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Related papers: High-precision methanol spectroscopy with a widely…

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For the growing demand of frequency combs in mid-infrared (mid-IR), known as the "molecular fingerprint" region of the spectrum [1], down conversion of near-IR frequency combs through half- harmonic generation offers numerous benefits…

Optics · Physics 2015-10-14 Alireza Marandi , Kirk A. Ingold , Marc Jankowski , Robert L. Byer

Dissipative solitons formed in Kerr microresonators may enable chip-scale frequency combs for precision optical metrology. Here we explore the creation of an octave-spanning, 15-GHz repetition-rate microcomb suitable for both f-2f…

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

Photometric instruments operating at far infrared to millimetre wavelengths often have broad spectral passbands (central wavelength/bandwidth ~ 3 or less), especially those operating in space. A broad passband can result in significant…

We report accurate laboratory measurements of selected methanol transition frequencies between 0.834 and 230 GHz in order to facilitate astronomical velocity analyses. New data have been obtained between 10 and 27 GHz and between 60 and 119…

Astrophysics · Physics 2011-03-02 H. S. P. Mueller , K. M. Menten , H. Maeder

Coherent dual-comb spectroscopy (DCS) enables high-resolution measurements at high speeds without the trade-off between resolution and update rate inherent to mechanical delay scanning approaches. However, high system complexity and limited…

The realization of ultrahigh quality (Q) resonators regardless of the underpinning material platforms has been a ceaseless pursuit, because the high Q resonators provide an extreme environment of storage of light to enable observations of…

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

We demonstrate the performance of a dual frequency comb QCL spectrometer for the application of vibrational Stark spectroscopy. Measurements performed on fluorobenzene with the dual-comb spectrometer (DCS) were compared to results obtained…

Chemical Physics · Physics 2019-11-22 Urszula Szczepaniak , Samuel H. Schneider , Raphael Horvath , Jacek Kozuch , Markus Geiser

We report on the engineering of broadband quantum cascade lasers (QCLs) emitting at Terahertz (THz) frequencies, which exploit a heterogeneous active region scheme and have a current density dynamic range (Jdr) of 3.2, significantly larger…

We demonstrate the first application of a liquid-metal ion source for collinear laser spectroscopy in proof-of-principle measurements on naturally abundant In$^+$. The superior beam quality, i.e., the actively stabilized current and energy…

A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric…

High finesse frequency combs (HFC) with large ratio of the frequency spacing to the width of the spectral components have demonstrated remarkable results in many applications such as precision spectroscopy and metrology. We found that low…

Thanks to intrinsically short electronic relaxation on the ps time scale, III-V semiconductor unipolar devices are ideal candidates for ultrahigh-speed operation at mid-infrared frequencies. In this work, antenna-coupled, GaAs-based multi…

Instrumentation and Detectors · Physics 2024-06-13 Quyang Lin , Michael Hakl , Sylvie Lepillet , Hua Li , Jean-Francois Lampin , Emilien Peytavit , Stefano Barbieri

Applications relying on mid-infrared radiation (Mid-IR, $\lambda\sim$ 3-30 $\mu$m) have progressed at a very rapid pace in recent years, stimulated by scientific and technological breakthroughs. Mid-IR cameras have propelled the field of…

Frequency combs based on nonlinear-optical phenomena in integrated photonics are a versatile light source that can explore new applications, including frequency metrology, optical communications, and sensing. We demonstrate robust…

Harnessing the quantum interference of photon-pair generation processes, infrared quantum absorption spectroscopy (IRQAS) can extract the infrared optical properties of a sample through visible or near-infrared photon detection without the…

Optics · Physics 2022-06-22 Yu Mukai , Ryo Okamoto , Shigeki Takeuchi

Using a turn-key Ti:sapphire femtosecond laser frequency comb, an off-the-shelf supercontinuum device, and Fabry-Perot mode filters, we report the generation of a 16 GHz frequency comb spanning a 90 nm band about a center wavelength of 566…

High-speed measurement confronts the extreme speed limit when the signal becomes comparable to the noise level. In the context of broadband mid-infrared spectroscopy, state-of-the-art ultrafast Fourier-transform infrared spectrometers, in…

A laser frequency combs is a broad spectrum composed of equidistant narrow lines. Initially invented for frequency metrology, such combs enable new approaches to spectroscopy over broad spectral bandwidths, of particular relevance to…

Optics · Physics 2019-03-01 Nathalie Picqué , Theodor W. Hänsch