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The interaction of relativistically strong tailored laser pulses with an atomic system is considered. Due to a special tailoring of the laser pulse, the suppression of the relativistic drift of the ionized electron and a dramatic…

Atomic Physics · Physics 2007-05-23 M. Klaiber , K. Z. Hatsagortsyan , C. H. Keitel

High-harmonic generation (HHG) is a typical high-order nonlinear optical phenomenon and can be used to probe electronic structures of solids. Here, we investigate the temperature dependence of HHG from Pr_{0.6}Ca_{0.4}MnO_{3} in the range…

Strongly Correlated Electrons · Physics 2025-01-27 A. Nakano , K. Uchida , Y. Tomioka , M. Takaya , Y. Okimoto , K. Tanaka

We report the observations of unexpected layer-dependent, strong, and anisotropic second harmonic generations (SHGs) in atomically thin ReS2. Appreciable (negligible) SHGs are obtained from even (odd) numbers of ReS2 layers, which is…

Optics · Physics 2018-08-20 Yu Song , Siqi Hu , Miao-Ling Lin , Xuetao Gan , Ping-Heng Tan , Jianlin Zhao

We theoretically investigated the dependence of higher-order harmonic generation (HHG) in solid-state materials on the ellipticity of the electric field. We found that in the multiphoton absorption and ac Zener regimes, the intensity of HHG…

Materials Science · Physics 2016-12-28 T. Tamaya , A. Ishikawa , T. Ogawa , K. Tanaka

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

Light sources based on high-harmonic generation (HHG) underpin ultrafast spectroscopy experiments across a large range of photon energies, spanning from the extreme-ultraviolet to the soft x-ray. To this day their design, implementation and…

We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking…

Atomic Physics · Physics 2023-07-25 Fulong Dong , Qinzhi Xia , Jie Liu

Vector beam, with a spatial nonuniform polarization distribution, is important for many applications due to its unique field characteristics and novel effects when interacting with matter. Here through three-dimensional particle-in-cell…

Optics · Physics 2021-03-22 Zi-Yu Chen , Ronghao Hu

Second harmonic generation in a two dimensional nonlinear quasi-crystal is demonstrated for the first time. Temperature and wavelength tuning of the crystal reveal the uniformity of the pattern while angle tuning reveals the dense nature of…

Optics · Physics 2007-05-23 Neil Broderick , Anna Peacock , Katia Gallo , Ruth Lewen , Radu Bratfalean

Generation of odd harmonics by a super strong focused laser beam in vacuum is considered. The process occurs due to the plural light-by-light scattering effect. In the leading order of perturbation theory, generation of $(2k+1)$th harmonic…

High Energy Physics - Phenomenology · Physics 2008-11-26 A. M. Fedotov , N. B. Narozhny

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

Optics · Physics 2022-03-03 Davis M. Welakuh , Prineha Narang

Structural chirality plays an important role in solid state physics and leads to a variety of novel physics. The feasibility of probing structural chirality of crystals using high harmonic generation in solids is explored in this work.…

Optics · Physics 2020-05-15 Zi-Yu Chen , Rui Qin

We report measurements and theoretical simulations of high-order harmonic generation (HHG) in aligned N$_2$ molecules using a 1200-nm intense laser field when the generating pulse is perpendicular to the aligning one. With increasing laser…

We investigate the polarization properties of high harmonic generation from polar molecules with a linearly polarized field. It is found that elliptically polarized harmonics are observed in a wide spectral range from the plateau to the…

Optics · Physics 2011-12-06 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu

We analyze the influence of different recombination scenarios, involving one or two centers, on high-order harmonic generation (HHG) in diatomic molecules, for different values of the internuclear separation. We work within the strong-field…

Atomic Physics · Physics 2015-05-13 C. Figueira de Morisson Faria

High harmonic generation (HHG) records the ultrafast electronic response of matter to light, encoding key properties of the interrogated quantum system, such as chirality. The first implementation of chiral HHG [Cireasa et al. Nat. Phys.…

Structured ultrafast laser beams offer unique opportunities to explore the interplay of the angular momentum of light with matter at the femtosecond scale. Linearly polarized vector beams are paradigmatic examples of structured beams whose…

The landscape of ultrafast structured light pulses has recently evolved driven by the capability of high-order harmonic generation (HHG) to up-convert orbital angular momentum (OAM) from the infrared to the extreme-ultraviolet (EUV)…

Optical harmonic generation on excitons is found in ZnSe/BeTe quantum wells with type-II band alignment. Two experimental approaches with spectrally-broad femtosecond laser pulses and spectrally-narrow picosecond pulses are used for…

In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…

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