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We report the results of the experiment aimed at measuring the mobility of O2- ions in dense argon gas in the temperature range 180 K < T < 300 K. We show that an adequate theoretical description of the data is obtained by using the…

Chemical Physics · Physics 2022-10-05 Armando Francesco Borghesani , Frederic Aitken

We report experimental data of the mobility of O\(_2^-\) ions in argon gas as a function of the density in the temperature range between \(180\,\mbox{K}\le T\le 300\,\mbox{K}\). At the intermediate, though fairly large, densities of the…

Chemical Physics · Physics 2022-02-10 Armando Francesco Borghesani , Frédéric Aitken

We report new measurements of the mobility \(\mu\) of O$_{2}^{-}$ ions in supercritical neon in the range $45\,\mathrm{K}\le T\le 334\,\mathrm{K}$ for number density $N\ge 0.5\,$nm$^{-3}.$ We rationalize the experimental data of all…

Chemical Physics · Physics 2019-03-13 A. F , : , Borghesani , F. Aitken

We report here the results of Molecular Dynamics simulations of the drift mobility of negative oxygen ions in very dense neon gas in the supercritical phase. The simulations relatively well reproduce the trend of the experimental data. The…

Chemical Physics · Physics 2017-02-20 A. F. Borghesani , F. Aitken

New Molecular Dynamics simulations have been carried out in order to get an insight on the physical mechanisms that determine the drift mobility of negative Oxygen ions in very dense Neon gas in the supercritical phase close to the critical…

Chemical Physics · Physics 2017-10-06 A. F. Borghesani , F. Aitken

Using classical molecular dynamics simulations, we investigate the mobility of ions in [Bmim][TFSI], a typical room temperature ionic liquid. Analyzing the trajectories of individual cations and anions, we estimate the time that ions spend…

A two-dimensional fluid model is used to investigate the electron heating dynamics and the production of neutral species in a capacitively coupled radio-frequency micro atmospheric pressure helium plasma jet -- specifically the COST jet --…

Experimental studies of electron mobilities in Neon as a function of the gas density have persistently shown mobilities up to an order of magnitude smaller than expected and predicted. A previously ignored mechanism (gas in--homogeneity…

Atomic Physics · Physics 2009-11-07 A. F. Borghesani , T. F. O'Malley

The investigation of the mobility \(\mu\) of quasi-free electrons in dense, cold helium gas as a function of its density \(N\) is made difficult by the fact that a significant fraction of electrons is localized in low mobility bubbles. The…

Chemical Physics · Physics 2022-02-10 A. F. Borghesani

Atom-in-jellium calculations of the Einstein frequency were used to calculate the mean displacement of an ion over a wide range of compression and temperature. Expressed as a fraction of the Wigner-Seitz radius, the displacement is a…

A new analysis and new Molecular Dynamics (MD) simulations of the measurements of the mobility $\mu_{i}$ of O$_{2}^{-} $ ions in dense supercritical Ar gas are reported. $\mu_{i}$ shows a marked dependence on the distance from the critical…

Plasma Physics · Physics 2011-06-01 A. F. Borghesani

This study provides the first comprehensive analysis of how ion mobility affects electron density and temperature in hypersonic flows. We compare two ion mobility models: one derived from Gupta-Yos cross-sections, and the other from swarm…

Plasma Physics · Physics 2025-01-07 Felipe Martin Rodriguez Fuentes , Bernard Parent

This paper presents a study on the relationship between transport properties and geometric free volume for hard sphere (HS) system in dense fluid region. Firstly, a generic free volume distribution function is proposed based on recent…

Soft Condensed Matter · Physics 2021-02-24 Hongqin Liu

We present a model for electron-ion transport in Warm Dense Matter that incorporates Coulomb coupling effects into the quantum Boltzmann equation of Uehling and Uhlenbeck through the use of a statistical potential of mean force. Although…

Plasma Physics · Physics 2021-06-23 Shane Rightley , S. D. Baalrud

We present a semi-analytical free-energy model aimed at characterizing the thermodynamic properties of dense fluid helium, from the low-density atomic phase to the high-density fully ionized regime. The model is based on a free-energy…

Plasma Physics · Physics 2008-12-18 Christophe Winisdoerffer , Gilles Chabrier

We study the motion of an electron bubble in the zero temperature limit where neither phonons nor rotons provide a significant contribution to the drag exerted on an ion moving within the superfluid. By using the Gross-Clark model, in which…

Other Condensed Matter · Physics 2018-03-21 Alberto Villois , Hayder Salman

We report measurements of excess electron mobility in dense Argon gas at the two temperatures $T=152.15$ and 162.30 K, fairly close to the critical one ($T_c =150.7$ K), as a function of the gas density $N$ up to 14 atoms$\cdot$nm$^{-3}$…

Plasma Physics · Physics 2007-05-23 A. F. Borghesani

A detector has been constructed for measuring ion mobilities of gas mixtures at atmospheric pressure and room temperature. The detector consists of a standard triple GEM amplification region and a drift region where ions drift. A method has…

Instrumentation and Detectors · Physics 2018-07-23 Alexander Deisting , Chilo Garabatos , Alexander Szabo

Mobility is a key parameter for SnO2, which is extensively studied as a practical transparent oxide n-type semiconductor. In experiments, the mobility of electrons in bulk SnO2 single crystals varies from 70 to 260 cm2V-1s-1 at room…

Materials Science · Physics 2022-11-11 Zhen Li , Patrizio Graziosi , Neophytos Neophytou

The oxygen self-diffusion coefficient in UO${_2}$ has been recently studied [Cooper et al. Solid State Ionics 282 (2015) 26-30] over a range of pressures (0-10GPa) and temperatures (300-1900K) by combining molecular dynamics calculations…

Materials Science · Physics 2016-01-25 N. V. Sarlis , E. S. Skordas
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