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We report Monte Carlo simulations of a lattice-polymer model that can account for both polymer crystallization and liquid-liquid demixing in solutions of semiflexible homopolymers. In our model, neighboring polymer segments can have…

Soft Condensed Matter · Physics 2009-11-07 Wenbing Hu , Daan Frenkel , Vincent B. F. Mathot

We propose a highly coarse-grained simulation model for crystalline polymer solids with crystalline lamellar structures. The mechanical properties of a crystalline polymer solid are mainly determined by the crystalline lamellar structures.…

Soft Condensed Matter · Physics 2025-01-13 Takashi Uneyama

Two types of high-strength composite hydrogels possessing the structure of interpenetrating polymer networks were synthesized via free-radical polymerization of acrylamide carried out straight within the matrix of plant or bacterial…

Chemical Physics · Physics 2019-04-02 Alexander Buyanov , Iosif Gofman , Natalya Saprykina

We exploit the controlled drying of millimeter-sized gel beads to investigate isotropic compression of colloidal fractal gels. Using a custom dynamic light scattering setup, we demonstrate that stresses imposed by drying on the bead surface…

Soft Condensed Matter · Physics 2026-01-22 M. Milani , E. Cavalletti , V. Ruzzi , A. Martinelli , P. Dieudonne-George , C. Ligoure , T. Phou , L. Cipelletti , L. Ramos

Liquid crystal elastomers (LCEs) are soft phase-changing solids that exhibit large reversible contractions upon heating, Goldstone-like soft modes and resultant microstructural instabilities. We heat a planar LCE slab to isotropic, clamp…

Soft Condensed Matter · Physics 2023-12-04 Morgan Barnes , Fan Feng , John S. Biggins

Soft materials, such as colloidal suspensions, polymer solutions, and biological systems, are typically multicomponent mixtures of macromolecules and simpler components (e.g., microions, monomers, solvent) that can assemble into complex…

Soft Condensed Matter · Physics 2015-05-13 Alan R. Denton

Bio-conjugated nanomaterials play a promising role in the development of novel supramolecular structures, molecular machines, and biosensing devices. In this study, lipid-conjugated gold nanoparticles were synthesized and allowed to form a…

Materials Science · Physics 2012-07-24 Subhasish Chatterjee , Markrete Krikorian , Harry D. Gafney , Bonnie Gersten

We have performed parallel tempering Monte Carlo simulations using a simple continuum heteropolymer model for proteins. All ten heteropolymer sequences which we have studied have shown first-order transitions at low temperature to ordered…

Soft Condensed Matter · Physics 2010-01-05 J. E. Magee , J. Warwicker , L. Lue

Astrophysical gases such as the interstellar-, circumgalactic- or intracluster-medium are commonly multiphase, which poses the question of the structure of these systems. While there are many known processes leading to fragmentation of cold…

Astrophysics of Galaxies · Physics 2023-07-18 Max Gronke , S. Peng Oh

Hydrogels are widespread soft materials, which can serve a wide range of applications. The control over the viscoelastic properties of the gel is of paramount importance. Ongoing environmental issues have raised the consumer's concern…

Soft Condensed Matter · Physics 2022-12-23 Chloé Seyrig , Alexandre Poirier , Thomas Bizien , Niki Baccile

Understanding the complex self-assembly of biomacromolecules is a major outstanding question. Microtubules are one example of a biopolymer that possesses characteristics quite distinct from standard synthetic polymers that are derived from…

Soft Condensed Matter · Physics 2013-01-10 Shengfeng Cheng , Ankush Aggarwal , Mark J. Stevens

Short DNA linkers are increasingly being exploited for driving specific self-assembly of Brownian objects. DNA-functionalised colloids can assemble into ordered or amorphous materials with tailored morphology. Recently, the same approach…

Soft Condensed Matter · Physics 2015-01-12 Lucia Parolini , Bortolo M. Mognetti , Jurij Kotar , Erika Eiser , Pietro Cicuta , Lorenzo Di Michele

Microgels are soft colloidal particles constituted by cross-linked polymer networks with a high potential for applications. In particular, after adsorption at a fluid interface, interfacial tension provides two-dimensional (2D) confinement…

Soft Condensed Matter · Physics 2021-09-03 Jacopo Vialetto , Natalie Nussbaum , Jotam Bergfreund , Peter Fischer , Lucio Isa

We investigate a lattice model of polymers where the nearest-neighbour monomer-monomer interaction strengths differ according to whether the local configurations have so-called ``hydrogen-like'' formations or not. If the interaction…

Soft Condensed Matter · Physics 2009-11-13 J Krawczyk , A L Owczarek , T Prellberg

Using exhaustive Monte Carlo simulations we study the kinetics and mechanism of fibril formation using lattice models as a function of temperature and the number of chains. While these models are, at best, caricatures of peptides, we show…

Biomolecules · Quantitative Biology 2009-11-13 Mai Suan Li , D. K. Klimov , J. E. Straub , D. Thirumalai

The simulation of industrial processes involving cold compaction of powders allows for the optimization of the production of both traditional and advanced ceramics. The capabilities of a constitutive model previously proposed by the authors…

Materials Science · Physics 2014-04-30 S. Stupkiewicz , A. Piccolroaz , D. Bigoni

By means of multicanonical computer simulations, we investigate thermodynamic properties of the aggregation of interacting semiflexible polymers. We analyze a mesoscopic bead-stick model, where nonbonded monomers interact via Lennard-Jones…

Soft Condensed Matter · Physics 2015-05-28 Christoph Junghans , Michael Bachmann , Wolfhard Janke

Hydrogels are soft materials engineered to suit a multitude of applications that exploit their tunable mechanochemical properties. Dynamic hydrogels employing noncovalent, physically crosslinked networks dominated by either enthalpic or…

Soft Condensed Matter · Physics 2023-11-28 Samya Sen , Anthony C. Yu , Changxin Dong , Andrea I. D'Aquino , Eric A. Appel

We analyze plane strain cold rolling processes, at large strains but slow strain rates, by finite element modeling. At low temperatures, slow strain rates, and moderate thickness reductions during rolling (at which Bauschinger effect can be…

Soft Condensed Matter · Physics 2022-06-30 Nikhil Padhye

Softer means stickier for solid adhesives, because material compliance facilitates close contact between non-conformal surfaces. Recent discoveries have revealed that soft materials can exhibit a rich array of new physics arising from…