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Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…

Optics · Physics 2025-05-14 Sanchayeeta Jana , Simon Durst , Lucas Ludwig , Markus Lippitz

Spectroscopic photoemission microscopy is a well-established method to investigate the electronic structure of surfaces. In modern photoemission microscopes the electron optics allows imaging of the image plane, momentum plane, or…

Photoemission spectroscopy, an experimental method based on the photoelectric effect, is now an indispensable technique used in various fields such as materials science, life science, medicine, and nanotechnology. However, part of the…

Materials Science · Physics 2023-03-20 Takuma Masuda , Masaki Kobayashi , Koji Yatani

Ultrafast pump-probe experiments open the possibility to track fundamental material behaviour like changes in its electronic configuration in real time. To date, most of these experiments are performed using an electron or a high-energy…

The evolution of both information and energy technology is intimately connected to complex condensed matter systems, the properties of which are determined by electronic and chemical interactions and processes on a broad range of length and…

Materials Science · Physics 2015-03-19 Martina Müller , Slavomir Nemsak , Lukasz Plucinski , Claus M. Schneider

Scanning Transmission Electron Microscopy (STEM) coupled with Electron Energy Loss Spectroscopy (EELS) presents a powerful platform for detailed material characterization via rich imaging and spectroscopic data. Modern electron microscopes…

Instrumentation and Detectors · Physics 2024-06-18 Utkarsh Pratiush , Austin Houston , Sergei V Kalinin , Gerd Duscher

Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…

Optics · Physics 2019-11-13 Albert Polman , Mathieu Kociak , F. Javier García de Abajo

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

Ultrafast electron-photon spectroscopy in electron microscopes commonly requires ultrafast laser setups. Photoemission from an engineered electron source is used to generate pulsed electrons, interacting with a sample that is excited by the…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Masoud Taleb , Mario Hentschel , Kai Rossnagel , Harald Giessen , Nahid Talebi

(Scanning) transmission electron microscopy ((S)TEM) has significantly advanced materials science but faces challenges in correlating precise atomic structure information with the functional properties of devices due to its time-intensive…

Techniques in time- and angle-resolved photoemission spectroscopy have facilitated a number of recent advances in the study of quantum materials. We review developments in this field related to the study of incoherent nonequilibrium…

Strongly Correlated Electrons · Physics 2016-10-04 Christopher L. Smallwood , Robert A. Kaindl , Alessandra Lanzara

A novel Bloch-waves based one-step theory of photoemission is developed within the augmented plane wave formalism. Implications of multi-Bloch-wave structure of photoelectron final states for band mapping are established. Interference…

Materials Science · Physics 2009-11-11 E. E. Krasovskii , V. N. Strocov , N. Barrett , H. Berger , W. Schattke , R. Claessen

A phenomenological approach is presented that allows one to model, and thereby interpret, photoemission spectra of strongly correlated electron systems. A simple analytical formula for the self-energy is proposed. This self-energy describes…

Strongly Correlated Electrons · Physics 2009-11-07 Krzysztof Byczuk , Ralf Bulla , Ralph Claessen , Dieter Vollhardt

Electrochemistry workflows utilize various instruments and computing systems to execute workflows consisting of electrocatalyst synthesis, testing and evaluation tasks. The heterogeneity of the software and hardware of these ecosystems…

Distributed, Parallel, and Cluster Computing · Computer Science 2025-01-15 Anees Al-Najjar , Nageswara S. V. Rao , Craig A. Bridges , Sheng Dai , Alex Walters

The electronic properties of two-dimensional (2D) materials depend sensitively on the underlying atomic arrangement down to the monolayer level. Here we present a novel strategy for the determination of the band gap and complex dielectric…

Spectroscopy is a well-established nonintrusive tool that has played an important role in identifying substances and quantifying their compositions, from quantum descriptions to chemical and biomedical diagnostics. Challenges exist in…

Atmospheric and Oceanic Physics · Physics 2020-12-02 S. Yu , Z. Zhang , H. Xia , X. Dou , M. Li , T. Wei , L. Wang , P. Jiang , Y. Wu , C. Zhang , L. You , Y. Hu , T. Wu , L. Zhao , M. Shangguan , L. Tao , J. Qiu

Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…

Optics · Physics 2021-07-07 Szilard Szoke , Manni He , Bryce P. Hickam , Scott K. Cushing

Orchestrating parametric fitting of multicomponent spectra at scale is an essential yet underappreciated task in high-throughput quantification of materials and chemical composition. To automate the annotation process for spectroscopic and…

Materials Science · Physics 2021-03-30 Rui Patrick Xian , Ralph Ernstorfer , Philipp Michael Pelz

Photon emission correlation spectroscopy is an indispensable tool for the study of atoms, molecules, and, more recently, solid-state quantum defects. In solid-state systems, its most common use is as an indicator of single-photon emission,…

Quantum Physics · Physics 2023-11-28 Rebecca E. K. Fishman , Raj N. Patel , David A. Hopper , Tzu-Yung Huang , Lee C. Bassett
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