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The optical nonlinearity of WS2, MoS2 monolayer and few-layer films was investigated using the Z-scan technique with femtosecond pulses from the visible to the near infrared. The dependence of nonlinear absorption of the WS2 and MoS2 films…

In this paper we present a modification to the recently proposed transmission F-scan technique, the differential F-scan technique. In differential F-scan technique the programmed focal distance in the electronic-tunable lens oscillates,…

Applied Physics · Physics 2019-06-26 Edgar Rueda , Juan H. Serna , Abdulatiff Hamad , Hernando Garcia

We have expressed the nonlinear optical absorption of a semiconductor in terms of its linear spectrum. We determined that the two-photon absorption coefficient in a strong DC-electric field of a direct gap semiconductor can be expressed as…

Optics · Physics 2009-11-13 Hernando Garcia , Ramki Kalyanaraman

Two-photon lasers require materials with large two-photon gain (2PG) coefficients and low linear and nonlinear losses. Our previous demonstration of large enhancement of two-photon absorption in semiconductors for very different photon…

We experimentally and theoretically investigate the non-degenerate two-photon absorption coefficient $\beta(\omega_1,\omega_2)$ in the prototypical semiconductor ZnSe. In particular, we provide a comprehensive data set on the dependence of…

Mesoscale and Nanoscale Physics · Physics 2021-08-13 L. Krauss-Kodytek , W. -R. Hannes , T. Meier , C. Ruppert , M. Betz

Non-degenerate two-photon absorption (TPA) is investigated in a nanophotonic silicon waveguide in a configuration such that the dispersion of the nonlinear absorption and refraction cannot be neglected. It is shown that a signal wave can…

Nonlinear transmission of 80 and 140 femtosecond pulsed light with $0.79 \mu m$ wavelength through single walled carbon nanotubes suspended in water containing sodium dodecyl sulphate is studied. Pulse-width independent saturation…

Materials Science · Physics 2009-11-13 N. Kamaraju , Sunil Kumar , Srinivasan Krishnamurthy , Shekhar Guha , A. K. Sood , C. N. R. Rao

Recent theoretical and experimental studies have shown that squeezed states of light can be engineered to enhance the resolution of nonlinear optical measurements. Here, we analyze non-degenerate two-photon absorption signals obtained from…

Quantum Physics · Physics 2025-06-10 Gaurav Shukla , Shahram Panahiyan , Devendra Kumar Mishra , Frank Schlawin

We introduce a toluene-filled fiber platform for two-photon absorption measurements. By confining both the light and molecular sample inside the 5 $\mu$m hollow core of the fiber, we increase the distance over which the nonlinear…

We investigate the nonlinear optical response of a commercial extended-wavelength In$_{0.81}$Ga$_{0.19}$As photodetector. Degenerate two-photon absorption in the mid-infrared range is observed at room temperature using a quantum cascade…

Femtosecond high-order harmonic transient absorption spectroscopy is used to observe electromagnetically induced transparency-like behavior as well as induced absorption in the extreme ultraviolet by laser dressing of the He 2s2p (1Po) and…

Atomic Physics · Physics 2009-11-13 Zhi-Heng Loh , Chris H. Greene , Stephen R. Leone

We utilize the recently demonstrated orders of magnitude enhancement of extremely nondegenerate two-photon absorption in direct-gap semiconductor photodiodes to perform scanned imaging of 3D structures using IR femtosecond illumination…

We present and implement a new scheme for extended multi-channel selective femtosecond coherent control based on symmetry properties of the excitation channels. Here, an atomic non-resonant two-photon absorption channel is coherently…

Atomic Physics · Physics 2008-05-17 Andrey Gandman , Lev Chuntonov , Leonid Rybak , Zohar Amitay

We discuss how two-photon absorption (TPA) of squeezed and coherent states of light can be detected in measurements of the transmitted light fields. Such measurements typically suffer from competing loss mechanisms such as experimental…

Quantum Physics · Physics 2022-05-24 Shahram Panahiyan , Carlos Sánchez Muñoz , Maria V. Chekhova , Frank Schlawin

We analyze optical soliton propagation in the presence of weak absorption lines with much narrower linewidths as compared to the soliton spectrum width using the novel perturbation analysis technique based on an integral representation in…

Optics · Physics 2010-03-25 V. L. Kalashnikov , E. Sorokin

Nonlinear absorption can limit the efficiency of nonlinear optical devices. However, it can also be exploited for optical limiting or switching applications. Thus, characterization of nonlinear absorption in photonic devices is imperative.…

Plasmonic detectors have the potential to provide a method of rapid spectroscopy without the need of moving mirrors or gratings. Previous measurements have demonstrated frequency tunable detection based on plasmonic excitations, however…

Materials Science · Physics 2015-02-09 Che Jin Bae , Deepu George , Rohit Singh , Gottfried Strasser , Andrea Markelz

We present femtosecond pump-probe measurements of the nondegenerate (1960$\,$nm excitation and 1176--1326$\,$nm probe) two-photon absorption spectra of 8 $\,$nm GaAs/12$\,$nm Al$_{0.32}$Ga$_{0.68}$As quantum well waveguides. Experiments…

Multi-photon absorption processes have a nonlinear dependence on the amplitude of the incident optical field i.e. the number of photons. However, multi-photon absorption is generally weak and multi-photon events occur with extremely low…

A simple yet precise optical technique for measuring the ambipolar carrier mobility in semiconductors is presented. Using tightly focused Gaussian laser beams in a photo-reflectance system, the modulated reflectance signal is measured as a…

Instrumentation and Detectors · Physics 2017-11-06 Will Chism
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