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The dynamics of vibrational wave packets in triplet states of rubidium dimers (Rb2) formed on helium nanodroplets are studied using femtosecond pump-probe photoionization spectroscopy. Due to fast desorption of the excited Rb2 molecules off…

Atomic and Molecular Clusters · Physics 2011-12-19 M. Mudrich , Ph. Heister , T. Hippler , Ch. Giese , O. Dulieu , F. Stienkemeier

We report here a molecular dynamics simulation study on water and aqueous LiCl solutions confined in 1.6 nm cylindrical pores of silica to investigate a dynamical cross-over, observed earlier experimentally, wherein LiCl slows down confined…

Soft Condensed Matter · Physics 2025-04-10 Siddharth Gautam , Lukas Vlcek , Eugene Mamontov , David Cole

We theoretically study physical properties of one-dimensionally and regularly placed solutes. The solute is rigid-body, has arrow-like shape, and changes its direction up or down. If the solutes are immersed in continuum solvent, nothing…

Chemical Physics · Physics 2011-10-19 Ken-ichi Amano

Using molecular dynamics simulations, we study supercritical fluids near the gas-liquid critical point under heat flow in two dimensions. We calculate the steady-state temperature and density profiles. The resultant thermal conductivity…

Statistical Mechanics · Physics 2009-11-10 Toshiyuki Hamanaka , Ryoichi Yamamoto , Akira Onuki

A good representation of mesoscopic fluids is required to combine with molecular simulations at larger length and time scales (De Fabritiis {\it et. al}, Phys. Rev. Lett. 97, 134501 (2006)). However, accurate computational models of the…

Fluid Dynamics · Physics 2015-06-26 G. De Fabritiis , M. Serrano , R. Delgado-Buscalioni , P. V. Coveney

The liquid-liquid phase separation of biomolecules is an important process for intracellular organization. Biomolecular sequence combinatorics leads to a large variety of proteins and nucleic acids which can interact to form a diversity of…

Soft Condensed Matter · Physics 2025-08-27 Aria S. Chaderjian , Sam Wilken , Omar A. Saleh

The coherence time of an electron spin decohered by the nuclear spin environment in a quantum dot can be substantially increased by subjecting the electron to suitable dynamical decoupling sequences. We analyze the performance of high-level…

Mesoscale and Nanoscale Physics · Physics 2008-03-27 Wenxian Zhang , N. P. Konstantinidis , V. V. Dobrovitski , B. N. Harmon , Lea F. Santos , Lorenza Viola

Electric deflection measurements on liquid helium nanodroplets doped with individual polar molecules demonstrate that the cold superfluid matrix enables full orientation of the molecular dipole along the external field. This translates into…

Atomic and Molecular Clusters · Physics 2016-11-21 Daniel J. Merthe , Vitaly V. Kresin

A roughly constant temperature over a wide range of densities is maintained in molecular clouds through radiative heating and cooling. An isothermal equation of state is therefore frequently employed in molecular cloud simulations. However,…

Astrophysics · Physics 2009-11-11 G. Pavlovski , M. D. Smith , M. -M. Mac Low

Molecular dynamics in pure water and aqueous salt solutions remain incompletely understood, partly due to the apparent contradictions between results from different spectroscopic techniques. In this work, we demonstrate, by detailed…

Soft Condensed Matter · Physics 2025-12-22 Rolf Zeißler , Florian Pabst , Thomas Blochowicz

Extracting from trajectory data meaningful information to understand complex molecular systems might be non-trivial. High-dimensional analyses are typically assumed to be desirable, if not required, to prevent losing important information.…

Chemical Physics · Physics 2025-12-01 Chiara Lionello , Matteo Becchi , Simone Martino , Giovanni M. Pavan

When an ensemble of particles interact hydrodynamically, they generically display large-scale transient structures such as swirls in sedimenting particles [1], or colloidal strings in sheared suspensions [2]. Understanding these…

Soft Condensed Matter · Physics 2013-01-24 Nicolas Desreumaux , Jean-Baptiste Caussin , Raphael Jeanneret , Eric Lauga , Denis Bartolo

We present a novel dynamic light scattering setup to probe, with time and space resolution, the microscopic dynamics of soft matter systems confined within millimeter-sized spherical drops. By using an ad-hoc optical layout, we tackle the…

Soft Condensed Matter · Physics 2024-02-16 Matteo Milani , Ty Phou , Guillame Prevot , Laurence Ramos , Luca Cipelletti

A new setup for doping helium nanodroplets by means of laser ablation at kilohertz repetition rate is presented. The doping process is characterized and two distinct regimes of laser ablation are identified. The setup is shown to be…

Atomic and Molecular Clusters · Physics 2011-12-19 M. Mudrich , B. Forkl , S. Mueller , M. Dvorak , O. Buenermann , F. Stienkemeier

We have investigated the formation of helium droplets in two physical situations. In the first one, droplets are atomised from superfluid or normal liquid by a fast helium vapour flow. In the second, droplets of normal liquid are formed…

Soft Condensed Matter · Physics 2009-11-13 Pierre-Etienne Wolf , Fabien Bonnet , Sylvain Perraud , Laurent Puech , Bernard Rousset , Pierre Thibault

A critical study of the wave mechanics of a particle trapped in a 1-D box having infinite potential walls and small flexibility in its size reveals its several important and hither to unknown aspects which could be relevant for better…

Materials Science · Physics 2009-04-03 Yatendra S. Jain

The autoionization dynamics of superexcited superfluid He nanodroplets doped with Na atoms is studied by extreme-ultraviolet (XUV) time-resolved electron spectroscopy. Following excitation into the higher-lying droplet absorption band, the…

Stable ultracold ensembles of dipolar molecules hold great promise for many-body quantum physics, but high inelastic loss rates have been a long-standing challenge. Recently, it was shown that gases of fermionic molecules can be effectively…

The frontiers of quantum electronics have been linked to the discovery of new refrigeration methods since the discovery of superconductivity at a temperature around $4\,$K, enabled by the liquefaction of helium. Since then, the advances in…

Mesoscale and Nanoscale Physics · Physics 2020-03-05 Nikolai Yurttagül , Matthew Sarsby , Attila Geresdi