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Magnetic insulators are often antiferromagnetic (AFM) and layered AFM compounds usually show low ordering temperature. On the other hand, layered ferromagnetic (FM) insulators with high-TC are very rare although they could be quite useful…

Materials Science · Physics 2018-11-12 Ke Yang , Feng-Ren Fan , Alessandro Stroppa , Hua Wu

Ab initio calculations of the electric polarization of correlation-driven insulating materials, namely Mott insulators, have not been possible so far. Using a combination of density functional theory and dynamical-mean-field theory we study…

Materials Science · Physics 2014-12-11 R. Nourafkan , G. Kotliar , A. -M. S. Tremblay

An antiferromagnetic ordering in Pb3TeCo3V2O14 takes place through formation of short range correlation regime with T* ~ 10.5 K and succession of second order phase transition at TN1 = 8.9 K and first order phase transition at TN2 = 6.3 K.…

Strongly Correlated Electrons · Physics 2014-04-01 M. M. Markina , B. V. Mill , E. A. Zvereva , A. V. Ushakov , S. V. Streltsov , A. N. Vasiliev

We use a combination of density functional theory and Monte Carlo calculations to calculate the surface magnetization in magnetoelectric $\mathrm{Cr_2O_3}$ at finite temperatures. Such antiferromagnets, lacking both inversion and…

Materials Science · Physics 2023-04-19 Sophie F. Weber , Nicola A. Spaldin

The magnetic and dielectric properties under high magnetic fields are studied in the single crystal of Cu3Mo2O9. This multiferroic compound has distorted tetrahedral spin chains. The effects of the quasi-one dimensionality and the…

Strongly Correlated Electrons · Physics 2013-11-13 H. Kuroe , K. Aoki , R. Kino , T. Sato , H. Kuwahara , T. Sekine , T Kihara , M. Akaki , Y. Kohama , M. Tokunaga , A. Matsuo , K. Kindo , M. Hase , K. Takehana , H. Kitazawa , K. Oka , T. Ito , H. Eisaki

We report a comprehensive set of density functional theory calculations on the family of layered antiferromagnetic manganese pnictides (Ba, Ca, Sr)$\mathrm{Mn}_2\mathrm{(P, As, Sb)}_2$. We characterize all components to the linear…

Materials Science · Physics 2024-06-18 John Mangeri , Martin Ovesen , Thomas Olsen

Magnetoelectric effect is a fundamental physics phenomenon that synergizes electric and magnetic degrees of freedom to generate distinct material responses like electrically tuned magnetism, which serves as a key foundation of the emerging…

Measurements of ferroelectric polarization and dielectric constant were done on $R$Mn$_2$O$_5$ ($R$=Tb, Dy, and Ho) with applied hydrostatic pressures of up to 18 kbar. At ambient pressure, distinctive anomalies were observed in the…

Strongly Correlated Electrons · Physics 2009-11-13 C. R. dela Cruz , B. Lorenz , Y. Y. Sun , Y. Wang , S. Park , S-W. Cheong , M. M. Gospodinov , C. W. Chu

Using neutron diffraction, we have studied the magnetic field effect on charge structures in the charge-ordered multiferroic material LuFe$_2$O$_4$. An external magnetic field is able to change the magnitude and correlation lengths of the…

Strongly Correlated Electrons · Physics 2009-04-10 Jinsheng Wen , Guangyong Xu , Genda Gu , S. M. Shapiro Brookhaven National Laboratory

We performed magnetic and ferroelectric measurements, first principle calculations and Landau theory analysis on hexagonal YMnO3. The polarization and the AFM order parameter were found to present different temperature dependence at TN. A…

Strongly Correlated Electrons · Physics 2011-12-06 Kiran Singh , Natalia Bellido , Charles Simon , Julien Varignon , Marie-B Lepetit , Albin De Muer , Stephane Pailhès

The dielectric properties of MnFe$_2$O$_4$ and $\gamma$-Fe$_2$O$_3$ magnetic nanoparticles embedded in insulating matrices were investigated. The samples showed frequency dependent dielectric anomalies coincident with the magnetic blocking…

Materials Science · Physics 2007-05-23 G. Lawes , R. Tackett , O. Masala , B. Adhikary , R. Naik , R. Seshadri

The magnetoelectric behavior of BiFeO$_3$ has been explored on the basis of accurate density functional calculations. The structural, electronic, magnetic, and ferroelectric properties of BiFeO$_3$ are predicted correctly without including…

Materials Science · Physics 2007-05-23 P. Ravindran , R. Vidya , A. Kjekshus , H. Fjellvåg , O. Eriksson

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

Hexagonal YMnO_3 with space group P63cm is one of the rare examples of multiferroic materials that exhibit co-dependence of a robust ferroelectric phase along with antiferromagnetic ordering. This is primarily ascribed to tilting of the…

Strongly Correlated Electrons · Physics 2010-05-25 A. K. Singh , S. D. Kaushik , V. Siruguri , S. Patnaik

The antiferromagnet Mn$_5$Si$_3$ has recently attracted attention because a noncollinear spin arrangement has been shown to produce a topological anomalous Hall effect and an inverse magnetocaloric effect. Here we synthesize single crystals…

The magnetic properties of GdBaMn_{2}O_{5.0}, which exhibits charge ordering, are studied from 2 to 400 K using single crystals. In a small magnetic field applied along the easy axis, the magnetization M shows a temperature-induced reversal…

Materials Science · Physics 2009-11-13 A. A. Taskin , Yoichi Ando

Neutron diffraction is used to probe the (H,T) phase diagram of magneto-electric (ME) LiNiPO4 for magnetic fields along the c-axis. At zero field the Ni spins order in two antiferromagnetic phases. One has commensurate (C) structures and…

Electric and magnetic properties of multiferroic GdMn2O5 in external magnetic fields were investigated to map out the magnetoelectric phases in this material. Due to strong magnetoelectric coupling, the dielectric permittivity is highly…

It is shown that external magnetic field or magnetization induces electric polarization of microscopic isolated magnetic/non-magnetic hybrid structures due to the spin-dependent electron redistribution and mutual capacity. The…

Mesoscale and Nanoscale Physics · Physics 2015-04-15 P. V. Pyshkin , A. V. Yanovsky

The magnetoelectric effect in the system $RAl_3(BO_3)_4$ ($R$ = Tb, Ho, Er, Tm) is investigated between 3 K and room temperature and at magnetic fields up to 70 kOe. We show a systematic increase of the magnetoelectric effect with…

Strongly Correlated Electrons · Physics 2015-04-27 K. -C. Liang , R. P. Chaudhury , B. Lorenz , Y. Y. Sun , L. N. Bezmaternykh , I. A. Gudim , V. L. Temerov , C. W. Chu