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We propose a theoretical model for a gapless spin liquid phase that may have been observed in a recent experiment on $\mathrm{H_3Li Ir_2 O_6}$. Despite the insulating and non-magnetic nature of the material, the specific heat coefficient…

Strongly Correlated Electrons · Physics 2018-03-29 Kevin Slagle , Wonjune Choi , Li Ern Chern , Yong Baek Kim

Motivated by the recent synthesis of two insulating Li$_2$IrO$_3$ polymorphs, where Ir$^{4+}$ $S_{eff}$=1/2 moments form 3D ("harmonic") honeycomb structures with threefold coordination, we study magnetic Hamiltonians on the resulting…

Strongly Correlated Electrons · Physics 2014-11-26 Itamar Kimchi , James G. Analytis , Ashvin Vishwanath

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

Strongly Correlated Electrons · Physics 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

The layered triangular lattice owing to $1:2$ order of $B$ and $B'$ sites in the triple perovskite $A_3 B B'_2$O$_9$ family provides an enticing domain for exploring the complex phenomena of quantum spin liquids (QSLs). We report a…

Strongly Correlated Electrons · Physics 2024-08-07 K. Bhattacharya , S. Mohanty , A. D. Hillier , M. T. F. Telling , R. Nath , M. Majumder

Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…

We report structural studies of the spin-orbit Mott insulator family K$_x$Ir$_y$O$_2$, with triangular layers of edge-sharing IrO$_6$ octahedra bonded by potassium ions. The potassium content acts as a chemical tuning parameter to control…

Strongly Correlated Electrons · Physics 2019-12-25 R. D. Johnson , I. Broeders , K. Mehlawat , Y. Li , Y. Singh , R. Valenti , R. Coldea

Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically…

We present a comprehensive experimental investigation of the temperature evolution of magnetic states in triangular-lattice delafossite YbCuSe$_2$. Magnetization measurements on high-quality single crystals reveal easy-plane anisotropy.…

Strongly Correlated Electrons · Physics 2026-04-08 K. Bhattacharya , Y. Tokiwa , M. Majumder

The physics of Mott insulators underlies diverse phenomena ranging from high temperature superconductivity to exotic magnetism. Although both the electron spin and the structure of the local orbitals play a key role in this physics, in most…

The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…

Strongly Correlated Electrons · Physics 2007-05-23 Yasuhiro Shimizu , Kazuya Miyagawa , Kazushi Kanoda , Maesato Mitsuhiko , Gunzi Saito

Magnetic moments arranged at the corners of a honeycomb lattice are predicted to form a novel state of matter, Kitaev quantum spin liquid, under the influence of frustration effects between bond-dependent Ising interactions. Some layered…

Strongly Correlated Electrons · Physics 2022-03-09 Sean K. Takahashi , Jiaming Wang , Alexandre Arsenault , Mykola Abramchuk , Fazel Tafti , Philip M. Singer , Takashi Imai

Kitaev magnets are materials with bond-dependent Ising interactions between localized spins on a honeycomb lattice. Such interactions could lead to a quantum spin-liquid (QSL) ground state at zero temperature. Recent theoretical studies…

Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model more than half a century…

Strongly Correlated Electrons · Physics 2022-11-15 T. Arh , B. Sana , M. Pregelj , P. Khuntia , Z. Jagličić , M. D. Le , P. Biswas , A. Ozarowski , A. Zorko

The honeycomb lattice iridates $A_2$IrO$_3$ ($A =$ Na, Li) are candidates for realization of the Kitaev-Heisenberg model although their proximity to Kitaev's quantum Spin-Liquid (QSL) is still debated. We report on heat capacity $C$ and…

Strongly Correlated Electrons · Physics 2017-04-12 K. Mehlawat , A. Thamizhavel , Yogesh Singh

We report results of our study of a newly synthesized honeycomb iridate NaxIrO3 (0.60 < x < 0.80). Single-crystal NaxIrO3 adopts a honeycomb lattice noticeably without distortions and stacking disorder inherently existent in its sister…

Strongly Correlated Electrons · Physics 2021-07-28 Hengdi Zhao , Bing Hu , Feng Ye , Minhyea Lee , Pedro Schlottmann , Gang Cao

Strong spin-orbital-coupling magnetic systems with the honeycomb structure can provide bond-directional interactions which may result in Kitaev quantum spin liquids and exotic anyonic excitations. However, one of the key ingredients in real…

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

Quantum spin liquid (QSL) state in rare-earth triangular lattice has attracted much attention recently due to its potential application in quantum computing and communication. Here we report the single-crystal growth synthesis, crystal…

Strongly Correlated Electrons · Physics 2021-11-16 Jie Xing , Liurukara D. Sanjeewa , Andrew F. May , Athena S. Sefat

In transition-metal compounds with partially filled $4d$ and $5d$ shells spin-orbit entanglement, electronic correlations, and crystal-field effects conspire to give rise to a variety of novel forms of topological quantum matter. This…

Strongly Correlated Electrons · Physics 2017-01-26 Simon Trebst

Anderson proposed structural topology in frustrated magnets hosting novel quantum spin liquids (QSLs). The QSL state is indeed exactly derived by fractionalizing the spin excitation into spinless Majorana fermions in a perfect two…

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