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Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical…

Mesoscale and Nanoscale Physics · Physics 2017-05-12 Andrew K. Mitchell , Kim G. L. Pedersen , Per Hedegaard , Jens Paaske

Destructive quantum interference in molecular junctions might be used to build molecular quantum rulers, allowing to quantify changes in external control parameters electrically. For this reason, it is important to understand which patterns…

Mesoscale and Nanoscale Physics · Physics 2025-07-10 Lukas Krieger , Gert-Ludwig Ingold , Fabian Pauly

Using exact-diagonalization techniques supplemented by a Dyson equation embedding procedure, the transport properties of multilevel quantum dots are investigated in the Kondo regime. The conductance can be decomposed into the contributions…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 C. A. Büsser , G. B. Martins , K. A. Al-Hassanieh , Adriana Moreo , Elbio Dagotto

As the dimensions of a conductor approach the nano-scale, quantum effects will begin to dominate its behavior. This entails the exciting possibility of controlling the conductance of a device by direct manipulation of the electron wave…

We analyze quantum interference and decoherence effects in single-molecule junctions both experimentally and theoretically by means of the mechanically controlled break junction technique and density-functional theory. We consider the case…

Mesoscale and Nanoscale Physics · Physics 2012-09-26 Stefan Ballmann , Rainer Härtle , Pedro B. Coto , Marcel Mayor , Mark Elbing , Martin R. Bryce , Michael Thoss , Heiko B. Weber

The linear transport properties of a model molecular transistor with electron-electron and electron-phonon interactions were investigated analytically and numerically. The model takes into account phonon modulation of the electronic energy…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 P. S. Cornaglia , D. R. Grempel , H. Ness

Coherent electronic transport through individual molecules is crucially sensitive to quantum interference. Using exact diagonalization techniques, we investigate the zero-bias and zero-temperature conductance through $\pi$-conjugated…

Strongly Correlated Electrons · Physics 2015-05-14 Julian Rincon , K. Hallberg , S. Ramasesha

Destructive quantum interference in electron transport through molecules provides an unconventional route for suppressing electric current. In this work we introduce "interference vectors" for each interference and use them to characterize…

Mesoscale and Nanoscale Physics · Physics 2017-07-20 Panu Sam-ang , Matthew G. Reuter

Recent observations of destructive quantum interference in single-molecule junctions confirm the role played by quantum effects in the electronic conductance properties of molecular systems. We show here that the destructive interference…

Mesoscale and Nanoscale Physics · Physics 2017-09-25 Riccardo Frisenda , Vera Jansen , Ferdinand C. Grozema , Herre S. J. van der Zant , Nicolas Renaud

We look for manifestations of quantum interference effects in the Seebeck coefficient of a molecular junction, when the electronic conductance exhibits pronounced destructive interference features due to the presence of quasi-degenerate…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Lena Simine , Wei Jia Chen , Dvira Segal

Quantum interference can profoundly affect charge transport in single molecules, but experiments can usually measure only the conductance at the Fermi energy. Because in general the most pronounced features of the quantum interference are…

We calculate the finite temperature and non-equilibrium electric current through systems described generically at low energy by a singlet and \emph{two} spin doublets for $N$ and $N \pm 1$ electrons respectively, coupled asymmetrically to…

Strongly Correlated Electrons · Physics 2011-08-24 P. Roura-Bas , L. Tosi , A. A. Aligia , K. Hallberg

Quantum interference effects and decoherence mechanisms in single-molecule junctions are analyzed employing a nonequilibrium Green's function approach. Electrons tunneling through quasi-degenerate states of a nanoscale molecular junction…

Mesoscale and Nanoscale Physics · Physics 2011-07-25 R. Härtle , M. Butzin , O. Rubio-Pons , M. Thoss

Molecular junctions -- whether actual single molecules in nanowire break junctions or artificial molecules realized in coupled quantum dot devices -- offer unique functionality due to their orbital complexity, strong electron interactions,…

Mesoscale and Nanoscale Physics · Physics 2024-08-15 Sudeshna Sen , Andrew K. Mitchell

We provide a simple set of rules for predicting interference effects in off-resonant transport through single-molecule junctions. These effects fall in two classes, showing respectively an odd or an even number of nodes in the linear…

Mesoscale and Nanoscale Physics · Physics 2014-09-12 Kim G. L. Pedersen , Mikkel Strange , Martin Leijnse , Per Hedegård , Gemma Solomon , Jens Paaske

We discuss the electronic transport through molecules in the Kondo regime. We concentrate here on the influence of molecular vibrations. Two types of vibrations are investigated: (i) the breathing internal molecular modes, where the…

Mesoscale and Nanoscale Physics · Physics 2009-12-21 J. Mravlje , A. Ramsak

We systematically investigate electron transport through double quantum dots with particular emphasis on interference induced via multiple paths of electron propagation. By means of the slave-boson mean-field approximation, we calculate the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yoichi Tanaka , Norio Kawakami

We review mechanisms of low-temperature electronic transport through a quantum dot weakly coupled to two conducting leads. Transport in this case is dominated by electron-electron interaction. At temperatures moderately lower than the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Pustilnik , L. I. Glazman

Inelastic effects in the Coulomb blockade and Kondo regimes of electron transport through molecular junctions are considered within a simple nonequilibrium equation-of-motion (EOM) approach. The scheme is self-consistent, and can…

Mesoscale and Nanoscale Physics · Physics 2007-07-02 Michael Galperin , Abraham Nitzan , Mark A. Ratner

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic…

Mesoscale and Nanoscale Physics · Physics 2013-02-18 R. Härtle , M. Butzin , M. Thoss
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