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We introduce in detail our newly developed \textit{ab initio} LDA+Gutzwiller method, in which the Gutzwiller variational approach is naturally incorporated with the density functional theory (DFT) through the "Gutzwiller density functional…

Strongly Correlated Electrons · Physics 2013-05-29 XiaoYu Deng , Lei Wang , Xi Dai , Zhong Fang

A major challenge in creating a quantum computer is to find a quantum system that can be used to implement the qubits. For this purpose, deep centers are prominent candidates, and ab initio calculations are one of the most important tools…

Materials Science · Physics 2017-08-30 Bruno Lucatto , Lucy V. C. Assali , Ronaldo Rodrigues Pela , Marcelo Marques , Lara K. Teles

Ab initio description of point defects in semiconductors, characterized by in-gap states of significant multideterminant character, presents a longstanding theoretical challenge for density functional theory (DFT) methods. In this study, we…

Materials Science · Physics 2024-11-27 Zsolt Benedek , Ádám Ganyecz , Anton Pershin , Viktor Ivády , Gergely Barcza

We present an efficient computational approach to perform real-space electronic structure calculations using an adaptive higher-order finite-element discretization of Kohn-Sham density-functional theory (DFT). To this end, we develop an…

Computational Physics · Physics 2015-06-05 Phani Motamarri , Michael R Nowak , Kenneth Leiter , Jaroslaw Knap , Vikram Gavini

The temperature-induced structural and electronic transformation in VO$_2$ between the monoclinic M1 and tetragonal rutile phases was studied by means of \textit{ab initio} molecular dynamics, based on density functional theory with Hubbard…

Materials Science · Physics 2017-10-11 Dušan Plašienka , Roman Martoňák , Marcus C. Newton

The DFT/vdW-WF2s1 method based on the generation of localized Wannier functions, recently developed to include the van der Waals interactions in the Density Functional Theory and describe adsorption processes on metal surfaces by taking…

Chemical Physics · Physics 2016-04-06 Pier Luigi Silvestrelli , Alberto Ambrosetti

We report a comprehensive electronic structure investigation of the paramagnetic (PM), the large moment antiferromagnetic (LMAF), and the hidden order (HO) phases of URu$_2$Si$_2$. We have performed relativistic full-potential calculations…

Strongly Correlated Electrons · Physics 2015-05-19 P. M. Oppeneer , J. Rusz , S. Elgazzar , M. -T. Suzuki , T. Durakiewicz , J. A. Mydosh

This work presents electronic properties of the kagome metal ScV6Sn6 using de Haas-van Alphen (dHvA) oscillations and density functional theory (DFT) calculations. The torque signal with the applied fields up to 43 T shows clear dHvA…

Electronic structure calculation of atoms and molecules, in the past few decades has largely been dominated by density functional methods. This is primarily due to the fact that this can account for electron correlation effects in a…

Chemical Physics · Physics 2013-07-12 Amlan K. Roy

The LDA+DMFT approach merges conventional band structure theory in the local density approximation (LDA) with a state-of-the-art many-body technique, the dynamical mean-field theory (DMFT). This new computational scheme has recently become…

Strongly Correlated Electrons · Physics 2009-10-31 K. Held , I. A. Nekrasov , N. Blümer , V. I. Anisimov , D. Vollhardt

Tungsten (W) is considered a leading candidate for structural and functional materials in future fusion energy devices. The most attractive properties of tungsten for magnetic and inertial fusion energy reactors are its high melting point,…

Materials Science · Physics 2024-10-15 Yichen Qian , Mark R. Gilbert , Lucile Dezerald , Duc Nguyen-Manh , David Cereceda

We present a formulation and implementation of the DFT+\textit{U} method within the framework of linear combination of numerical atomic orbitals (NAO). Our implementation not only enables single-point total energy and electronic-structure…

Materials Science · Physics 2022-06-29 Xin Qu , Peng Xu , Hong Jiang , Lixin He , Xinguo Ren

Precise and accurate predictions of the two-dimensional (2D) material's fundamental gap are crucial for next-generation flexible electronic and photonic devices. We, therefore, evaluated the predictivity of the GW approach in its several…

Materials Science · Physics 2025-09-25 Miroslav Kolos , František Karlický

We have calculated the ground state electronic structure of He under pressure from 0 to 1500 GPa using both all-electron full-potential and pseudopotential methods based on the density functional theory (DFT). We find that throughout this…

Materials Science · Physics 2012-01-10 W. Xiao , Z. X. Tian , W. T. Geng

The electronic structures of the localized $5f$ systems UTSn (T=Ni, Pd) have been investigated using photoemission spectroscopy (PES). The extracted U $5f$ PES spectra of UTSn (T=Ni, Pd) exhibit a broad peak centered at $\sim 0.3$ eV below…

Materials Science · Physics 2007-05-23 J. -S. Kang , S. C. Wi , J. H. Kim , K. A. McEwen , C. G. Olson , J. H. Shim , B. I. Min

LDA+DMFT method in the framework of the iterative perturbation theory (IPT) with full LDA Hamiltonian without mapping onto the effective Wannier orbitals. We then apply this LDA+DMFT method to ferromagnetic bcc-Fe and fcc-Ni as a test of…

Strongly Correlated Electrons · Physics 2008-09-26 Oki Miura , Takeo Fujiwara

We present a combined density-functional theory and dynamical mean-field theory (DFT+DMFT) study of the full structural phase space of rutile-based vanadium dioxide (VO$_2$), including also the less studied M2 and T phases, using an…

Strongly Correlated Electrons · Physics 2026-03-30 Peter Mlkvik , Nicola A. Spaldin , Claude Ederer

We calculate, via spin density functional theory (SDFT) and exact diagonalization, the eigenstates for electrons in a variety of external potentials, including double and triple dots. The SDFT calculations employ realistic wafer profiles…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Stopa , A. Vidan , T. Hatano , S. Tarucha , R. M. Westervelt

The multi-tier $GW$+EDMFT scheme is an ab-initio method for calculating the electronic structure of correlated materials. While the approach is free from ad-hoc parameters, it requires a selection of appropriate energy windows for…

Strongly Correlated Electrons · Physics 2024-08-15 Ruslan Mushkaev , Francesco Petocchi , Viktor Christiansson , Philipp Werner

We have implemented the $GW$+dynamical mean field theory (DMFT) approach in the Vienna ab initio simulation package. Employing the interaction values obtained from the locally unscreened random phase approximation (RPA), we compare…

Strongly Correlated Electrons · Physics 2014-12-15 Ciro Taranto , Merzuk Kaltak , Nicolaus Parragh , Giorgio Sangiovanni , Georg Kresse , Alessandro Toschi , Karsten Held