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Indirect excitons (IXs) in van der Waals transition-metal dichalcogenide (TMD) heterostructures are characterized by a high binding energy making them stable at room temperature and giving the opportunity for exploring fundamental phenomena…

Mesoscale and Nanoscale Physics · Physics 2018-05-24 E. V. Calman , M. M. Fogler , L. V. Butov , S. Hu , A. Mishchenko , A. K. Geim

We investigate the ultrafast dynamics of photo-induced non-thermal lattice disorder in a polycrystalline aluminium thin film to elucidate transient short- and long-range lattice distortions, their thermalization and electron-phonon coupling…

Materials Science · Physics 2026-01-06 Fernando Rodriguez Diaz , Kasra Amini

We present a unified description of the excitonic properties of four monolayer transition-metal dichalcogenides (TMDC's) using an equation of motion method for deriving the Bethe-Salpeter equation in momentum space. Our method is able to…

Mesoscale and Nanoscale Physics · Physics 2017-08-08 A. J. Chaves , R. M. Ribeiro , T. Frederico , N. M. R. Peres

Vertical heterostructures (HS) of transition metal dichalcogenides (TMDs) host interlayer excitons (ILX), with electrons and holes residing in different layers. With respect to their intralayer counterparts, ILX feature much longer…

We show how two different mobile-immobile type models explain the observation of negative diffusion of excitons reported in experimental studies in quasi-two-dimensional semiconductor systems. The main reason for the effect is the initial…

Mesoscale and Nanoscale Physics · Physics 2024-10-24 Alerksandr A. Kurilovich , Vladimir N. Mantsevich , Aleksey V. Chechkin , Vladimir V. Palyulin

The transition-metal dicyanides M(CN)$_2$ (M = Zn, Cd) are amongst the most important negative thermal expansion (NTE) materials known, favoured for the magnitude, isotropy, and thermal persistence of the NTE behaviour they show. The…

The optically dark states play an important role in the electronic and optical properties of monolayers (MLs) of semiconducting transition metal dichalcogenides. The effect of temperature on the in-plane-field activation of the neutral and…

We develop a non-local dielectric response theory to describe the temperature dependence of exciton lifetime in metal-semiconductor heterostructures. Coupling between excitons and surface plasmons results in a strongly nonmonotonous…

Mesoscale and Nanoscale Physics · Physics 2015-05-07 M. V. Durnev , A. V. Kavokin , B. Gil

We show that the "dark condensates" that arise when excitons form a Bose-Einstein condensate in a material with an indirect bandgap are not completely dark to optical emission. Rather, such states are "leaky condensates" in which optical…

Mesoscale and Nanoscale Physics · Physics 2022-05-31 Benjamin Remez , Nigel R. Cooper

Excitons in a monolayer transition metal dichalcogenide (1L-TMD) are highly bound states characterized by a Rydberg-like spectrum of discrete energy levels. Among these, states with odd-parity are known as dark excitons due to selection…

The role and impact of spatial heterogeneity in two-dimensional quantum materials represents one of the major research quests regarding the future application of these materials in optoelectronics and quantum information science. In the…

The latest breakthroughs in time-varying photonics are fueling novel thermal emission phenomena, for example, showing that the dynamic amplification of quantum vacuum fluctuations, induced by the time-modulation of material properties,…

Two-dimensional transition metal dichalcogenides (TMDCs) have recently become attractive semiconductor materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and…

Optics · Physics 2018-07-04 Alex Krasnok , Sergey Lepeshov , Andrea Alú

Exciton spectra of monolayer transition metal dichalcogenides (TMDs) in various dielectric environments are studied. The screened hydrogen model (SHM) [Phys. Rev. Lett. 116, 056401 (2016)] is examined by comparing its exciton spectra with…

Mesoscale and Nanoscale Physics · Physics 2019-02-20 Jian-zhong Zhang , Jin-zhong Ma

When electron-hole pairs are excited in a semiconductor, it is a priori not clear if they form a fermionic plasma of unbound particles or a bosonic exciton gas. Usually, the exciton phase is associated with low temperatures. In atomically…

Transition metal dichalcogenides (TMDs) have valley degree of freedom, which features optical selection rule and spin-valley locking, making them promising for valleytronics devices and quantum computation. For either application, a long…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 Chongyun Jiang , Weigao Xu , Abdullah Rasmita , Zumeng Huang , Ke Li , Qihua Xiong , Wei-bo Gao

How ordered phases melt in low-dimensional quantum materials remain difficult to resolve because the relevant fluctuations are dynamic and charge neutral. In this work, we show that thermal transport provides a sensitive probe of these…

Electric field-controlled, two-dimensional (2D) exciton dynamics in transition metal dichalcogenide monolayers is a current research focus in condensed matter physics. We have experimentally investigated the spectral and temporal properties…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 Michael Engel , Mathias Steiner

Two-dimensional transition metal dichalcogenides (TMDs) offer tunable optical and electronic properties, making them highly promising for next-generation optoelectronic devices. One effective approach to engineering these properties is…

Two-dimensional perovskites, in which inorganic layers are stabilized by organic spacer molecules, are attracting increasing attention as a more robust analogue to the conventional three-dimensional metal-halide perovskites. However,…

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