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In polar semiconductors and oxides, the long-range nature of the electron-phonon (\textit{e}-ph) interaction is a bottleneck to compute charge transport from first principles. Here, we develop an efficient ab initio scheme to compute and…

Materials Science · Physics 2016-12-07 Jin-Jian Zhou , Marco Bernardi

In this article we propose two novel 3D finite element models, denoted method A and B, for electron and hole Drift-Diffusion (DD) current densities. Method A is based on a primal-mixed formulation of the DD model as a function of the…

Numerical Analysis · Mathematics 2014-12-12 Aurelio Mauri , Andrea Bortolossi , Giovanni Novielli , Riccardo Sacco

In this paper, we propose a new framework named Communication Optimal Transport (CommOT) for computing the rate distortion (RD) function. This work is motivated by observing the fact that the transition law and the relative entropy in…

Information Theory · Computer Science 2022-12-21 Shitong Wu , Wenhao Ye , Hao Wu , Huihui Wu , Wenyi Zhang , Bo Bai

Computational physics simulation can be a powerful tool to accelerate industry deployment of new scientific technologies. However, it must address the challenge of computationally tractable, moderately accurate prediction at large industry…

We present a real-space method for first-principles nano-scale electronic transport calculations. We use the non-equilibrium Green's function method with density functional theory and implement absorbing boundary conditions (ABCs, also…

Mesoscale and Nanoscale Physics · Physics 2014-07-29 Baruch Feldman , Tamar Seideman , Oded Hod , Leeor Kronik

Based on structure prediction method, the machine learning method is used instead of the density function theory (DFT) method to predict the material properties, thereby accelerating the material search process. In this paper, we…

Materials Science · Physics 2020-07-17 Wen Tong , Qun Wei , Haiyan Yan , Meiguang Zhang , Xuanmin Zhu

We present an ab initio calculation of the DC conductivity of amorphous silicon and hydrogenated amorphous silicon. The Kubo-Greenwood formula is used to obtain the DC conductivity, by thermal averaging over extended dynamical simulation.…

Materials Science · Physics 2009-11-13 T. A. Abtew , M. Zhang , D. A. Drabold

Pairing the accuracy of Kohn-Sham density-functional framework with the efficiency of a stochastic algorithmic approach, mixed stochastic-deterministic Density Functional Theory (mDFT) achieves a favorable computational scaling with system…

Chemical Physics · Physics 2025-10-07 Vidushi Sharma , Lee A. Collins , Alexander J. White

We report the derivation and implementation of orbital optimization algorithms for the active space decomposition (ASD) model, which are extensions of complete active space self-consistent field (CASSCF) and its occupation-restricted…

Chemical Physics · Physics 2015-08-17 Inkoo Kim , Shane M. Parker , Toru Shiozaki

Fullerene like cages and naonotubes of carbon and other inorganic materials are currently under intense study due to their possible technological applications. First principle simulations of these materials are computationally challenging…

Materials Science · Physics 2007-05-23 Rajendra R. Zope , Brett I. Dunlap

We present a novel implementation of the first-principles approach to molecular charge transport using the non-equilibrium Green's function formalism in combination with the ADF/BAND periodic band-structure DFT code, together with results…

Materials Science · Physics 2014-03-18 C. J. O. Verzijl , J. M. Thijssen

The cluster multipole (CMP) expansion for magnetic structures provides a scheme to systematically generate candidate magnetic structures specifically including noncollinear magnetic configurations adapted to the crystal symmetry of a given…

Materials Science · Physics 2021-02-19 Marie-Therese Huebsch , Takuya Nomoto , Michi-To Suzuki , Ryotaro Arita

In this paper, we present ab initio computer models of Cu-doped amorphous Ta2O5 , a promising candidate for Conducting Bridge Random Access Memory (CBRAM) memory devices, and study the structural, electronic, charge transport and…

Materials Science · Physics 2020-07-01 Rajendra Thapa , Bishal Bhattarai , M. N. Kozicki , Kashi N. Subedi , D. A. Drabold

We present a methodology to calculate radiative carrier capture coefficients at deep defects in semiconductors and insulators from first principles. Electronic structure and lattice relaxations are accurately described with hybrid density…

Materials Science · Physics 2020-08-07 Cyrus E. Dreyer , Audrius Alkauskas , John L. Lyons , Chris G. Van de Walle

We present a first-principles framework to extract deformation potentials in Silicon based on density-functional theory (DFT) and density-functional perturbation theory (DFPT). We compute the electronic band structures, phonon dispersion…

Materials Science · Physics 2021-11-05 Zhen Li , Patrizio Graziosi , Neophytos Neophytou

Kinetic transport equations are notoriously difficult to simulate because of their complex multiscale behaviors and the need to numerically resolve a high dimensional probability density function. Past literature has focused on building…

Numerical Analysis · Mathematics 2022-11-10 Zhichao Peng , Yanlai Chen , Yingda Cheng , Fengyan Li

Liquid NaSn alloys in five different compositions (20, 40, 50, 57 and 80% sodium) are studied using density functional calculations combined with molecular dynamics(Car-Parrinello method). The frequency-dependent electric conductivities for…

mtrl-th · Physics 2009-10-30 R. Kaschner , M. Schoene , G. Seifert , G. Pastore

This chapter concerns with the recent development of a new DFT methodology for accurate, reliable prediction of many-electron systems. Background, need for such a scheme, major difficulties encountered, as well as their potential remedies…

Chemical Physics · Physics 2019-04-19 Amlan K. Roy

A novel, general Green's function technique for elastic spin-dependent transport calculations is presented, which (i) scales linearly with system size and (ii) allows straightforward application to general tight-binding Hamiltonians (spd in…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 S. Sanvito , C. J. Lambert , J. H. Jefferson , A. M. Bratkovsky

Significant progress on parameter-free calculations of carrier mobilities in real materials has been made during the past decade; however, the role of various approximations remains unclear and a unified methodology is lacking. Here, we…

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