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We present an \emph{ab-initio} approach for computing the photoionization spectrum near autoionization resonances in multi-electron systems. While traditional (Hermitian) theories typically require computing the continuum states, which are…

Single molecule X-ray scattering experiments using free electron lasers hold the potential to resolve both single structures and structural ensembles of biomolecules. However, molecular electron density determination has so far not been…

Computational Physics · Physics 2026-04-17 Steffen Schultze , Helmut Grubmüller

The tomographic imaging of arbitrary molecular orbitals via high-order harmonic generation requires that electrons recollide from one direction only. Within a semi-classical model, we show that extremely short phase-stabilized laser pulses…

Atomic Physics · Physics 2009-11-13 Elmar V. van der Zwan , Manfred Lein

Recently, sparsity-based algorithms are proposed for super-resolution spectrum estimation. However, to achieve adequately high resolution in real-world signal analysis, the dictionary atoms have to be close to each other in frequency,…

Machine Learning · Statistics 2015-06-05 Yiyuan She , Huanghuang Li , Jiangping Wang , Dapeng Wu

We develop a computational method to learn a molecular Hamiltonian matrix from matrix-valued time series of the electron density. As we demonstrate for three small molecules, the resulting Hamiltonians can be used for electron density…

Computational Physics · Physics 2020-09-01 Harish S. Bhat , Karnamohit Ranka , Christine M. Isborn

In this work, we study the spectral properties of matrix Hamiltonians generated by linearizing the nonlinear Schr\"odinger equation about soliton solutions. By a numerically assisted proof, we show that there are no embedded eigenvalues for…

Analysis of PDEs · Mathematics 2015-05-18 Jeremy L. Marzuola , Gideon Simpson

We discuss a method of solving the time dependent Schrodinger equation for atoms with two active electrons in a strong laser field, which we used in a previous paper [A. Scrinzi and B. Piraux, Phys. Rev. A 56, R13 (1997)] to calculate…

Atomic Physics · Physics 2014-05-19 Armin Scrinzi , Bernard Piraux

Periodicity analysis of unevenly collected data is a relevant issue in several scientific fields. In astrophysics, for example, we have to find the fundamental period of light or radial velocity curves which are unevenly sampled…

Astrophysics · Physics 2009-10-31 R. Tagliaferri , A. Ciaramella , L. Milano , F. Barone , G. Longo

We develop the theory of pure dephasing in a solid exposed to an ultrashort laser pulse beyond the commonly used Markov approximation. This approach takes into account the finite cutoff energy of the bath and can be applied to both…

Mesoscale and Nanoscale Physics · Physics 2019-11-06 S. Yu. Kruchinin

We derive the Hamiltonian in the rotating frame for NMR quantum computing with homonucleus molecules as its computational resource. The Hamiltonian thus obtained is different from conventional Hamiltonians that appear in literature. It is…

Quantum Physics · Physics 2007-05-23 Yasushi Kondo , Mikio Nakahara , Kazuya Hata , Shogo Tanimura

Laser pulses traveling through a plasma can feature group velocities significantly differing from the speed of light in vacuum. This modifies the well-known Volkov states of an electron inside a strong laser-field from the vacuum case and…

Plasma Physics · Physics 2019-04-03 F. Mackenroth , N. Kumar , N. Neitz , C. H. Keitel

Raw images taken in low-light conditions are very noisy due to low photon count and sensor noise. Learning-based denoisers have the potential to reconstruct high-quality images. For training, however, these denoisers require large paired…

Computer Vision and Pattern Recognition · Computer Science 2025-12-04 Liying Lu , Raphaël Achddou , Sabine Süsstrunk

We introduce a pruning algorithm that provably sparsifies the parameters of a trained model in a way that approximately preserves the model's predictive accuracy. Our algorithm uses a small batch of input points to construct a data-informed…

Machine Learning · Computer Science 2021-03-16 Cenk Baykal , Lucas Liebenwein , Igor Gilitschenski , Dan Feldman , Daniela Rus

Nonlinear optical processing of ambient natural light is highly desired in computational imaging and sensing applications. A strong optical nonlinear response that can work under weak broadband incoherent light is essential for this…

We present a driving scheme for solid-state quantum emitters using frequency-swept pulses containing a spectral hole resonant with the optical transition in the emitter. Our scheme enables high-fidelity state inversion, exhibits robustness…

We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered…

Quantum Physics · Physics 2017-08-25 Jacob G. Koefoed , Søren M. M. Friis , Jesper B. Christensen , Karsten Rottwitt

Entanglement purification allows the creation of qubit pairs of arbitrarily high fidelity with respect to a maximally entangled state, starting from a larger number of low-fidelity pairs. Purification requires quantum memory, a role for…

Quantum Physics · Physics 2016-01-20 Adrian Auer , Guido Burkard

The local interaction of charges and light in organic solids is the basis of distinct and fundamental effects. We here observe, at the single molecule scale, how a focused laser beam can locally shift by hundreds-time their natural…

Deep neural networks have been successfully applied to a broad range of problems where overparametrization yields weight matrices which are partially random. A comparison of weight matrix singular vectors to the Porter-Thomas distribution…

Disordered Systems and Neural Networks · Physics 2024-01-22 Max Staats , Matthias Thamm , Bernd Rosenow

We propose a simple all-in-line single-shot scheme for diagnostics of ultrashort laser pulses, consisting of a multi-mode fiber, a nonlinear crystal and a CCD camera. The system records a 2D spatial intensity pattern, from which the pulse…

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