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Attosecond streaking camera is an ex situ technique in which a linearly polarized (LP) XUV attopulse produces an electron wavepacket by photoionization in the presence of an IR femtopulse. By moving the two synchronous oppositely circularly…

Atomic Physics · Physics 2025-11-27 M. A. H. B. Md Yusoff , H. B. Ambalampitiya , J. M. Ngoko Djiokap

We design a phase-sensitive Rydberg-atom interferometry by implementing Floquet electromagnetically induced transparency (FEIT). The FEIT mixes the sidebands of a Rydberg state induced by a MHz radio frequency (RF) field and recombines them…

Quantum Physics · Physics 2025-01-22 Yingying Han , Changfa He , Peng Xu , Yanting Zhao , Tao Wang , Weidong Li

Conical intersections between electronic states often dictate the chemistry of photoexcited molecules. Recently developed sources of ultrashort extreme ultraviolet (XUV) pulses tuned to element-specific transitions in molecules allow for…

We realize and model a Rydberg-state atom interferometer for measurement of phase and intensity of radio-frequency (RF) electromagnetic waves. A phase reference is supplied to the atoms via a modulated laser beam, enabling atomic…

We develop a novel technique for modeling of atomic and molecular ionization in superposition of XUV and IR fields with characteristics typical for attosecond streaking and RABBITT experiments. The method is based on solving the…

Atomic Physics · Physics 2016-06-29 Vladislav V. Serov , A. S. Kheifets

Using a spectrally resolved electron interferometry technique, we measure photoionization time delays between the $3s$ and $3p$ subshells of argon over a large 34-eV energy range covering the Cooper minima in both subshells. The observed…

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…

Atomic Physics · Physics 2015-05-28 Feng He , Camilo Ruiz , Andreas Becker , Uwe Thumm

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

Atomic Physics · Physics 2017-03-08 Lisa Torlina , Olga Smirnova

Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a powerful photoelectron spectroscopy, offering direct access to internal dynamics of the target. It is being increasingly applied to molecular…

Chemical Physics · Physics 2023-04-10 Serguei Patchkovskii , Jakub Benda , Dominik Ertel , David Busto

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…

Atomic Physics · Physics 2020-02-19 C. Figueira de Morisson Faria , A. S. Maxwell

The introduction of mid-IR optical parametric chirped pulse amplifiers (OPCPAs) has catalyzed interest in multi-millijoule, infrared femtosecond pulse-based filamentation. As tunneling ionization is a fundamental first stage in these…

Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field's oscillation period. However, synthesizing such a gate pulse is…

We analyze interference processes in atomic ionization induced by a two-color laser with fundamental frequency $\omega $ and its second harmonic $2\omega $. The interplay between inter- and intracycle interference processes give rise to…

Atomic Physics · Physics 2021-09-13 Diego G. Arbó , Sebastián D. López

Wave front sensing of the surface of equal phase for a propagating electromagnetic wave is a vital technology in fields ranging from real time adaptive optics, to high accuracy metrology, to medical optometry. We have developed a new method…

Optics · Physics 2025-10-01 C. L. Carilli , L. Torino , B. Nikolic , N. Thyagarajan , U. Iriso

Precise measurement of the angular deviation of an object is a common task in science and technology. Many methods use light for this purpose. Some of these exploit interference effects to achieve technological advantages, such as…

Quantum Physics · Physics 2020-08-19 G. H. Aguilar , R. S. Piera , P. L. Saldanha , R. L. de Matos Filho , S. P. Walborn

The kinetic energy of an atom recoiling due to absorption of a photon was measured as a frequency using an interferometric technique called ``contrast interferometry''. Optical standing wave pulses were used as atom-optical elements to…

Condensed Matter · Physics 2009-11-07 S. Gupta , K. Dieckmann , Z. Hadzibabic , D. E. Pritchard

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

We present a novel technique to assess the focal volume of petawatt-class lasers at full power. Our approach exploits quantitative measurement of the angular distribution of electrons born in the focus via ionization of rarefied gas, which…

We present an \emph{ab-initio} approach for computing the photoionization spectrum near autoionization resonances in multi-electron systems. While traditional (Hermitian) theories typically require computing the continuum states, which are…

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