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Harnessing the enhanced light-matter coupling and quantum vacuum fluctuations resulting from mode volume compression in optical cavities is a promising route towards functionalizing quantum materials and realizing exotic states of matter.…

Strongly Correlated Electrons · Physics 2024-05-30 Emil Vinas Boström , Adithya Sriram , Martin Claassen , Angel Rubio

Materials potentially hosting Kitaev spin-liquid states are considered crucial for realizing topological quantum computing. However, the intricate nature of spin interactions within these materials complicates the precise measurement of…

Maximizing the ratio between Kitaev and residual Heisenberg interactions is a major goal in nowadays research on Kitaev-Heisenberg quantum magnets. Here we investigate Kitaev-Heisenberg exchange in a recently discovered crystalline phase of…

Strongly Correlated Electrons · Physics 2023-12-15 Pritam Bhattacharyya , Liviu Hozoi , Quirin Stahl , Jochen Geck , Nikolay A. Bogdanov

We compute the rotational anisotropy of the free energy of $\alpha$-RuCl$_3$ in an external magnetic field. This quantity, known as the magnetotropic susceptibility, $k$, relates to the second derivative of the free energy with respect to…

Strongly Correlated Electrons · Physics 2023-12-07 Toshihiro Sato , B. J. Ramshaw , K. A. Modic , Fakher F. Assaad

Spin liquids may host emergent quasiparticles, collective excitations of the spin degrees of freedom with characteristic features of Majorana fermions, which experimentally are detectable by broad excitation continua due to spin…

Strongly Correlated Electrons · Physics 2019-09-18 S. Reschke , V. Tsurkan , S. -H. Do , K. -Y. Choi , P. Lunkenheimer , Zhe Wang , A. Loidl

A prominent feature of quantum spin liquids is fractionalization of the spin degree of freedom. Fractionalized excitations have their own dynamics in different energy scales, and hence, affect finite-temperature ($T$) properties in a…

Strongly Correlated Electrons · Physics 2017-08-04 Junki Yoshitake , Joji Nasu , Yasuyuki Kato , Yukitoshi Motome

The magnetism of Kitaev materials has been widely studied, but their charge properties and the coupling to other degrees of freedom are less known. Here we investigate the charge states of $\alpha$-RuCl$_3$, a promising Kitaev quantum spin…

Strongly Correlated Electrons · Physics 2024-08-27 Xiaohu Zheng , Zhengxin Liu , Cuiwei Zhang , Huaxue Zhou , Chongli Yang , Youguo Shi , Katsumi Tanigaki , Rui-Rui Du

Mott insulators with strong spin-orbit coupling display a strongly anisotropic response to applied magnetic fields. This applies in particular to Kitaev materials, with $\alpha$-RuCl$_3$ and Na$_2$IrO$_3$ representing two important…

Strongly Correlated Electrons · Physics 2020-10-06 Eric C. Andrade , Lukas Janssen , Matthias Vojta

Ultrafast time-resolved photoinduced reflectivity is measured for the itinerant antiferromagnet UNiGa$_{5}$ ($T_{N} \approx$85 K) from room temperature to 10 K. The relaxation time $\tau$ shows a sharp increase at $T_{N}$ consistent with…

Strongly Correlated Electrons · Physics 2009-11-11 Elbert E. M. Chia , H. J. Lee , Namjung Hur , E. D. Bauer , T. Durakiewicz , R. D. Averitt , J. L. Sarrao , A. J. Taylor

$\alpha$-RuCl3 is a magnetic insulator exhibiting quantum spin liquid phases possibly found in the Kitaev honeycomb model. Much of the effort towards determining Hamiltonian parameters has focused on low magnetic field ordered phases. We…

Strongly Correlated Electrons · Physics 2023-01-05 Michael J. Lawler , Kimberly A. Modic , B. J. Ramshaw

We present thermal expansion alpha, magnetostriction and specific heat C measurements of \tal, which shows a quantum phase transition from a spin-gap phase to a Neel-ordered ground state as a function of magnetic field around H_{C0}->4.8T.…

Strongly Correlated Electrons · Physics 2009-11-11 T. Lorenz , S. Stark , O. Heyer , N. Hollmann , A. Vasiliev , A. Oosawa , H. Tanaka

Two-dimensional honeycomb antiferromagnet becomes an important class of materials as it can provide a route to Kitaev quantum spin liquid, characterized by massive quantum entanglement and fractional excitations. The signatures of its…

Ultracold atoms and molecules trapped in optical lattices are expected to serve as simulators of strongly correlated systems and topological states of matter. A fascinating example is to realize the Kitaev quantum spin liquid by using…

Strongly Correlated Electrons · Physics 2022-07-29 Kiyu Fukui , Yasuyuki Kato , Joji Nasu , Yukitoshi Motome

The pure Kitaev honeycomb model harbors a quantum spin liquid in zero magnetic fields, while applying finite magnetic fields induces a topological spin liquid with non-Abelian anyonic excitations. This latter phase has been much sought…

Strongly Correlated Electrons · Physics 2020-03-31 Dirk Wulferding , Youngsu Choi , Seung-Hwan Do , Chan Hyeon Lee , Peter Lemmens , Clement Faugeras , Yann Gallais , Kwang-Yong Choi

The Kitaev model belongs to an unconventional class of two-dimensional spin systems characterized by anisotropic, bond-dependent interactions that give rise to Quantum Spin Liquid (QSL) states. These exotic phases, marked by the absence of…

Strongly Correlated Electrons · Physics 2026-01-29 A. R. Moura , L. V. Santos

There has been a great interest in magnetic field induced quantum spin liquids in Kitaev magnets after the discovery of neutron scattering continuum and half quantized thermal Hall conductivity in the material $\alpha$-RuCl$_3$. In this…

Strongly Correlated Electrons · Physics 2020-01-10 Li Ern Chern , Ryui Kaneko , Hyun-Yong Lee , Yong Baek Kim

We introduce a matrix-product state based method to efficiently obtain dynamical response functions for two-dimensional microscopic Hamiltonians, which we apply to different phases of the Kitaev-Heisenberg model. We find significant broad…

Strongly Correlated Electrons · Physics 2017-10-18 Matthias Gohlke , Ruben Verresen , Roderich Moessner , Frank Pollmann

Recently, $\alpha$-$\textrm{RuCl}_3$ has attracted much attention as a possible material realization of the honeycomb Kitaev model, which may stabilize a quantum-spin-liquid state. Compared to extensive studies on its magnetic properties,…

In this work, we study magnetoelastic interactions by means of ultrasound experiments in $\alpha$-RuCl$_3$ -- a prototypical material for the Kitaev spin model on the honeycomb lattice, with a possible spin-liquid state featuring Majorana…

Strongly Correlated Electrons · Physics 2023-03-17 A. Hauspurg , S. Zherlitsyn , T. Helm , V. Felea , J. Wosnitza , V. Tsurkan , K. -Y. Choi , S. -H. Do , Mengxing Ye , Wolfram Brenig , Natalia B. Perkins

Fe$_3$GeTe$_2$ is a prototypical metallic van der Waals ferromagnet with itinerant magnetism and a highly tunable Curie temperature, yet how electronic excitations couple to spin and lattice degrees of freedom across its magnetic transition…

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