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Single- and few-layer chromium triiodide (CrI3), which has been intensively investigated as a promising platform for two-dimensional magnetism, was usually prepared by mechanical exfoliation. Here, we report on the growth of single-layer…

Materials Science · Physics 2020-07-16 Peigen Li , Cong Wang , Jihai Zhang , Shenwei Chen , Donghui Guo , Wei Ji , Dingyong Zhong

We present results of comprehensive first-principles and kp-method studies of electronic, magnetic, and topological properties of graphene on a monolayer of CrI$_3$. First, we identify a twist angle between the graphene and CrI$_3$, that…

Mesoscale and Nanoscale Physics · Physics 2025-09-16 M. Jafari , M. Gmitra , A. Dyrdał

Bulk chromium triiodide (CrI$_3$) has long been known as a layered van der Waals ferromagnet. However, its monolayer form was only recently isolated and confirmed to be a truly two-dimensional (2D) ferromagnet, providing a new platform for…

After the discovery of magnetism in monolayer CrI3, the magnetic properties of different 2D materials from the chromium-trihalide family are intuitively assumed to be similar, yielding magnetic anisotropy from the spin-orbit coupling on…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 C. Bacaksiz , D. Šabani , R. M. Menezes , M. V. Milošević

Few-layer CrI$_3$ is the most known example among two-dimensional (2D) ferromagnets, which have attracted growing interest in recent years. Despite considerable efforts and progress in understanding the properties of 2D magnets both from…

Strongly Correlated Electrons · Physics 2021-01-14 I. V. Kashin , V. V. Mazurenko , M. I. Katsnelson , A. N. Rudenko

The challenge of controlling magnetism using electric fields raises fundamental questions and addresses technological needs such as low-dissipation magnetic memory. The recently reported two-dimensional (2D) magnets provide a new system for…

Two-dimensional (2D) magnetic materials offer unprecedented opportunities for fundamental physics and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2Ge2Te6, this emerging field has expanded to…

CrI3 is a layered ferromagnetic insulator that has recently attracted enormous interest as it was the first example of a stand-alone monolayer ferromagnet, paving the way towards the study of two-dimensional magnetic materials and their use…

Commensurable twisted bilayers can drastically change the magnetic properties of chromium trihalide layered compounds, which opens novel opportunities for tuning magnetic states through layer rotations. Here, we introduce a mathematical…

Materials Science · Physics 2022-01-06 A. M. León , E. A. Velásquez , F. Caro-Lopera , J. Mejía-López

Magnons dominate the magnetic response of the recently discovered insulating ferromagnetic two dimensional crystals such as CrI$_3$. Because of the arrangement of the Cr spins in a honeycomb lattice, magnons in CrI$_3$ bear a strong…

Mesoscale and Nanoscale Physics · Physics 2020-02-04 A. T. Costa , D. L. R. Santos , N. M. R. Peres , J. Fernández-Rossier

Layered antiferromagnetism is the spatial arrangement of ferromagnetic layers with antiferromagnetic interlayer coupling. Recently, the van der Waals magnet, chromium triiodide (CrI3), emerged as the first layered antiferromagnetic…

Two-dimensional honeycomb lattice ferromagnet chromium tri-iodide (CrI$_3$) has attracted tremendous interest because it retains ferromagnetism down to the monolayer limit and hosts intriguing topological magnons. As a prototypical van der…

Materials Science · Physics 2026-05-08 Weiliang Yao , Matthew B. Stone , Colin L. Sarkis , Yi Li , Ruixian Liu , Xingye Lu , Pengcheng Dai

We present a detailed study on the microscopic origin of magnetism in suspended and dielectrically embedded CrI$_3$ monolayer. To this end, we down-fold two distinct minimal generalized Hubbard models with different orbital basis sets from…

Strongly Correlated Electrons · Physics 2021-10-06 D. Soriano , A. N. Rudenko , M. I. Katsnelson , M. Rösner

Manipulating physical properties using the spin degree of freedom constitutes a major part of modern condensed matter physics and is very important for spintronics devices. Using the newly discovered two dimensional van der Waals…

Materials Science · Physics 2018-05-29 Peiheng Jiang , Lei Li , Zhaoliang Liao , Y. X. Zhao , Zhicheng Zhong

The integration of diverse electronic phenomena, such as magnetism and nontrivial topology, into a single system is normally studied either by seeking materials that contain both ingredients, or by layered growth of contrasting materials.…

Motivated by the potential of atomically-thin magnets towards tunable high-frequency magnonics, we detail the spin-wave dispersion of bilayer CrI$_3$. We demonstrate that the magnonic behavior of the bilayer strongly depends on its stacking…

Materials Science · Physics 2023-03-01 M. Soenen , C. Bacaksiz , R. M. Menezes , M. V. Milosevic

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

CrI3, which belongs to a rare category of two-dimensional (2D) ferromagnetic semiconductors, is of great interest for spintronic device applications. Unlike CrCl3 whose magnetism presents a 2D-Heisenberg behavior, CrI3 exhibits a larger van…

Materials Science · Physics 2018-03-14 G. T. Lin , X. Luo , F. C. Chen , J. Yan , J. J. Gao , Y. Sun , W. Tong , P. Tong , W. J. Lu , Z. G. Sheng , W. H. Song , X. B. Zhu , Y. P. Sun

By exploiting proximity coupling, we probe the spin state of the surface layers of CrI3, a van der Waals magnetic semiconductor, by measuring the induced magnetoresistance (MR) of Pt in Pt/CrI3 nano-devices. We fabricate the devices with…

Mesoscale and Nanoscale Physics · Physics 2020-06-19 Tang Su , Mark Lohmann , Junxue Li , Yadong Xu , Ben Niu , Mohammed Alghamdi , Haidong Zhou , Yongtao Cui , Ran Cheng , Takashi Taniguchi , Kenji Watanabe , Jing Shi

In this letter, we report the visualization of topologically protected spin textures, in the form of magnetic skyrmions, in recently discovered monoatomic-thin two-dimensional CrI$_3$. By combining density functional theory and atomistic…

Materials Science · Physics 2019-07-24 Aroop K. Behera , Sugata Chowdhury , Suprem R. Das