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The ferrimagnetic insulator Mn3Si2Te6, which features a Curie temperature Tc at 78 K and a delicate yet consequential magnetic frustration, exhibits colossal magnetoresistance (CMR) when the magnetic field is applied along the magnetic hard…

Strongly Correlated Electrons · Physics 2022-11-02 Feng Ye , Masaaki Matsuda , Zachary Morgan , Todd Sherline , Yifei Ni , Hengdi Zhao , G. Cao

The gigantic decrease of resistance by an applied magnetic field, which is often referred to as colossal magnetoresistance (CMR), has been an attracting phenomenon in strongly correlated electron systems. The discovery of CMR in manganese…

Strongly Correlated Electrons · Physics 2019-09-25 S. Yamada , N. Abe , H. Sagayama , K. Ogawa , T. Yamagami , T. Arima

The ordered double perovskites Sr2CrOsO6 and Ca2CrOsO6 have been synthesized and characterized with neutron powder diffraction, electrical transport measurements, and high field magnetization experiments. Sr2CrOsO6 and Ca2CrOsO6 crystallize…

Magnetic double perovskite compounds provide a fertile playground to explore interesting electronic and magnetic properties. By complementary macroscopic characterizations, neutron powder diffraction measurements and first-principles…

Strongly Correlated Electrons · Physics 2024-04-03 Cheng Su , Xu-Tao Zeng , Kaitong Sun , Denis Sheptyakov , Ziyu Chen , Xian-Lei Sheng , Haifeng Li , Wentao Jin

Coupling between different interactions allows to control physical aspects in multifunctional materials by perturbing any of the degrees of freedom. Here, we aim to probe the correlation among structural, electronic and magnetic observables…

Materials Science · Physics 2025-07-28 S. Majumder , M. Tripathi , D. O. de Souza , A. Sagdeo , L. Olivi , M. N. Singh , S. Pal , R. J. Choudhary , D. M. Phase

Materials with strong magnetoresistive responses are the backbone of spintronic technology, magnetic sensors, and hard drives. Among them, manganese oxides with a mixed valence and a cubic perovskite structure stand out due to their…

The magnetic susceptibility, crystal and magnetic structures, and electronic structure of double perovskite Sr2ScOsO6 are reported. Using both neutron and x-ray powder diffraction we find that the crystal structure is monoclinic P21/n from…

Strongly Correlated Electrons · Physics 2015-04-06 A. E. Taylor , R. Morrow , D. J. Singh , S. Calder , M. D. Lumsden , P. M. Woodward , A. D. Christianson

The double-perovskite A$_2$BB'O$_6$ with heavy transition metal ions on the ordered B' sites is an important family of compounds to study the interplay between electron correlation and spin-orbit coupling (SOC). Here we prepared…

Strongly Correlated Electrons · Physics 2020-07-01 Shang Gao , Daigorou Hirai , Hajime Sagayama , Hiroyuki Ohsumi , Zenji Hiroi , Taka-hisa Arima

We present a comprehensive study on the magnetic structure, dynamics, and phase evolution in the single-phase double perovskite $La_2CoMnO_6$. The mixed valence state due to oxygen deficiency is verified by X-ray photoelectron spectroscopy,…

In order to gain insights into the origin of colossal magneto-resistance (CMR) in manganese oxides, we performed a ^{139}La NMR study in the double-layered compound La_{1.2}Sr_{1.8}Mn_2O_7. We find that above the Curie temperature T_C=126…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Shiotani , J. L. Sarrao , Guo-qing Zheng

The magnetic structure of Ca$_2$MnReO$_6$ double perovskite is investigated by neutron powder diffraction and bulk magnetization, showing dominant non-collinear Mn magnetic moments [$4.35(7)$ $\mu_B$] that are orthogonally aligned with the…

Strongly Correlated Electrons · Physics 2018-03-01 A. S. Cavichini , M. T. Orlando , J. B. Depianti , J. L. Passamai , F. Damay , F. Porcher , E. Granado

The electron spin polarization on half-metallic double-perovskites is usually conditioned to the ordered rock-salt arrangement of the transition-metal ions along the lattice. In this work, we investigate a polycrystalline sample of the…

The rise of high-entropy oxides as a major functional materials design principle in recent years has prompted us to investigate how compositional disorder affects long-range magnetic ordering in double perovskite oxides. Since ferromagnetic…

Colossal magnetoresistance (CMR) is commonly observed in magnetic semiconductors when an external magnetic field is applied, usually accompanied by anomalous resistivity peaks or humps which were previously considered as evidence of a…

Materials Science · Physics 2025-03-26 Zhihao Liu , Zhong Fang , Hongming Weng , Quansheng Wu

Room-temperature ferrimagnetism was discovered for the anti-site-disordered perovskite Ca2MnOsO6 with Tc = 305 K. Ca2MnOsO6 crystallizes into an orthorhombic structure with a space group of Pnma, in which Mn and Os share the…

Recent experiments suggest a new paradigm towards novel colossal magnetoresistance (CMR) in a family of materials EuM$_2$X$_2$(M=Cd, In, Zn; X=P, As), distinct from the traditional avenues involving Kondo-RKKY crossovers, magnetic phase…

The magnetic correlations in double perovskites La2Mn2-xNixO6 (x = 0.5, 0.75, 1.0, 1.25 and 1.5) have been systematically investigated across macroscopic, mesoscopic, and microscopic length scales using temperature-dependent bulk DC…

Materials Science · Physics 2025-10-14 A. K. Bera , K. S. Chikara , B. Saha , S. M. Yusuf , Mohd. Nasir , S. Sen

Recent reports of colossal negative magnetoresistance (CMR) in a few magnetic semimetals and semiconductors have attracted attention, because these materials are devoid of the conventional mechanisms of CMR such as mixed valence, double…

The magnetism of ordered and disordered La$_2$NiMnO$_6$ is explained using a model involving double exchange and superexchange. The concept of majority spin hybridization in the large coupling limit is used to explain the ferromagnetism of…

Strongly Correlated Electrons · Physics 2017-12-13 Prabuddha Sanyal

The functional characteristics of double perovskites with unique ferromagnetic-insulator ground state have been controversial due to the unavoidable presence of anti-site disorders (ASDs). Here, we aim to investigate the origin of magnetic…

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