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Tree tensor network states (TTNSs) combined with the density matrix renormalization group (DMRG) are emerging as powerful tools for vibrational and vibronic structure simulations in molecules with strong coupling and fluxionality. In this…

Chemical Physics · Physics 2026-05-28 Henrik R. Larsson , Brieuc Le Dé , Gino E. Gamboni

We develop and employ general Tree Tensor Networks (TTNs) to compute the vibrational spectra for two model systems: a set of 64-dimensional coupled oscillators and acetonitrile. We explore various tree architectures, ranging from the simple…

Chemical Physics · Physics 2025-12-19 Shuo Sun , Richard M. Milbradt , Stefan Knecht , Chandan Kumar , Christian B. Mendl

Accurate vibrational spectra are essential for understanding how molecules behave, yet their computation remains challenging and benchmark data to reliably compare different methods are sparse. Here, we present high-accuracy eigenstate…

Chemical Physics · Physics 2025-04-16 Henrik R. Larsson

Tree tensor network states (TTNS) decompose the system wavefunction to the product of low-rank tensors based on the tree topology, serving as the foundation of the multi-layer multi-configuration time-dependent Hartree (ML-MCTDH) method. In…

Quantum Physics · Physics 2024-08-29 Weitang Li , Jiajun Ren , Hengrui Yang , Haobin Wang , Zhigang Shuai

The multilayer multiconfiguration time-dependent Hartree (ML-MCTDH) method and the density matrix renormalization group (DMRG) are powerful workhorses applied mostly in different scientific fields. Although both methods are based on tensor…

Chemical Physics · Physics 2024-09-05 Henrik R. Larsson

We propose a new algorithm for calculation of vibrational spectra of molecules using tensor train decomposition. Under the assumption that eigenfunctions lie on a low-parametric manifold of low-rank tensors we suggest using well-known…

Numerical Analysis · Mathematics 2016-10-12 Maxim Rakhuba , Ivan Oseledets

To understand the dynamics of quantum many-body systems, it is essential to study excited eigenstates. While tensor network states have become a standard tool for computing ground states in computational many-body physics, obtaining…

Chemical Physics · Physics 2025-10-24 Madhumita Rano , Henrik R. Larsson

We present a new variational tree tensor network state (TTNS) ansatz, the three-legged tree tensor network state (T3NS). Physical tensors are interspersed with branching tensors. Physical tensors have one physical index and at most two…

Strongly Correlated Electrons · Physics 2018-06-26 Klaas Gunst , Frank Verstraete , Sebastian Wouters , Örs Legeza , Dimitri Van Neck

We investigate tree tensor network states for quantum chemistry. Tree tensor network states represent one of the simplest generalizations of matrix product states and the density matrix renormalization group. While matrix product states…

Strongly Correlated Electrons · Physics 2013-04-09 Naoki Nakatani , Garnet Kin-Lic Chan

Matrix product states (MPS), a tensor network designed for one-dimensional quantum systems, has been recently proposed for generative modeling of natural data (such as images) in terms of `Born machine'. However, the exponential decay of…

Machine Learning · Statistics 2019-05-13 Song Cheng , Lei Wang , Tao Xiang , Pan Zhang

Numerical methods based on tensor networks have been extensively explored in the research of quantum many-body systems in recent years. It has been recognized that the ability of tensor networks to describe a quantum many-body state…

Statistical Mechanics · Physics 2025-11-19 Toshiya Hikihara , Hiroshi Ueda , Kouichi Okunishi , Kenji Harada , Tomotoshi Nishino

Given in the title are two algorithms to compute the extreme eigenstate of a high-dimensional Hermitian matrix using the tensor train (TT) / matrix product states (MPS) representation. Both methods empower the traditional alternating…

Numerical Analysis · Mathematics 2014-12-02 Sergey V. Dolgov , Dmitry V. Savostyanov

We present an approach based upon binary tree tensor network (BTTN) states for computing steady-state current statistics for a many-particle 1D ratchet subject to volume exclusion interactions. The ratcheted particles, which move on a…

Statistical Mechanics · Physics 2023-01-02 Nils E. Strand , Hadrien Vroylandt , Todd R. Gingrich

Tensor network states are an indispensable tool for the simulation of strongly correlated quantum many-body systems. In recent years, tree tensor network states (TTNS) have been successfully used for two-dimensional systems and to benchmark…

Quantum Physics · Physics 2026-01-23 Thomas Barthel

We introduce an adaptive-weighted tree tensor network, for the study of disordered and inhomogeneous quantum many-body systems. This ansatz is assembled on the basis of the random couplings of the physical system with a procedure that…

Disordered Systems and Neural Networks · Physics 2022-06-07 Giovanni Ferrari , Giuseppe Magnifico , Simone Montangero

An augmented tree tensor network (aTTN) is a tensor network ansatz constructed by applying a layer of unitary disentanglers to a tree tensor network. The disentanglers absorb a part of the system's entanglement. This makes aTTNs suitable…

Quantum Physics · Physics 2025-07-30 Nora Reinić , Luka Pavešić , Daniel Jaschke , Simone Montangero

Tensor Network States (TNS) offer an efficient representation for the ground state of quantum many body systems and play an important role in the simulations of them. Numerous TNS are proposed in the past few decades. However, due to the…

Quantum Physics · Physics 2022-06-28 Xiangjian Qian , Mingpu Qin

Tensor networks, such as matrix product states (MPS) and tree tensor network states (TTNS), are powerful ans\"atze for simulating quantum dynamics. While both ans\"atze are theoretically exact in the limit of large bond dimensions, [J.…

Chemical Physics · Physics 2025-12-15 Weitang Li , Jiajun Ren , Jun Yan

We investigate the disordered spin-$\frac12$Heisenberg model in two dimensions and employ tree tensor networks (TTNs) with a physics-informed structural optimization of the tree layout, to simulate dynamics in the many-body localization…

Disordered Systems and Neural Networks · Physics 2025-12-23 Lars Humpert , Dante M. Kennes , Jan-Niklas Herre

Hybrid Tensor Networks (hTN) offer a promising solution for encoding variational quantum states beyond the capabilities of efficient classical methods or noisy quantum computers alone. However, their practical usefulness and many…

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