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By means of first-principles methods we analyze the optical response of transparent dense sodium as a function of applied pressure. We discover an unusual kind of charge-transfer exciton that proceeds from the interstitial distribution of…

Materials Science · Physics 2015-05-18 Matteo Gatti , Ilya V. Tokatly , Angel Rubio

We investigate the thermodynamic properties of a polyelectrolyte solution in a presence of {\it multivalent} salts. The polyions are modeled as rigid cylinders with the charge distributed uniformly along the major axis. The solution,…

Condensed Matter · Physics 2015-06-25 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa

We explore, using the recently developed efficient Monte Carlo simulation method, the interaction of an anionic polyelectrolyte solution with a like-charged dielectric surface. In addition to polyions, the solution also contains salt with…

Soft Condensed Matter · Physics 2018-01-12 Alexandre P. dos Santos , Matheus Girotto , Yan Levin

A new scenario of thermalization process of the adsorbate attached at solid surfaces is proposed. The scenario is based on existence of electric dipole layer in which the electron wavefunctions extend over the positive ions. Thus the strong…

Chemical Physics · Physics 2017-04-26 Paweł Strak , Konrad Sakowski , Stanisław Krukowski

Cononsolvency is a phenomenon for which the solubility of a macromolecule decreases or even vanishes in the mixture of two good solvents. Although it has been widely applied in physicochemical, green chemical and pharmaceutical industry,…

Controlling the dissociation of single water molecule on an insulating surface plays a crucial role in many catalytic reactions. In this Letter, we have identified the enhanced chemical reactivity of ultrathin MgO(100) films deposited on…

Chemical Physics · Physics 2016-04-28 Zhenjun Song , Jing Fan , Hu Xu

We study the salt-dependent conformations of dilute flexible polyelectrolytes in solution via computer simulations. Low concentrations of multivalent salt induce the known conformational collapse of individual polyelectrolyte chains, but as…

Soft Condensed Matter · Physics 2009-11-11 Pai-Yi Hsiao , Erik Luijten

The electrostatic Schwinger-Dyson equations are derived and solved for an electrolyte mixture composed of mono- and multivalent ions confined to a negatively charged nanoslit. The closure of these equations is based on an asymmetric…

Soft Condensed Matter · Physics 2020-01-06 Sahin Buyukdagli

The freshwater crisis is a growing concern and a pressing problem for the world because of the increasing population, civilization, and rapid industrial growth. The water treatment facilities are able to supply less than 1% of the total…

Soft Condensed Matter · Physics 2023-11-28 Nudrat Nawal , Md Rashed Nizam , Priom Das , A K M Monjur Morshed

The forces between colloidal particles at a decane-water interface, in the presence of low concentrations of a monovalent salt (NaCl) and of the surfactant sodium dodecylsulfate (SDS) in the aqueous subphase, have been studied using laser…

Soft Condensed Matter · Physics 2008-07-11 B. J. Park , J. P. Pantina , E. Furst , M. Oettel , S. Reynaert , J. Vermant

A theory of the static electron polarizability of crystals whose energy spectrum is modified by quantizing magnetic fields is presented. It is argued that The polarizability is strongly affected by non-dissipative Hall currents induced by…

Mesoscale and Nanoscale Physics · Physics 2008-04-14 Pavel Streda , Thibaut Jonckheere , Thierry Martin

When we place conducting bodies in electrolyte solutions, their surface potential $\Phi_s$ appears to be much smaller in magnitude than the intrinsic one $\Phi_0$ and normally does not obey the classical electrostatic boundary condition of…

Soft Condensed Matter · Physics 2024-08-09 Olga I. Vinogradova , Elena F. Silkina , Evgeny S. Asmolov

We investigate electro-osmosis in aqueous solutions of polyelectrolytes using mean-field equations. A solution of positively charged polyelectrolytes is confined between two negatively charged planar surfaces, and an electric field is…

Soft Condensed Matter · Physics 2015-06-16 Yuki Uematsu , Takeaki Araki

Capacitive deionization (CDI) is a technology in which water is desalinated by ion electrosorption into the electric double layers (EDLs) of charging porous electrodes. In recent years significant advances have been made in modeling the…

Chemical Physics · Physics 2017-02-01 Amit N. Shocron , Matthew E. Suss

The development of advanced electrochemical devices for energy conversion and storage requires fine tuning of electrode reactions, which can be accomplished by altering the electrode/solution interface structure. Particularly, in case of an…

Soft Condensed Matter · Physics 2020-07-02 Yu. A. Budkov , A. V. Sergeev , S. V. Zavarzin , A. L. Kolesnikov

The free standing solid polymer nanocomposite films has been prepared through standard solution cast technique. The improvement in structural, microstructural and electrochemical properties has been observed on the dispersion of nanofiller…

Materials Science · Physics 2018-07-16 Anil Arya , A. L. Sharma

Like-charge attraction, driven by ionic correlations, challenges our understanding of electrostatics both in soft and hard matter. For two charged planar surfaces confining counterions and water, we prove that even at relatively low…

Soft Condensed Matter · Physics 2023-03-15 Ivan Palaia , Abhay Goyal , Emanuela del Gado , Ladislav Šamaj , Emmanuel Trizac

The present article provides an overview of the recent progress in the direct force measurements between individual pairs of colloidal particles in aqueous salt solutions. Results obtained by two different techniques are being highlighted,…

Soft Condensed Matter · Physics 2016-06-02 Gregor Trefalt , Thomas Palberg , Michal Borkovec

Ionic liquids (ILs) are appealing electrolytes for their favorable physicochemical properties. However, despite their longstanding use, understanding the capacitive behavior of ILs remains challenging. This is largely due to the formation…

Soft Condensed Matter · Physics 2024-01-02 YeongKyu Lee , JunBeom Cho , Yongkyu Lee , Won Bo Lee , YongSeok Jho

The dielectric constant of ionic solutions is known to reduce with increasing ionic concentrations. However, the origin of this effect has not been thoroughly explored. In this paper we study two such possible sources: long-range Coulombic…

Statistical Mechanics · Physics 2022-08-04 Ram M. Adar , Tomer Markovich , Amir Levy , Henri Orland , David Andelman