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Combining quasistatic and time-resolved transport measurements with X-ray and neutron diffraction experiments we study the non-equilibrium states that arise in pure and in Ti substituted Ca$_2$RuO$_4$ under the application of current…

Strongly Correlated Electrons · Physics 2020-08-12 K. Jenni , F. Wirth , K. Dietrich , L. Berger , Y. Sidis , S. Kunkemöller , C. P. Grams , D. I. Khomskii , J. Hemberger , M. Braden

We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the…

Strongly Correlated Electrons · Physics 2009-11-10 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

An appealing direction to change the properties of strongly correlated materials is to induce nonequilibrium steady states by the application of a direct current. While access to these novel states is of high scientific interest, Joule…

Strongly Correlated Electrons · Physics 2024-07-26 Giordano Mattoni , Kazumi Fukushima , Shingo Yonezawa , Fumihiko Nakamura , Yoshiteru Maeno

A comprehensive study of the behavior of the Mott insulator Ca_2RuO_4 under electrical current drive is performed by combining two experimental probes: the macroscopic electrical transport and the microscopic X-Ray diffraction. The…

Strongly Correlated Electrons · Physics 2020-01-01 C. Cirillo , V. Granata , G. Avallone , R. Fittipaldi , C. Attanasio , A. Avella , A. Vecchione

The electric-current stabilized semi-metallic state in the quasi-two-dimensional Mott insulator Ca$_2$RuO$_4$ exhibits an exceptionally strong diamagnetism. Through a comprehensive study using neutron and X-ray diffraction, we show that…

We derive and employ a semi-classical Langevin equation obtained from path-integrals to describe the ionic dynamics of a molecular junction in the presence of electrical current. The electronic environment serves as an effective…

Mesoscale and Nanoscale Physics · Physics 2012-07-03 Jing Tao Lü , Mads Brandbyge , Per Hedegård , Tchavdar N. Todorov , Daniel Dundas

The novel ferroelectric-like structural transition observed in metallic LiOsO$_3$ [Y. Shi et al., Nat. Mater. 12, 1024 (2013)], has invoked many theoretical and experimental interests. In this work, we have performed polarized and…

Materials Science · Physics 2017-03-09 Feng Jin , Anmin Zhang , Jianting Ji , Kai Liu , Le Wang , Youguo Shi , Yong Tian , Xiaoli Ma , Qingming Zhang

Raman scattering experiments have been carried out on single crystals of Nd$_{0.5}$Sr$_{0.5}$MnO$_3$ as a function of temperature in the range of 320-50 K, covering the paramagnetic insulator-ferromagnetc metal transition at 250 K and the…

Materials Science · Physics 2007-05-23 Md. Motin Seikh , A. K. Sood , Chandrabhas Narayana

This is a preliminary acount of a theory for Raman scattering by current-carrying molecular junctions. The approach combines a non-equilibrium Green's function (NEGF) description of the non-equilibrium junction with a generalized scattering…

Mesoscale and Nanoscale Physics · Physics 2009-04-09 Michael Galperin , Mark A. Ratner , Abraham Nitzan

Electronic Raman scattering and optical phonon self-energies are studied on single crystals of $LuB_{12}$ with different isotopic composition in the temperature region 10-650K and at pressures up to 10 GPa. The shape and energy position of…

Materials Science · Physics 2016-08-09 Yu. S. Ponosov , A. A. Makhnev , S. V. Streltsov , V. B. Filipov , N. Yu. Shitsevalova

We investigated nonlinear conduction in bulk single crystals of VO2 with precise temperature control. Two distinct nonequilibrium phenomena were identified: a gradual reduction of the charge gap and a current-induced insulator-metal…

Strongly Correlated Electrons · Physics 2025-05-13 Akitoshi Nakano , Masato Imaizumi , Ichiro Terasaki

Polarized Raman scattering spectra of superconducting K$_x$Fe$_{2-y}$Se$_2$ and nonsuperconducting K$_{0.8}$Fe$_{1.8}$Co$_{0.2}$Se$_2$ single crystals were measured in a temperature range from 10 K up to 300 K. Two Raman active modes from…

Materials Science · Physics 2016-09-20 M. Opačić , N. Lazarević , M. Šćepanović , Hyejin Ryu , Hechang Lei , C. Petrovic , Z. V. Popović

We report on Raman scattering measurements of the A-site ordered YBaMn2O6 in the wide temperature range of 10-650K. Upon cooling almost all phonon modes show pronounced temperature dependencies of frequency, linewidth, and scattering…

Strongly Correlated Electrons · Physics 2009-09-30 X. N. Zhang , K. -Y. Choi , P. Lemmens , T. Nakajima , Y. Ueda

We report Raman scattering measurement of charge nematic fluctuations in the tetragonal phase of BaFe$_2$As$_2$ and Sr(Fe$_{1-x}$Co$_x$)$_2$As$_2$ (x=0.04) single crystals. In both systems, the observed nematic fluctuations are found to…

Current-driven insulator-metal transitions are in many cases driven by Joule heating proportional to the square of the applied current. Recent nano-imaging experiments in Ca$_2$RuO$_4$ reveal a metal-insulator phase boundary that depends on…

Strongly Correlated Electrons · Physics 2020-08-12 Giuliano Chiriacò , Andrew Millis

We investigate a lateral semiconductor quantum dot with a large number of electrons in the semi-open Fano regime. In transport measurements we observe three stable series of Fano resonances with similar lineshapes. We present a simple model…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. Fuhner , U. F. Keyser , R. J. Haug , D. Reuter , A. D. Wieck

Magnetic Raman scattering from a frustrated spin-1/2 Heisenberg-chain is considered with a focus on the uniform phase of the spin-Peierls compound CuGeO_3. The Raman intensity is analyzed in terms of a Loudon-Fleury scattering process using…

Strongly Correlated Electrons · Physics 2016-08-31 Wolfram Brenig

Surface enhanced Raman spectra from molecules (bipyridyl ethylene) adsorbed on gold dumbells are observed to become increasingly asymmetric (Fano-like) at higher incident light intensity. The electronic temperature (inferred from the…

Mesoscale and Nanoscale Physics · Physics 2016-01-12 S. Dey , M. Banik , E. Hulkko , K. Rodriguez , V. A. Apkarian , M. Galperin , A. Nitzan

We present Raman scattering studies of the structural and magnetic phases that accompany temperature- and field-dependent melting of charge- and orbital-order (COO) in La0.5Ca0.5MnO3 and La0.25Pr0.375Ca0.375MnO3. Our results show that…

Strongly Correlated Electrons · Physics 2016-08-14 M. Kim , H. Barath , S. L. Cooper , P. Abbamonte , E. Fradkin , M. Rübhausen , C. L. Zhang , S-W. Cheong

We report a Raman scattering study of nematic degrees of freedom in the iron-based superconductor parent compound BaFe$_2$As$_2$ under tunable uniaxial strain. We demonstrate that the polarization resolved arsenic (As) phonon intensity can…

Superconductivity · Physics 2022-02-02 J. -C. Philippe , J. Faria , A. Forget , D. Colson , S. Houver , M. Cazayous , A. Sacuto , Y. Gallais
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