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Effect of ionic solute on a near-critical binary aqueous mixture confined between charged walls with different adsorption preferences is considered within a simple density functional theory. For the near-critical system containing small…

Soft Condensed Matter · Physics 2015-05-28 F. Pousaneh , A. Ciach

It is known that in a water solution with multivalent counterions (Z-ions), two likely charged macroions can attract each other due to correlations of Z-ions adsorbed on their surfaces. This "correlation" attraction is short-ranged and…

Soft Condensed Matter · Physics 2009-11-10 Rui Zhang , B. I. Shklovskii

We study the interaction between two neutral plane-parallel dielectric bodies in the presence of a highly asymmetric ionic fluid, containing multivalent as well as monovalent (salt) ions. Image charge interactions, due to dielectric…

Soft Condensed Matter · Physics 2015-06-11 Matej Kanduc , Ali Naji , Jan Forsman , Rudolf Podgornik

In a circular channel passing over-limiting current (faster than diffusion), transient vortices of bulk electroconvection are observed in salt-depleted region within the horizontal plane. The spatiotemporal evolution of the salt…

Fluid Dynamics · Physics 2020-08-25 Zhibo Gu , Bingrui Xu , Peng Huo , Shmuel M. Rubinstein , Martin Z. Bazant , Daosheng Deng

A macroion with a strongly charged negative surface in 3:1 salt water solution becomes net positive due to adsorption of an excessive number of positive 3-ions. The widely accepted theory of such charge inversion is based on the idea that…

Soft Condensed Matter · Physics 2024-02-13 Boris Shklovskii

We study water between parallel metal walls under applied electric field accounting for the image effect at $T=298$ K. The electric field due to the surface charges serves to attract and orient nearby water molecules, while it tends to a…

Soft Condensed Matter · Physics 2015-07-24 Kyohei Takae , Akira Onuki

Most electrochemical processes, such as electrodialysis, are limited by diffusion, but in porous media, surface conduction and electro-osmotic flow also contribute to ionic fluxes. In this paper, we report experimental evidence for…

Water is essential for almost every aspect of life on our planet and, unsurprisingly, its properties have been studied in great detail. However, disproportionately little remains known about the electrical properties of interfacial and…

We study the variation of the dielectric response of a dielectric liquid (e.g. water) when a salt is added to the solution. Employing field-theoretical methods we expand the Gibbs free-energy to first order in a loop expansion and calculate…

Soft Condensed Matter · Physics 2012-07-06 Amir Levy , David Andelman , Henri Orland

We present a mechanism for the stabilization of colloids in liquid mixtures without use of surfactants or polymers. When a suitable salt is added to a solvent mixture, the coupling of the colloid's surface chemistry and the preferential…

Soft Condensed Matter · Physics 2015-06-18 Sela Samin , Yoav Tsori

We study the effect of salts on the thickness of wetting films on melting ice and interactions acting on CO$_2$ bubble near ice-water and vapor-water interfaces. Governing mechanisms are the Lifshitz and the double-layer interactions in the…

Soft Condensed Matter · Physics 2016-08-03 P. Thiyam , E. R. A. Lima , O. I. Malyi , D. F. Parsons , S. Y. Buhmann , C. Persson , M. Boström

The pronounced light-matter interactions in photonic crystals make them interesting as opto-fludic "building blocks" for lab-on-a-chip applications. We show how conducting electrolytes cause dissipation and smearing of the…

Optics · Physics 2007-05-23 Niels Asger Mortensen , Simon Ejsing , Sanshui Xiao

Salt crystallization is a major cause of weathering of artworks, monuments and rocks. Damage will occur if crystals continue to grow in confinement, i.e. within the pore space of these materials generating mechanical stresses. We report on…

Materials Science · Physics 2016-01-26 Julie Desarnaud , Daniel Bonn , Noushine Shahidzadeh

We present a novel microfield approach for studying the dependence of the orientational polarization of the water in aqueous electrolyte solutions upon the salt concentration and temperature. The model takes into account the orientation of…

Chemical Physics · Physics 2016-07-15 Nir Gavish , Keith Promislow

The dielectric constant of interfacial water has been predicted to be smaller than that of bulk water (= 80) because the rotational freedom of water dipoles is expected to decrease near surfaces, yet experimental evidence is lacking. We…

Mesoscale and Nanoscale Physics · Physics 2025-10-27 L. Fumagalli , A. Esfandiar , R. Fabregas , S. Hu , P. Ares , A. Janardanan , Q. Yang , B. Radha , T. Taniguchi , K. Watanabe , G. Gomila , K. S. Novoselov , A. K. Geim

A variational theory is developed to study electrolyte solutions, composed of interacting point-like ions in a solvent, in the presence of dielectric discontinuities and charges at the boundaries. Three important and non-linear…

Soft Condensed Matter · Physics 2013-05-29 Sahin Buyukdagli , Manoel Manghi , John Palmeri

Electrostatic correlations between ions dissolved in water are known to impact their transport properties in numerous ways, from conductivity to ion selectivity. The effects of these correlations on the solvent itself remain, however, much…

Soft Condensed Matter · Physics 2024-01-31 Paul Robin

We re-examine the problem of the dielectric response of highly polar liquids such as water in confinement between two walls using a simple two-variable density functional theory involving number and polarisation densities. In the…

Statistical Mechanics · Physics 2023-02-08 Daniel Borgis , Damien Laage , Luc Belloni , Guillaume Jeanmairet

Antagonistic salts are composed of hydrophilic and hydrophobic ions. In a mixture solvent (water-oil) such ion pairs are preferentially attracted to water or oil, giving rise to a coupling between the charge density and the composition.…

Soft Condensed Matter · Physics 2016-04-05 Akira Onuki , Shunsuke Yabunaka , Takeaki Araki , Ryuichi Okamoto

Superdielectric behavior was observed in pastes made of high surface area alumina filled to the level of incipient wetness with water containing dissolved sodium chloride (table salt). In some cases the dielectric constants were greater…

Materials Science · Physics 2014-05-01 Jonathan Phillips