Related papers: Circular dichroism of second harmonic generation r…
We show that spatially structured radiation generates second harmonic in a two-dimensional system even if the system is homogeneous and isotropic. The effect originates from non-locality of electric response to structured electromagnetic…
Molecular chirality is a key design property for many technologies including bioresponsive imaging, circularly polarized light detection and emission, molecular motors and switches. Imaging and manipulating the primary steps of transient…
We show that, under the effect of an external magnetic field, a photogalvanic effect and the generation of second harmonic wave can be induced in inversion-symmetric and time reversal invariant Dirac semimetals. The mechanism responsible of…
Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…
We show that a nonchiral atom can act as an antenna to induce a photoelectron circular dichroism in a nearby chiral molecule in a three-step process: The donor atom (antenna) is initially resonantly excited by circularly polarized…
We consider the reflection of a photon by a two-level system in a quasi-one-dimensional waveguide. This is important in part because it forms the backdrop for more complicated proposals where many emitters are coupled to the waveguide:…
The generation of high-order harmonics in a medium of chiral molecules driven by intense bi-elliptical laser fields can lead to strong chiroptical response in a broad range of harmonic numbers and ellipticities [D. Ayuso et al, J. Phys. B…
Chiroptical responses in atomic systems are usually weak, as they arise from the interference between electric- and much weaker magnetic-dipole transitions. We show that atoms arranged in chiral geometries can instead exhibit a strong…
It is commonly accepted that the magnitude of a photoelectron circular dichroism (PECD) is governed by the ability of an outgoing photoelectron wave packet to probe the chiral asymmetry of a molecule. To be able to accumulate this…
Material anisotropy and chirality produce polarization-dependent light-matter interactions. Absorption leads to linear and circular dichroism, whereas elastic forward scattering produces linear and circular birefringence. Here we highlight…
We report terahertz (THz) second harmonic generation (SHG) in superconductors (SC) with inversion symmetric equilibrium states that forbid even-order nonlinearities. Such SHG signal is observed in single-pulse emission by periodic driving…
Coupling of electric and magnetic responses of a scatterer known as bianisotropy enables rich physics and unique optical phenomena, including asymmetric absorption or reflection, one-way transparency, and photonic topological phases. Here…
We present a rigorous finite element method to calculate circular dichroism (CD) in various systems consisting of nanostructures and oriented chiral molecules with electric quadrupole transitions. The interaction between oriented molecule…
While plasmonic particles can provide optical resonances in a wide spectral range from the lower visible up to the near-infrared, often symmetry effects are utilized to obtain particular optical responses. By breaking certain spatial…
In photoelectron circular dichroism (PECD) it is generally difficult to trace how and when the chirality of the molecule is imprinted onto the photoelectron. We present simulations of PECD in a simple model and employ chirality measures to…
We investigate the interaction between a monolayer of WS2 and a chiral plasmonic metasurface. WS2 possesses valley excitons that selectively couple with one-handed circularly polarised light. At the same time, the chiral plasmonic…
We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…
We show that the second harmonic generation (SHG) is enhanced in the chiral one-dimensional electron currents in a broad frequency range. The origin of the enhancement is two-fold: first, the linear dispersion of the current and the…
We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…
We investigate how optimal control theory can be used to improve Circular Dichroism (CD) signals for A--band of fenchone measured via the photoionization yield upon further excitation. These transitions are electric dipole forbidden to…