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The polarized Raman spectra of stoichiometric LaTiO$_3$ (T$_N = 150$ K) were measured between 6 and 300 K. In contrast to earlier report on half-metallic LaTiO$_{3.02}$, neither strong background scattering, nor Fano shape of the Raman…

We study the Raman spectrum of CrI$_3$, a material that exhibits magnetism in a single-layer. We employ first-principles calculations within density functional theory to determine the effects of polarization, strain, and incident angle on…

Materials Science · Physics 2018-08-08 Daniel T. Larson , Efthimios Kaxiras

We investigate the experimental signatures of Raman spectroscopy of bi- and tri-magnon excitations in the distorted triangular lattice antiferromagnets alpha-LCr2O4 (L=Sr, Ca). We utilize spin wave theory to analyze the nearly 120 degree…

Strongly Correlated Electrons · Physics 2023-05-23 Junli Li , Shangjian Jin , Trinanjan Datta , Dao-Xin Yao

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

Raman scattering spectra of zigzag spin chain TaFe$_{1.25}$Te$_3$ single crystal are presented in a temperature range from 80 to 300 K. Nine Raman active modes of $A_g$ and $B_g$ symmetry are clearly observed and assigned by probing…

Resonance Raman scattering, which probes electrons, phonons and their interplay in crystals, is extensively used in two-dimensional materials. Here we investigate Raman modes in MoSe$_2$ at different laser excitation energies from 2.33 eV…

The recently discovered layered BiS2-based superconductors have attracted a great deal of interest due to their structural similarity to cuprate and iron-pnictide superconductors. We have performed Raman scattering measurements on two…

Superconductivity · Physics 2016-03-08 Yong Tian , Anmin Zhang , Kai Liu , Jianting Ji , Jianzhong Liu , Xiyu Zhu , Hai-Hu Wen , Feng Jin , Xiaoli Ma , Qing-Ming Zhang

We have carried out temperature-dependent x-ray diffraction and Raman scattering experiments on powder $Cs_3Bi_2Br_9$. Trigonal to monoclinic structural transition at around 95 K is discussed and shown to be driven by the softening of the…

A combined scattering mechanism involving the states of free electron-hole pairs (exciton continuum) and discrete excitons as intermediate states in the multi-phonon Raman scattering leads to (1) a strong increase of the scattering…

Condensed Matter · Physics 2009-10-28 I. G. Lang , A. V. Prokhorov , M. Cardona , V. I. Belitsky , A. Cantarero , S. T. Pavlov

We have studied polarized Raman spectra of (TMTSF)2PF6 single crystals in the wide spectral and temperature range using different laser energies. We observed and assigned 23 Raman active modes. The carbon C=C in-phase and out-of-phase…

Strongly Correlated Electrons · Physics 2007-05-23 Z. V. Popovic , V. A. Ivanov , O. P. Khoung , T. Nakamura , G. Saito , V. V. Moshchalkov

2D magnetism in triangular lattices has already shown potential for hosting exotic magnetic states. Control of these magnetic states, both in terms of magnetic properties and in terms of charge doping would be the next step. This makes…

The paper presents detailed Raman scattering study of the unusually broad E2g phonon mode in MgB2 crystal. For the first time, it is shown by the polarized Raman scattering on few-micron-size crystallites with natural faces that the…

Superconductivity · Physics 2012-12-18 J. Hlinka , I. Gregora , J. Pokorny , A. Plecenik , P. Kus , L. Satrapinsky , S. Benacka

We report on Raman scattering measurements of single crystalline La$_{1-x}$Sr$_x$MnO$_3$ ($x$=0, 0.06, 0.09 and 0.125), focusing on the high frequency regime. We observe multi-phonon scattering processes up to fourth-order which show…

We calculate the Raman spectrum of the two-dimensional (2D) spin-1/2 Heisenberg antiferromagnet by exact diagonalization and quantum Monte Carlo techniques on clusters of up to 144 sites and, on a 16-site cluster, by considering the…

Superconductivity · Physics 2016-08-31 Franco Nori , Roberto Merlin , Stephan Haas , Anders Sandvik , Elbio Dagotto

The quadruple Calcium manganite (CaMn7O12) is a multiferroic material that exhibits a giant magnetically-induced ferroelectric polarization which makes it very interesting for magnetoelectric applications. Here, we report the Raman…

Strongly Correlated Electrons · Physics 2019-01-16 C. Toulouse , C. Martin , M-A. Measson , Y. Gallais , A. Sacuto , M. Cazayous

We consider a model of Raman scattering for a two--dimensional $S=1/2$ Heisenberg Anti-Ferromagnet which includes a {\it dynamical} spin--phonon interaction. We observe a broadening of the line shape due to increased coupling with excited…

Condensed Matter · Physics 2009-10-28 Matthew J. Reilly , A. G. Rojo

To date, two types of coupling between electromagnetic radiation and a crystal lattice have been identified experimentally. One is direct, for infrared (IR)-active vibrations that carry an electric dipole. The second is indirect, it occurs…

Two aspects in connection with the magnetic properties of La_{2-x-y}Nd_ySr_xCuO_4 single crystals are discussed. The first is related to long wavelength magnetic excitations in x = 0, 0.01, and 0.03 La_{2-x}Sr_xCuO_4 detwinned crystals as a…

Strongly Correlated Electrons · Physics 2015-06-25 A. Gozar , Seiki Komiya , Yoichi Ando , G. Blumberg

Polarized Raman scattering has been performed on CaC6 superconductor. We identify two of the three Raman active Eg phonon modes at 440 and 1508 cm-1 expected for the R-3m space group of CaC6. These first order scattering modes appear along…

Materials Science · Physics 2009-11-13 A. Mialitsin , J. S. Kim , R. K. Kremer , G. Blumberg

We present a systematic study of spin and lattice dynamics in the quasi-one-dimensional spiral magnet CuBr2, using Raman scattering in conjunction with infrared and neutron spectroscopy. Along with the development of spin correlations upon…