Related papers: Time-resolved mid-infrared dual-comb spectroscopy
We demonstrate the first cavity-enhanced optical frequency comb spectroscopy in the mid-infrared wavelength region and report the sensitive real-time trace detection of hydrogen peroxide in the presence of a large amount of water. The…
Optical frequency combs have revolutionized high-precision spectroscopy, yet an intrinsic trade-off between spectroscopic signal-to-noise ratio (sSNR) and measurement bandwidth ($B$) fundamentally constrains sensitive, broadband…
Spectral imaging in the mid-infrared (MIR) range provides simultaneous morphological and chemical information of a wide variety of samples. However, current MIR technologies struggle to produce high-definition images over a broad spectral…
Fast (sub-second) spectroscopy with high spectral resolution is of vital importance for revealing quantum chemistry kinetics of complex chemical and biological reactions. Fourier transform (FT) spectrometers can achieve high spectral…
Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the…
In the current study, a quantum-cascade-laser-based dual-comb spectrometer (DCS) was used to paint a detailed picture of a 1.0 ms high-temperature reaction between propyne and oxygen. The DCS interfaced with a shock tube to provide…
Dual-comb spectroscopy is extended to the visible spectral range with a set-up based on two frequency-doubled femtosecond ytterbium-doped fiber lasers. The dense rovibronic spectrum of iodine around 19240 cm-1 is recorded within 12 ms at…
Dual-comb spectroscopy is a promising method for precise optical spectrum analysis with fast data acquisition speed. However, its implementation and applications are often hindered by the complexity of optical comb systems. Here, as a…
Here, ultra-low relative phase jitters over a wide optical spectrum were achieved for dual Ti:Sapphire optical frequency combs. The two optical frequency combs were independently phase-locked to a Sr optical lattice clock laser delivered…
We present a dual-comb spectrometer based on two passively mode-locked waveguide lasers integrated in a single Er-doped ZBLAN chip. This original design yields two free-running frequency combs having a high level of mutual stability. We…
Mid-infrared femtosecond optical frequency combs were produced by difference frequency generation of the spectral components of a near-infrared comb in a 3-mm-long MgO:PPLN crystal. We observe strong pump depletion and 9.3 dB parametric…
While mid-infrared radiation can be used to identify and quantify numerous chemical species, contemporary broadband mid-IR spectroscopic systems are often hindered by large footprints, moving parts and high power consumption. In this work,…
A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…
A facility for sub-nanosecond time-resolved (pump-probe) infrared spectroscopy has been developed at the National Synchrotron Light Source of Brookhaven National Laboratory. A mode-locked Ti:sapphire laser produces 2 ps duration, tunable…
Open-path dual-comb spectroscopy (DCS) significantly enhances our understanding of regional trace gases. However, due to technical challenges, cost considerations, and eye-safety regulations, its sensing range and flexibility remain…
Coherent anti-Stokes Raman scattering (CARS) spectroscopy with time-delayed ultrashort pulses and a single-pixel photodetector has shown great potential for spectroscopic imaging and transient studies in chemistry and biological research.…
Coherent laser beams in the 3 to 20 {\mu}m region of the spectrum are most applicable for chemical sensing by addressing the strongest vibrational absorption resonances of the media. Broadband frequency combs in this spectral range are of…
We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…
Sustained mutual coherence between two combs over extended periods is a prerequisite for dual-comb spectroscopy (DCS), particularly in achieving high-resolution molecular spectroscopy and precise spectral measurements. However, achieving…
There is an increasing demand for precise molecular spectroscopy, in particular in the mid-infrared fingerprint window that hosts a considerable number of vibrational signatures, whether it be for modeling our atmosphere, interpreting…