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Single crystals of CrSbSe$_3$, a structurally pseudo-one-dimensional ferromagnetic semiconductor, were grown using a high-temperature solution growth technique and were characterized by x-ray diffraction, anisotropic, temperature- and…

Materials Science · Physics 2018-01-24 Tai Kong , Karoline Stolze , Ni Danrui , Satya K. Kushwaha , Robert J. Cava

To date only a few two-dimensional (2D) magnetic crystals were experimentally confirmed, such as CrI3 and CrGeTe3, all with very low Curie temperatures (TC). High-throughput first-principles screening over a large set of materials yields 89…

Materials Science · Physics 2018-12-18 Hang Liu , Jia-Tao Sun , Miao Liu , Sheng Meng

By density functional theory calculations, we predict a stable two-dimensional (2D) ferromagnetic semiconductor Cr$_2$Ge$_2$Se$_6$, where the Curie temperature $T$$_c$ can be dramatically enhanced beyond room temperature by applying a few…

Materials Science · Physics 2019-07-17 Xue-Juan Dong , Jing-Yang You , Bo Gu , Gang Su

Intrinsic, two-dimensional (2D) ferromagnetic semiconductors are an important class of materials for spintronics applications. Cr$_2$X$_2$Te$_6$ (X = Si and Ge) semiconductors show 2D Ising-like ferromagnetism, which is preserved in…

Strongly Correlated Electrons · Physics 2019-01-10 Yu Liu , C. Petrovic

Novel 2D ferromagnets with high Curie temperature and large perpendicular magnetic anisotropy are especially attractive owing to the future promising application in modern spintronics, but meanwhile the 2D ferromagnetic materials with high…

Materials Science · Physics 2022-06-09 Haoyi Tan , Guangcun Shan , Jiliang Zhang

Nanoscale layered ferromagnets have demonstrated fascinating two-dimensional magnetism down to atomic layers, providing a peculiar playground of spin orders for investigating fundamental physics and spintronic applications. However,…

The development of room-temperature tunable magnetic semiconductors is crucial for the advancement of low-power, high-performance information technologies. Using density functional theory calculations, we propose a series of two-dimensional…

Materials Science · Physics 2025-06-12 Jia-Wen Li , Gang Su , Bo Gu

Two-dimensional (2D) ferromagnetic (FM) semiconductors with high Curie temperature have long been pursued for electronic and spintronic applications. Here we provide a general strategy to achieve robust FM state in bilayer CrI3 of the…

Materials Science · Physics 2020-09-23 Nanshu Liu , Si Zhou , Jijun Zhao

We compare three first-principles methods of calculating the Curie temperature in two-dimensional (2D) ferromagnetic materials (FM), modeled using the Heisenberg model, and propose a simple formula for estimating the Curie temperature with…

We report on magnetic and electrical transport properties of Sb2-xCrxTe3 single crystals with 0 <= x <= 0.095 over temperatures from 2 K to 300 K. A ferromagnetic state develops in these crystals at low temperatures with Curie temperatures…

Materials Science · Physics 2009-11-10 J. S. Dyck , C. Drasar , P. Lostak , C. Uher

Using \textit{ab-initio} methods we study structural, electronic and magnetic properties of two dimensional compounds with stoichiometry M$_2$N$_3$ (M-metal, N=S,Se,Te). Our study shows that structures with Cr, Ti, and Mn are stable, with…

Materials Science · Physics 2020-06-18 K. Zberecki

Recent discoveries of intrinsic two-dimensional (2D) ferromagnetism in insulating/semiconducting van der Waals (vdW) crystals open up new possibilities for studying fundamental 2D magnetism and devices employing localized spins. However, a…

A review is given of advances in the field of carrier-controlled ferromagnetism in Mn-based diluted magnetic semiconductors and their nanostructures. Experimental results for III-V materials, where the Mn atoms introduce both spins and…

Materials Science · Physics 2015-06-24 Tomasz Dietl

The ferrimagnetic insulator Mn3Si2Te6, which features a Curie temperature Tc at 78 K and a delicate yet consequential magnetic frustration, exhibits colossal magnetoresistance (CMR) when the magnetic field is applied along the magnetic hard…

Strongly Correlated Electrons · Physics 2022-11-02 Feng Ye , Masaaki Matsuda , Zachary Morgan , Todd Sherline , Yifei Ni , Hengdi Zhao , G. Cao

The realization of long-range magnetic ordering in two-dimensional (2D) systems can potentially revolutionize next-generation information technology. Here, we report the successful fabrication of crystalline Cr3Te4 monolayers with room…

We investigate the magnetocrystalline anisotropy, critical behavior, and magnetocaloric effect in ferromagnetic-layered Cr$_2$Te$_3$. We have studied the critical behavior around the Curie temperature ($T_C$) using various techniques,…

Materials Science · Physics 2024-07-26 Shubham Purwar , Tushar Kanti Bhowmik , Soumya Ghorai , Setti Thirupathaiah

In the quest for two-dimensional conducting materials with high ferromagnetic ordering temperature the new family of the layered Fe$_{n}$GeTe$_{2}$ compounds, especially the near-room-temperature ferromagnet Fe$_{4}$GeTe$_{2}$, receives a…

Intrinsic, two-dimensional ferromagnetic semiconductors are an important class of materials for overcoming the limitations of dilute magnetic semiconductors for spintronics applications. CrSiTe$_3$ is a particularly interesting member of…

Strongly Correlated Electrons · Physics 2015-10-06 T. J. Williams , A. A. Aczel , M. D. Lumsden , S. E. Nagler , M. B. Stone , J. -Q. Yan , D. Mandrus

Recently, two-dimensional ferromagnetic semiconductors have been an important class of materials for many potential applications in spintronic devices. Based on density functional theory, we systematically explore the magnetic and…

Materials Science · Physics 2020-01-14 Yulu Ren , Yanfeng Ge , Wenhui Wan , Qiaoqiao Li , Yong Liu

The Co$_2$Ge$_2$Te$_6$ shows intrinsic ferromagnetic (FM) order, which origins from superexchange interaction between Co and Te atoms, with higher Curie temperature ($T_c$) of 161 K. Co$_2$Ge$_2$Te$_6$ monolayer (ML) is half-metal (HM), and…

Materials Science · Physics 2022-07-06 Zhaoyong Guan , Ziyuan An , Yuzheng Jiang , Ya Su , Yanyan Jiang , Shuang Ni