The aim of this work is to outline in some detail the use of combinatorial algebra in planar quantum field theory. Particular emphasis is given to the relations between the different types of planar Green's functions. The key object is a…

Mathematical Physics · Physics 2016-08-16 Kurusch Ebrahimi-Fard , Frederic Patras

Hybrid spectral-spatial representations are introduced to rapidly calculate periodic scalar and dyadic Green's functions of the Helmholtz equation for 2D and 3D configurations with a 1D (linear) periodicity. The presented schemes work…

Computational Physics · Physics 2015-05-13 Derek Van Orden , Vitaliy Lomakin