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The structural and magnetic properties of double perovskiteTb2CoMnO6 have been investigated. Electronic structure analysis by XPS study reveals the presence of mixed oxidation state (Mn4+/Mn3+ and Co2+/Co3+) of B-site ions. The dc and ac…

Materials Science · Physics 2019-10-31 Khyati Anand , Arkadeb Pal , Prajyoti Singh , Md. Alam , Amish G Joshi , Anita Mohan , Sandip Chatterjee

Double perovskite (DP) oxide material receive extensive research interest due to exciting physical properties with potential technological application. 3$d$ based DP oxides are promising for exciting physics like magnetodielectric,…

Strongly Correlated Electrons · Physics 2019-04-26 Ilyas Noor Bhatti , Rabindra Nath Mahato , Imtiaz Noor Bhatti , M. A. H. Ahsan

We present a comprehensive study on the magnetic structure, dynamics, and phase evolution in the single-phase double perovskite $La_2CoMnO_6$. The mixed valence state due to oxygen deficiency is verified by X-ray photoelectron spectroscopy,…

The Griffiths phase-like features and the spin-phonon coupling effects observed in Tb$_2$NiMnO$_6$ are reported. The double perovskite compound crystallizes in monoclinic $P2_1/n$ space group and exhibits a magnetic phase transition at $T_c…

Strongly Correlated Electrons · Physics 2015-06-03 Harikrishnan S. Nair , Diptikanta Swain , Hariharan N. , Shilpa Adiga , Chandrabhas Narayana , Suja Elizabeth

We report here a comprehensive study on structural, magnetic, caloric and electronic properties of the monoclinic phase of double perovskite compound Tm2CoMnO6 (TCMO) in its polycrysttaline format. Magnetic measurements confirm the presence…

Materials Science · Physics 2023-07-13 A. Banerjee , Gangadhar Das , V. Rajaji , S. Majumdar , P. K. Chakrabarti

We report structural, magnetic, and Raman studies of the disordered double perovskite GdSrCoMnO$_{6}$~(GSCM). DC magnetization shows a ferromagnetic transition at $T_{C} \approx 153$~K. The inverse susceptibility exhibits a downturn above…

Combining experimental investigations and first-principles DFT calculations, we report physical and magnetic properties of Gd-substituted Y$_2$CoMnO$_6$ double perovskite, which are strongly influenced by antisite-disorder-driven spin…

Materials Science · Physics 2023-02-28 Anasua Khan , Sarita Rajput , M. Anas , V. K. Malik , T. Maitra , T. K Nath , A. Taraphder

The field of double perovskites is now advancing to three magnetic elements on the A, B and B$'$ sites. A series of iridium-based double perovskite compounds, $Ln_2$CoIrO$_6$ ($Ln$ = Eu, Tb, Ho) with three magnetic elements were synthesized…

We report the experimental observation of spin reorientation in the double perovskite Ho$_2$FeCoO$_6$. The magnetic phase transitions in this compound are characterized and studied through magnetization and specific heat, and the magnetic…

The subtle interplay between spin-orbit coupling, exchange interactions, and cation ordering can lead to exotic magnetic states in transition-metal ions. We report a comprehensive study of the Re-based (5$d^1$) ordered double perovskite…

Magnetic properties of an antiferromagnetic double perovskite oxide Ba2CaReO6, where Re6+ (5d1) ions with large spin-orbit coupling are arranged on the face-centered-cubic lattice, are investigated using pulsed high magnetic field up to 66…

The magnetic susceptibility, crystal and magnetic structures, and electronic structure of double perovskite Sr2ScOsO6 are reported. Using both neutron and x-ray powder diffraction we find that the crystal structure is monoclinic P21/n from…

Strongly Correlated Electrons · Physics 2015-04-06 A. E. Taylor , R. Morrow , D. J. Singh , S. Calder , M. D. Lumsden , P. M. Woodward , A. D. Christianson

Double perovskite-based magnets wherein frustration and competition between emergent degrees of freedom are at play can lead to novel electronic and magnetic phenomena. Herein, we report the electronic structure and magnetic properties of…

The magnetism of double perovskites is a complex phenomenon, determined from intra- or interatomic magnetic moment interactions, and strongly influenced by geometry. We take advantage of the complementary length and time scales of the muon…

We report the comprehensive experimental results identifying the magnetic spin ordering and the magnetization dynamics of a double perovskite Pr2CoFeO6 by employing the (dc and ac) magnetization, powder neutron diffraction (NPD) and X-ray…

Exploring new magnetic materials is essential for finding advantageous functional properties such as magnetoresistance, magnetocaloric effect, spintronic functionality, and multiferroicity. Versatile classes of double perovskite compounds…

Strongly Correlated Electrons · Physics 2019-05-03 M. K. Kim , J. Y. Moon , S. H. Oh , D. G. Oh , Y. J. Choi , N. Lee

We investigated the anisotropy of the magnetic and magnetocaloric properties of singlecrystalline double perovskite Tb2CoMnO6, which crystallizes in a monoclinic P21/n structure. Due to dissimilar magnetic anisotropy, the ferromagnetic…

Strongly Correlated Electrons · Physics 2018-12-17 J. Y. Moon , M. K. Kim , D. G. Oh , J. H. Kim , H. J. Shin , Y. J. Choi , N. Lee

We present a comprehensive experimental study of magnetization and magnetocaloric effect (MCE) in double perovskite (DP) materials $R_2$NiMnO$_6$ with $R =$ Pr, Nd, Sm, Gd, Tb, and Dy. While a paramagnetic to ferromagnetic transition, with…

Strongly Correlated Electrons · Physics 2021-12-30 Anzar Ali , Kanika Pasrija , Gyaneshwar Sharma , Sanjeev Kumar , Yogesh Singh

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

Strongly Correlated Electrons · Physics 2016-09-01 W. K. Zhu , J. -C. Tung , W. Tong , L. Ling , M. Starr , J. M. Wang , W. C. Yang , Y. Losovyj , H. D. Zhou , Y. Q. Wang , P. -H. Lee , Y. -K. Wang , Chi-Ken Lu , S. X. Zhang

We report magnetic, transport, neutron diffraction, and muon spin rotation data showing that Pb$_2$CoOsO$_6$, a newly synthesized metallic double-perovskite with a centrosymmetric space group at room temperature, exhibits a continuous…

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