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The coupling of the electron system to lattice vibrations and their time-dependent control and detection provides unique insight into the non-equilibrium physics of semiconductors. Here, we investigate the ultrafast transient response of…

We analyze the effect of electron-phonon coupling on photoemission properties and ultrafast response of doped monolayer MoS2. The analysis is based on combined DFT and many-body (Eliashberg theory) approaches. In particular, we have…

Materials Science · Physics 2015-02-02 Neha Nayyar , Duy Le , Volodymyr Turkowski , Talat S. Rahman

We apply an intense infrared laser pulse in order to perturb the electronic and vibrational states in the three-dimensional charge density wave material 1$T$-VSe$_2$. Ultrafast snapshots of the light-induced hot carrier dynamics and…

We compute the phonon dispersion, density of states, and the Gr\"uneisen parameters of bulk palladium in the combined density functional theory (DFT) and dynamical mean-field theory (DMFT). We find good agreement with experimental results…

Strongly Correlated Electrons · Physics 2020-02-20 W. H. Appelt , A. Östlin , I. Di Marco , I. Leonov , M. Sekania , D. Vollhardt , L. Chioncel

The complex coupling between charge carriers and phonons is responsible for diverse phenomena in condensed matter. We apply ultrafast electron diffuse scattering to unravel electron-phonon coupling phenomena in 1T-TiSe$_2$ in both momentum…

Strongly Correlated Electrons · Physics 2021-05-14 Martin R. Otto , Jan-Hendrik Pöhls , Laurent P. René de Cotret , Mark J. Stern , Mark Sutton , Bradley J. Siwick

The broadband and ultrafast photoresponse of graphene has been extensively studied in recent years, although the photoexcited carrier dynamics is still far from being completely understood. Different experimental approaches imply either one…

Mesoscale and Nanoscale Physics · Physics 2017-08-22 Sergey Menabde , Hyunwoo Cho , Namkyoo Park

Structural phase transitions and soft phonon modes pose a longstanding challenge to computing electron-phonon (e-ph) interactions in strongly anharmonic crystals. Here we develop a first-principles approach to compute e-ph scattering and…

Materials Science · Physics 2018-12-04 Jin-Jian Zhou , Olle Hellman , Marco Bernardi

We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond…

Ultrafast electron diffraction and phonon-diffuse scattering (UED(S)) experiments make use of photo-induced changes to electron scattering intensity across 2D detectors to report on a very wide range of dynamic structural phenomena in…

Instrumentation and Detectors · Physics 2026-04-20 Laurenz Kremeyer , David Cai , Malik Lahlou , Sebastian Hammer , Raphael Schwenzer , Bradley J. Siwick

Low-energy electrons scattered in the conduction band of a dielectric solid should behave like Bloch electrons and will interact with perturbations of the atomic lattice, i.e. with phonons. Thus the phonon-based description of low-energy…

Materials Science · Physics 2009-11-13 Hans-Joachim Fitting , Vsevolod S. Kortov , Guillaume Petite

Functional nanomaterials, including 2D materials and their heterostructures are expected to impact fields ranging from catalysis, optoelectronics to nanophotonics. To realize their potential, novel experimental approaches need to be…

Mesoscale and Nanoscale Physics · Physics 2025-10-13 Cana Elgvin , Fredrik S. Hage , Khairi F. Elyas , Katja Höflich , Øystein Prytz , Christoph T. Koch , Hannah C. Nerl

Phonon scattering by electrons, or "phonon-electron scattering", has been recognized as a significant scattering channel for phonons in materials with high electron concentration, such as thermoelectrics and nanoelectronics, even at room…

Materials Science · Physics 2019-09-11 Sheng-Ying Yue , Runqing Yang , Bolin Liao

High-energy optical transitions in monolayer transition-metal dichalcogenides exhibit characteristics that are markedly distinct from those of lower-lying band-edge excitons. These differences arise from the involvement of electronic states…

Stimulated Brillouin scattering (SBS), an optical nonlinearity arising from photon-phonon interactions, has formed the basis for a large class of optical signal processing devices, including Brillouin amplifiers. A limiting factor of such…

We report on the dynamics of coherent phonons in semimetal 1T'-MoTe2 using femtosecond pump-probe spectroscopy. On an ultrafast sub-picosecond time scale at room temperature, a low frequency and long-lifetime shear phonon mode was observed…

Materials Science · Physics 2020-03-09 T. Fukuda , K. Makino , Y. Saito , P. Fons , A. V. Kolobov , K. Ueno , M. Hase

The transient evolution of carriers in an intrinsic graphene under ultrafast excitation, which is caused by the collisionless interband transitions, is studied theoretically. The energy relaxation due to the quasielastic acoustic phonon…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 P. N. Romanets , F. T. Vasko

Beta eucryptite (LiAlSiO4) shows one-dimensional super-ionic conductivity as well as anisotropic thermal expansion behavior. We have performed inelastic neutron scattering measurements in beta eucryptite over 300 to 900 K and calculated the…

We present the results of a neutron scattering study of the high energy phonons in the superconducting graphite intercalation compound CaC$_6$. The study was designed to address hitherto unexplored aspects of the lattice dynamics in…

We present a combined density-functional-perturbation-theory and inelastic neutron scattering study of the lattice dynamical properties of YNi2B2C. In general, very good agreement was found between theory and experiment for both phonon…

Superconductivity · Physics 2015-06-19 F. Weber , L. Pintschovius , W. Reichardt , R. Heid , K. -P. Bohnen , A. Kreyssig , D. Reznik , K. Hradil

The thermalization of hot carriers and phonons gives direct insight into the scattering processes that mediate electrical and thermal transport. Obtaining the scattering rates for both hot carriers and phonons currently requires multiple…