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The recent experimental discovery of intrinsic ferromagnetism in single-layer CrI3 opens a new avenue to low-dimensional spintronics. However, the low Curie temperature Tc=45 K is still a large obstacle to its realistic device application.…

Materials Science · Physics 2019-06-26 Hongxing Li , Yuan-Kai Xu , Kang Lai , Wei-Bing Zhang

The monolayer halides CrX$_3$ (X=Cl, Br, I) attract significant attention for realizing 2D magnets with genuine long-range order (LRO), challenging the Mermin-Wagner theorem. Here, we show that monolayer CrCl$_3$ has the unique benefit of…

Strongly Correlated Electrons · Physics 2021-07-19 Maxime Dupont , Yaroslav O. Kvashnin , Mahroo Shiranzaei , Jonas Fransson , Nicolas Laflorencie , Adrian Kantian

Since the celebrated discovery of graphene, the family of two-dimensional (2D) materials has grown to encompass a broad range of electronic properties. Recent additions include spin-valley coupled semiconductors, Ising superconductors that…

To broaden the scope of van der Waals 2D magnets, we report the synthesis and magnetism of covalent 2D magnetic Cr$_2$Te$_3$ with a thickness down to one-unit-cell. The 2D Cr$_2$Te$_3$ crystals exhibit robust ferromagnetism with a Curie…

Identifying intrinsic low-dimensional ferromagnets with high transition temperature and electrically tunable magnetism is crucial for the development of miniaturized spintronics and magnetoelectrics. Recently long-range 2D ferromagnetism…

Materials Science · Physics 2020-08-27 Hua Wang , Jingshan Qi , Xiaofeng Qian

Magnetism in two-dimensional van der Waals materials has received significant attention recently. The Curie temperature reported for those materials, however, has been so far remained relatively low. Here, we measure magneto-optical Kerr…

Mesoscale and Nanoscale Physics · Physics 2019-12-09 H. Idzuchi , A. E. Llacsahuanga Allcca , X. C. Pan , K. Tanigaki , Y. P. Chen

Two-dimensional magnets have received increasing attention since Cr2Ge2Te6 and CrI3 were experimentally exfoliated and measured in 2017. Although layered ferromagnetic metals were demonstrated at room temperature, a layered ferromagnetic…

Materials Science · Physics 2019-03-19 Cong Wang , Xieyu Zhou , Linwei Zhou , Ninghua Tong , Zhong-Yi Lu , Wei Ji

The van der Waals magnets CrX$_3$ (X = I, Br, and Cl) exhibit highly tunable magnetic properties and are promising candidates for developing novel two-dimensional (2D) magnetic devices such as magnetic tunnel junctions and spin tunneling…

Mesoscale and Nanoscale Physics · Physics 2022-12-06 Jia Wang , Zahra Ahmadi , David Lujan , Jeongheon Choe , Takashi Taniguchi , Kenji Watanabe , Xiaoqin Li , Jeffrey E. Shield , Xia Hong

Recently, two-dimensional ferromagnetism in the family of Chromium compounds $\rm CrXTe_3 (X=Si, Ge)$ has attracted a broad research interest. Despite the structural similarity in $\rm CrTe_6$ octahedra, the size effect of inserted Ge or Si…

Applied Physics · Physics 2021-08-03 Zefang Li , Xue Li , Bei Ding , Hang Li , Yuan Yao , Xuekui Xi , Wenhong Wang

We predict that monolayer FeCl$_2$ is a two-dimensional piezoelectric ferromagnet (PFM) with easy-axis magnetism and a Curie temperature of 260 K. Our ab-initio calculations combined with data mining reveal 2H-FeCl$_2$ as the only easy-axis…

Materials Science · Physics 2022-05-03 Kayahan Saritas , Sohrab Ismail-Beigi

The recent discovery of magnetism in atomically thin layers of van der Waals (vdW) crystals has created new opportunities for exploring magnetic phenomena in the two-dimensional (2D) limit. In most 2D magnets studied to date the c-axis is…

Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane…

The van der Waals class of materials offer an approach to two-dimensional magnetism as their spin fluctuations can be tuned upon exfoliation of layers. Moreover, it has recently been shown that spin-lattice coupling and long-range magnetic…

We report an experimental discovery of CrSnS3, a new Van der Waals ferromagnetic (FM) with Curie temperature TC ~119K. The Curie temperature is in qualitative agreement of Chittari et. al. DFT prediction (TC =112.3K) for an Ising model with…

Strongly Correlated Electrons · Physics 2022-07-29 F. Obad , Kh. A. Ziq

We demonstrate room-temperature ferromagnetism with in-plane magnetic anisotropy in thin flakes of the CrTe$_2$ van der Waals ferromagnet. Using quantitative magnetic imaging with a single spin magnetometer based on a nitrogen-vacancy…

Materials Science · Physics 2021-03-31 F. Fabre , A. Finco , A. Purbawati , A. Hadj-Azzem , N. Rougemaille , J. Coraux , I. Philip , V. Jacques

Van der Waals magnetic materials are building blocks for novel kinds of spintronic devices and playgrounds for exploring collective magnetic phenomena down to the two-dimensional limit. Chromium-tellurium compounds are relevant in this…

We have synthesized unique colloidal nanoplatelets of the ferromagnetic two-dimensional (2D) van der Waals material CrI3 and have characterized these nanoplatelets structurally, magnetically, and by magnetic circular dichroism spectroscopy.…

Self-intercalated van der Waals magnets, characterized by self-intercalating native atoms into van der Waals layered structures with intrinsic magnetism, exhibit a variety of novel physical properties. Here, using first-principles…

Materials Science · Physics 2025-01-20 Jia-wan Li , Shi-Bo Zhao , Lin Zhuang , Yusheng Hou

We report a comprehensive high-field/high-frequency electron spin resonance (ESR) study on single crystals of the van der Waals magnet CrCl$_3$. This material, although being known for quite a while, has received recent significant…

Materials Science · Physics 2020-06-09 J. Zeisner , K. Mehlawat , A. Alfonsov , M. Roslova , T. Doert , A. Isaeva , B. Büchner , V. Kataev

The recent discovery of magnetic van der Waals materials has triggered a wealth of investigations in materials science, and now offers genuinely new prospects for both fundamental and applied research. Although the catalogue of van der…

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