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We investigate from first-principles theory and experiment the generation of phonons on picosecond timescales and the relaxation of carriers in multiple conduction band valleys of photo-excited Ge by inter-valley electron-phonon scattering.…

Mesoscale and Nanoscale Physics · Physics 2025-02-03 F. Murphy-Armando , É. D. Murray , I. Savić , M. Trigo , D. Reis , S. Fahy

The electron-phonon coupling in ultrafast heating systems is studied within the framework of Boltzmann transport equation (BTE) with coupled electron and phonon transport. A discrete unified gas kinetic scheme is developed to solve the BTE,…

Mesoscale and Nanoscale Physics · Physics 2023-08-25 Chuang Zhang , Rulei Guo , Meng Lian , Junichiro Shiomi

Neutron resonance spin-echo spectroscopy was used to monitor the temperature evolution of the linewidths of transverse acoustic phonons in lead across the superconducting transition temperature, $T_c$, over an extended range of the…

Superconductivity · Physics 2009-11-11 T. Keller , P. Aynajian , K. Habicht , L. Boeri , S. K. Bose , B. Keimer

We analyze the effects of the electronic coupling to bosonic modes in a d-wave superconductor. The role of the scattering due to boson on the momentum transfer between electronic states in the Brilloine zone is addressed. We consider…

Superconductivity · Physics 2009-11-11 Jian-Xin Zhu , A. V. Balatsky , T. P. Devereaux , Qimiao Si , J. Lee , K. McElroy , J. C. Davis

We use ultrafast electron diffraction to detect the temporal evolution of phonon populations in femtosecond laser-excited ultrathin single-crystalline gold films. From the time-dependence of the Debye-Waller factor we extract a 4.7 ps…

A combined experimental and computational methodology for interrogating the phonon contribution to polaron formation in real materials is developed. Using LiF as an example, we show that the recent ab-initio theory of Sio et. al [PRL 122,…

Materials Science · Physics 2024-02-05 Tristan L Britt , Fabio Caruso , Bradley J Siwick

We report an inelastic neutron scattering investigation of phonons with energies up to 159 meV in the conventional superconductor YNi$_2$B$_2$C. Using the SWEEP mode, a newly developed time-of-flight technique involving the continuous…

We report the lattice dynamics of transition metal thin films by using the ultrafast electron diffraction. We observe a suppression of the diffraction intensity in a few picosecond after the photoexcitation, which is directly interpreted as…

Materials Science · Physics 2016-01-19 A. Nakamura , T. Shimojima , M. Nakano , Y. Iwasa , K. Ishizaka

Understanding nonequilibrium electron-phonon interactions at the microscopic level and on ultrafast timescales is a central goal of modern condensed matter physics. Combining time- and angle-resolved extreme ultraviolet photoemission…

Scattering between individual charges and collective modes in materials governs fundamental phenomena such as electrical resistance, energy dissipation, switching between different phases, and ordering. The study of such scattering requires…

While there are many physical processes showing subdiffusion and some useful particle models for understanding the underlying mechanisms have been established, a systematic study of subdiffusive energy transport is still lacking. Here we…

Statistical Mechanics · Physics 2022-10-05 Daxing Xiong , Jianjin Wang

The ferropnictide superconductors exhibit a sensitive interplay between the lattice and magnetic degrees of freedom, including a number of phonon modes that are much softer than predicted by nonmagnetic calculations using density functional…

Superconductivity · Physics 2014-03-13 D. Parshall , R. Heid , J. L. Niedziela , Th. Wolf , M. B. Stone , D. L. Abernathy , D. Reznik

Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the…

Electron-phonon coupling (EPC) governs lattice dynamics, charge transport, and collective electronic phases in quantum materials. In several families of unconventional superconductors, including transition-metal dichalcogenides and kagome…

We have performed extensive ab initio calculations to investigate phonon dynamics and their possible role in superconductivity in BaFe2As2 and related systems. The calculations are compared to inelastic neutron scattering data that offer…

Superconductivity · Physics 2009-11-13 M. Zbiri , H. Schober , M. R. Johnson , S. Rols , R. Mittal , Y. Su , M. Rotter , D. Johrendt

The coupling between lattice vibration quanta and valence electrons can induce charge density modulations and decisively influence the transport properties of materials, e.g. leading to conventional superconductivity. In high critical…

We present a constrained density functional perturbation theory scheme for the calculation of structural and harmonic vibrational properties of insulators in the presence of an excited and thermalized electron-hole plasma. The method is…

Materials Science · Physics 2021-10-13 Giovanni Marini , Matteo Calandra

Linear response methods are applied to identify the increase in electron-phonon coupling in elemental yttrium that is responsible for its high superconducting critical temperature Tc, which reaches nearly 20 K at 115 GPa. While the…

Superconductivity · Physics 2007-05-23 Z. P. Yin , S. Y. Savrasov , W. E. Pickett

Our examination of the interplay of ultrafast charge dynamics and electron-phonon interaction in bilayer MoS2 provides a microscopic basis for understanding the features (two peaks) in the emission spectrum. We demonstrate that while the…

Materials Science · Physics 2021-12-14 Naseem Ud Din , Volodymyr Turkowski , Talat S Rahman

An $\it{ab \,\, initio}$ based fully microscopic many-body approach is used to study the carrier relaxation dynamics in monolayer transition-metal dichalcogenides. Bandstructures and wavefunctions as well as phonon energies and coupling…

Mesoscale and Nanoscale Physics · Physics 2022-05-25 J. Hader , J. Neuhaus , J. V. Moloney , S. W. Koch