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We study how time- and angle-resolved photoemission (tr-ARPES) reveals the dynamics of BCS-type, s-wave superconducting systems with time-varying order parameters. Approximate methods are discussed, based on previous approaches to either…

Superconductivity · Physics 2019-01-10 Tianrui Xu , Takahiro Morimoto , Alessandra Lanzara , Joel E. Moore

The interaction of light with a material's electronic system creates an out-of-equilibrium (non-thermal) distribution of optically excited electrons. Non-equilibrium dynamics relaxes this distribution on an ultrafast timescale to a hot…

Strongly Correlated Electrons · Physics 2014-03-05 Søren Ulstrup , Jens Christian Johannsen , Marco Grioni , Philip Hofmann

Time- and angle-resolved photoemission spectroscopy (TR-ARPES) accesses the electronic structure of solids under optical excitation, and is a powerful technique for studying the coupling between electrons and collective modes. One approach…

Motivated by recent experimental progress we revisit the theory of pump-probe time- and angle-resolved photoemission spectroscopy (trARPES), which is one of the most powerful techniques to trace transient pump-driven modifications of the…

Mesoscale and Nanoscale Physics · Physics 2022-01-14 Michael Schüler , Michael A. Sentef

Angle-resolved photoemission spectroscopy (ARPES) -- with its exceptional sensitivity to both the binding energy and momentum of valence electrons in solids -- provides unparalleled insights into the electronic structure of quantum…

Strongly Correlated Electrons · Physics 2024-09-06 Fabio Boschini , Marta Zonno , Andrea Damascelli

In the last decade, there has been a proliferation of laser sources for time- and angle-resolved photoemission spectroscopy (TR-ARPES), building on the proven capability of this technique to tackle important scientific questions. In this…

Optics · Physics 2023-10-26 MengXing Na , Arthur K. Mills , David J. Jones

Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental technique for directly probing electron dynamics in solids. The energy vs. momentum dispersion relations and the associated spectral broadenings measured by ARPES…

Materials Science · Physics 2010-01-19 Cheol-Hwan Park , Feliciano Giustino , Catalin D. Spataru , Marvin L. Cohen , Steven G. Louie

Various technical developments extended the potential of angle-resolved photoemission (ARPES) tremendously during the last twenty years. In particular improved momentum, energy and spin resolution as well as the use of photon energies from…

Materials Science · Physics 2020-07-08 Jan Minar , Sergey Mankovsky , Jurgen Braun , Hubert Ebert

The dynamics of photo-generated electron-hole pairs in solids are dictated by many-body interactions such as electron-electron and electron-phonon scattering. Hence, understanding and controlling these scattering channels is crucial for…

Materials Science · Physics 2016-07-13 Isabella Gierz

Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of non-thermal electrons, a material's dominant…

In pump-probe time and angle-resolved photoemission spectroscopy (TR-ARPES) experiments the presence of the pump pulse adds a new level of complexity to the photoemission process in comparison to conventional ARPES. This is evidenced by…

First-principles methods for time-resolved angular resolved photoelectron spectroscopy play a pivotal role in providing interpretation and microscopic understanding of the complex experimental data and in exploring novel observables or…

Materials Science · Physics 2021-12-28 Umberto De Giovannini , Shunsuke A. Sato , Hannes Hübener , Angel Rubio

The presence of an electrical transport current in a material is one of the simplest and most important realisations of non-equilibrium physics. The current density breaks the crystalline symmetry and can give rise to dramatic phenomena,…

In order to exploit the intriguing optical properties of graphene it is essential to gain a better understanding of the light-matter interaction in the material on ultrashort timescales. Exciting the Dirac fermions with intense ultrafast…

Time- and angle-resolved photoemission spectroscopy (trARPES) is a powerful spectroscopic method to measure the ultrafast electron dynamics directly in momentum-space. However, band gap materials with exceptional strong Coulomb interaction…

Mesoscale and Nanoscale Physics · Physics 2019-12-09 Dominik Christiansen , Malte Selig , Ermin Malic , Ralph Ernstorfer , Andreas Knorr

Angle-resolved photoemission spectroscopy (ARPES) measures the single-particle excitations of a many-body quantum system with both energy and momentum resolution, providing detailed information about strongly interacting materials. ARPES is…

We put forward a first-principle NonEquilibrium Green's Function (NEGF) approach to calculate the transient photoabsorption spectrum of optically thin samples. The method can deal with pump fields of arbitrary strength, frequency and…

Atomic Physics · Physics 2015-09-30 E. Perfetto , A. -M. Uimonen , R. van Leeuwen , G. Stefanucci

In the past decade, the advent of time-resolved spectroscopic tools has provided a new ground to explore fundamental interactions in solids and to disentangle degrees of freedom whose coupling leads to broad structures in the frequency…

The pursuit of a comprehensive understanding of the dynamical nature of intertwined orders in quantum matter has fueled the development of several new experimental techniques, including time- and angle-resolved photoemission spectroscopy…

Superconductivity · Physics 2021-07-21 Marta Zonno , Fabio Boschini , Andrea Damascelli

Pumping graphene with circularly polarized light is the archetype of light-tailoring topological bands. Realizing the induced Floquet-Chern insulator state and tracing clear experimental manifestions has been a challenge, and it has become…

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