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PrV2Al20 is the heavy fermion superconductor based on the cubic Gamma3 doublet that exhibits non- magnetic quadrupolar ordering below ~ 0.6 K. Our magnetotransport study on PrV2Al20 reveals field-induced quadrupolar quantum criticality at…

Strongly Correlated Electrons · Physics 2016-10-31 Yasuyuki Shimura , Masaki Tsujimoto , Bin Zeng , Luis Balicas , Akito Sakai , Satoru Nakatsuji

Strange-metal behavior observed in the praseodymium-based heavy-fermion material PrV2Al20 has been tentatively interpreted in the framework of proximity to a quantum critical point (QCP) associated with quadrupolar ordering. Here, we…

Strongly Correlated Electrons · Physics 2024-10-10 Marvin Lenk , Fei Gao , Johann Kroha , Andriy H. Nevidomskyy

Our single crystal study reveals that PrTr2Al20 (Tr = Ti and V) provides the first examples of a cubic {\Gamma}3 nonmagnetic ground doublet system that shows the Kondo effect including a -ln T dependent resistivity. The {\Gamma}3…

Strongly Correlated Electrons · Physics 2015-03-19 Akito Sakai , Satoru Nakatsuji

The cubic compound PrTi$_2$Al$_{20}$ is a quadrupolar Kondo lattice system that exhibits quadrupolar ordering due to the non-Kramers $\Gamma_3$ ground doublet and has strong hybridization between $4f$ and conduction electrons. Our study…

Strongly Correlated Electrons · Physics 2015-06-05 Akito Sakai , Kentaro Kuga , Satoru Nakatsuji

Orbital degrees of freedom in condensed matters could play important roles in forming a variety of exotic electronic states by interacting with conduction electrons. In 4f electron systems, because of strong intra-atomic spin-orbit…

Strongly Correlated Electrons · Physics 2016-08-24 T. Onimaru , K. Izawa , K. T. Matsumoto , T. Yoshida , Y. Machida , T. Ikeura , K. Wakiya , K. Umeo , S. Kittaka , K. Araki , T. Sakakibara , T. Takabatake

In non-Kramers Kondo systems with a quadrupolar degrees of freedom, an ordinary magnetic Kondo effect can compete with the quadrupolar Kondo effect. We discuss such competition keeping Pr$T_{2}$Zn$_{20}$ ($T$=Ir, Rh) and Pr$T_{2}$Al$_{20}$…

Strongly Correlated Electrons · Physics 2016-06-22 Hiroaki Kusunose

Among heavy fermion materials, there is a set of rare-earth intermetallics with non-Kramers Pr$^{3+}$ $4f^2$ moments which exhibit a rich phase diagram with intertwined quadrupolar orders, superconductivity, and non-Fermi liquid behavior.…

Strongly Correlated Electrons · Physics 2018-03-08 Frederic Freyer , Jan Attig , SungBin Lee , Arun Paramekanti , Simon Trebst , Yong Baek Kim

PrV$_2$Al$_{20}$ is a rare example of a heavy fermion system based on strong hybridization between conduction electrons and nonmagnetic quadrupolar moments of the cubic $\Gamma_3$ ground doublet. Here, we report that a high-quality single…

Strongly Correlated Electrons · Physics 2015-06-22 Masaki Tsujimoto , Yosuke Matsumoto , Takahiro Tomita , Akito Sakai , Satoru Nakatsuji

Electrical resistivity $\rho(T)$ and specific heat $C(T)$ measurements have been made on the diluted 4$f^2$ system Y(Pr)Ir$_2$Zn$_{20}$. Both data of $\rho$ and magnetic specific heat $C_{\rm m}$ per Pr ion are well scaled as a function of…

Strongly Correlated Electrons · Physics 2018-08-22 Y. Yamane , T. Onimaru , K. Wakiya , K. T. Matsumoto , K. Umeo , T. Takabatake

Multipolar Kondo systems offer unprecedented opportunities for designing astonishing quantum phases and functionalities beyond spin-only descriptions. A model material platform of this kind is the cubic heavy-fermion system…

Strongly Correlated Electrons · Physics 2023-08-29 Takachika Isomae , Akito Sakai , Mingxuan Fu , Takanori Taniguchi , Masashi Takigawa , Satoru Nakatsuji

A scaling consideration of the Kondo lattices is performed with account of singularities in the spin excitation spectral function. It is shown that a non-Fermi-liquid (NFL) behavior between two critical values of the bare $s-f$ coupling…

Strongly Correlated Electrons · Physics 2009-10-31 V. Yu. Irkhin , M. I. Katsnelson

We present a single crystal study of low temperature magnetism and transport in Sm$Tr_2$Al$_{20}$ ($Tr =$ Ti, V and Cr). Strong valence fluctuation is manifested as Kondo effects including a large Sommerfeld coefficient $\gamma$, a weak…

Strongly Correlated Electrons · Physics 2015-05-30 Akito Sakai , Satoru Nakatsuji

We have measured the specific heat of PrV$_2$Al$_{20}$ at very low temperatures, using high quality single crystals with the residual resistivity ratio ~ 20. The high-quality single crystals exhibit clear double transitions at $T_{\rm Q} =$…

Strongly Correlated Electrons · Physics 2015-06-23 Masaki Tsujimoto , Yosuke Matsumoto , Satoru Nakatsuji

We discuss possible competition between magnetic and quadrupole Kondo effects in non-Kramers doublet systems under cubic symmetry. The quadrupole Kondo effect leads to non-Fermi-liquid (NFL) ground state, while the magnetic one favors…

Strongly Correlated Electrons · Physics 2015-06-22 Hiroaki Kusunose , Takahiro Onimaru

We report magnetization, heat capacity and electrical resistivity for a newly discovered heavy fermion (HF) compound $\mathrm{YbV_6Sn_6}$ which is crystallized in a hexagonal $\mathrm{HfFe_6Ge_6}$-type structure, highlighted by the stacking…

Strongly Correlated Electrons · Physics 2023-06-07 Kaizhen Guo , Junyao Ye , Shuyue Guan , Shuang Jia

We consider an interacting nanowire/superconductor heterostructure attached to metallic leads. The device is described by an unusual low-energy model involving spin-1 conduction electrons coupled to a nonlocal spin-1/2 Kondo impurity built…

Strongly Correlated Electrons · Physics 2014-02-11 Martin R. Galpin , Andrew K. Mitchell , Jesada Temaismithi , David E. Logan , Benjamin Béri , Nigel R. Cooper

Notable non-Fermi liquid and quantum critical behaviors are observed in rare-earth metallic systems with non-Kramers local moments supporting a number of different multipolar moments. A prominent example is…

Strongly Correlated Electrons · Physics 2022-11-24 SangEun Han , Daniel J. Schultz , Yong Baek Kim

Recent experiments have examined the impact of a magnetic field on ferroquadrupolar orders in the intermetallic Kondo material PrTi$_2$Al$_{20}$. Motivated by this, we use extensive Monte Carlo simulations to study a diamond lattice XY…

Strongly Correlated Electrons · Physics 2020-08-04 Frederic Freyer , SungBin Lee , Yong Baek Kim , Simon Trebst , Arun Paramekanti

Recent experiments on quantum criticality in the Ge-substituted heavy-electron material YbRh2Si2 under magnetic field have revealed a possible non-Fermi liquid (NFL) strange metal (SM) state over a finite range of fields at low…

Strongly Correlated Electrons · Physics 2018-01-31 Yung-Yeh Chang , Silke Paschen , Chung-Hou Chung

CeRh2As2 has recently been reported to be a rare case of multi-phase unconventional superconductor [S. Khim et al., arXiv:2101.09522] close to a quantum critical point (QCP). Here, we present a comprehensive study of its normal state…

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