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We investigate the spin-induced polarization in the multiferroic compound Ba2CuGe2O7 using variarional and finite temperature mean field approaches. The compound is described by a spin-3/2 Heisenberg model extended with easy plane…

Strongly Correlated Electrons · Physics 2012-02-21 Judit Romhanyi , Miklos Lajko , Karlo Penc

Magnetic systems with noncentrosymmetric crystal structures are renowned for their complex magnetic ordering and diverse and fascinating physical properties. In this report, we provide a comprehensive study of the chiral magnetic system…

Magneto-electric multiferroics exemplified by TbMnO3 possess both magnetic and ferroelectric long-range order. The magnetic order is mostly understood, whereas the nature of the ferroelectricity has remained more elusive. Competing models…

Strongly Correlated Electrons · Physics 2011-10-14 H. C. Walker , F. Fabrizi , L. Paolasini , F. de Bergevin , J. Herrero-Martin , A. T. Boothroyd , D. Prabhakaran , D. F. McMorrow

We have demonstrated magnetodielectric (MD) coupling in an Ising-chain magnet Sr2Ca2CoMn2O9, via detailed investigation of ac susceptibility and dielectric constant as a function of temperature, magnetic field and frequency. Sr2Ca2CoMn2O9…

Strongly Correlated Electrons · Physics 2021-07-23 Tathamay Basu , Nahed Sakly , Alain Pautrat , Fabien Veillon , Olivier Perez , Vincent Caignaert , Bernard Raveau , Vincent Hardy

We present a phenomenological model for magnetoelectricity in multiferroic materials. The distinctive feature of the model is a two-component complex order parameter that encodes the electric polarization, along with a direct coupling…

Materials Science · Physics 2024-04-11 Pei Wang , You-Quan Li

We have investigated the magnetoelectric coupling in the lone pair containing piezoelectric ferrimagnet Cu2OSeO3. Significant magnetocapacitance develops in the magnetically ordered state (TC = 60 K). We find critical behavior near TC and a…

Materials Science · Physics 2010-02-25 Jan-Willem G. Bos , Claire V. Colin , Thomas T. M. Palstra

Magnetic field induced ferroelectric hysteresis loop observed in Bi0.75Sr0.25FeO3-delta is of prime importance. The coexistence of antiferromagnetism and weak ferromagnetism is responsible for the original magnetoelastic and…

Materials Science · Physics 2009-11-13 Bohdan Kundys , Antoine Maignan , Christine Martin , Ninh Nguyen , Charles Simon

We have studied the influence of antiferromagnetic ordering on the local dielectric moments of the MnO_5 and LuO_7 polyhedra by measuring neutron powder diffraction patterns of LuMnO_3 at temperatures near T_N. We show that the coupling is…

Strongly Correlated Electrons · Physics 2009-11-10 Bas B. Van Aken , Thomas T. M. Palstra

The structural, electronic, magnetic and ferroelectric properties of Pb free double perovskite multiferroic Bi2FeTiO6 are investigated using density functional theory within the general gradient approximation (GGA) method. Our structural…

Materials Science · Physics 2018-05-23 Lokanath Patra , P. Ravindran

The effects of high magnetic fields applied perpendicular to the spontaneous ferroelectric polarization on single crystals of BiFeO$_3$ were investigated through magnetization, magnetostriction, and neutron diffraction measurements. The…

The polycrystalline co-doped samples of Sm0.5Y0.5Fe0.58Mn0.42O3 were prepared by solid-state reaction route and its various physical properties with their correlations have been investigated. The dc magnetization measurements on the sample…

We report the results of various measurements, namely magnetization, complex dielectric permittivity and electric polarization (P) on Dy2BaNiO5 as a function of temperature (T) and magnetic-field (H), apart from heat-capacity (C), with the…

Materials Science · Physics 2015-06-15 Kiran Singh , Tathamay Basu , S. Chowki , N. Mahapotra , K. Iyer , P. L. Paulose , E. V. Sampathkumaran

Magnetoelectric coupling in the polycrystalline antiferromagnets CuFe0.95Rh0.05O2 and CuFeO2 has been investigated. For both samples, electric polarization was observed in the absence of an applied external magnetic field demonstrating that…

Materials Science · Physics 2009-05-27 B. Kundys , A. Maignan , D. Pelloquin , Ch. Simon

Magnetoelectric (ME) effect is recognized for its utility for low-power electronic devices.Largest ME coefficients are often associated with phase transitions in which ferroelectricity is induced by magnetic order. Unfortunately, in these…

The chain-like system Ba_{3}Cu_{3}Sc_4O_{12} has potentially interesting magnetic properties due to the presence of Cu^{2+} and a structure-suggested low-dimensionality. We present magnetization M versus magnetic field H and temperature T,…

Strongly Correlated Electrons · Physics 2012-11-16 B. Koteswararao , A. V. Mahajan , F. Bert , P. Mendels , J. Chakraborty , V. Singh , I. Dasgupta , S. Rayaprol , V. Siruguri , A. Hoser , S. D. Kaushik

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

We have recently reported that the Haldane spin-chain system, Er2BaNiO5, undergoing antiferromagnetic order below 32 K, is characterized by the onset of ferroelectricity near 60K due to magnetoelectric coupling induced by short-range…

Strongly Correlated Electrons · Physics 2015-06-22 Tathamay Basu , Kiran Singh , N. Mohapatra , E. V. Sampathkumaran

Neutron scattering studies and measurements of the dielectric susceptibility and ferroelectric polarization P have been carried out in various magnetic fields H for single-crystal samples of the multiferroic system LiVCuO4 with quasi…

Strongly Correlated Electrons · Physics 2015-05-13 Yukio Yasui , Yutaka Naito , Kenji Sato , Taketo Moyoshi , Masatoshi Sato* , Kazuhisa Kakurai

We present a theoretical analysis of the magnetocaloric effect in the frustrated antiferromagnet \Eu. Monte Carlo simulations indicate a large magnetic entropy change $\Delta S_M^{\text{max}} \sim 5.14$ J kg$^{-1}$K$^{-1}$ at $T=2.45$K for…

Strongly Correlated Electrons · Physics 2022-07-05 D. J. García , D. G. Franco , Pablo S. Cornaglia

We present a unique example of giant magnetoelectric effect in a conventional multiferroic HoMnO3, where polarization is very large (~56 mC/m2) and the ferroelectric transition temperature is higher than the magnetic ordering temperature by…

Strongly Correlated Electrons · Physics 2015-05-13 N. Hur , I. K. Jeong , M. F. Hundley , S. B. Kim , S. -W. Cheong