Related papers: Control defeseance by anti-alignment in the excite…
The phase diagram of a frustrated S=1/2 antiferromagnetic spin ladder with additional next-nearest neighbor exchanges, both diagonal and inchain, is studied by a weak-coupling effective field theory approach combined with exact…
We study how polaronic states form as a function of time due to strong electron-phonon coupling, starting from a hot electron distribution which is representative of a photo-induced metallic state immediately after laser excitation. For…
Ionization of acetylene by linearly-polarized, vacuum ultraviolet (VUV) laser pulses is modelled using time-dependent density functional theory. Several laser wavelengths are considered including one that produces direct ionization to the…
We have demonstrated, both theoretically and experimentally, that it is possible to control (i.e., to enhance or cancel) the contrast of the interference pattern appearing in the intensity images obtained with a laser optical feedback…
The measured multi-dimensional spectral response of different light harvesting complexes exhibits oscillatory features which suggest an underlying coherent energy transfer. However, making this inference rigorous is challenging due to the…
The impact of the optical field polarization on the spectrum of magnetically-induced transitions, a class of transitions forbidden at zero magnetic field, is studied with a weak-probe sub-Doppler technique. The high spectral resolution of…
We study the nonlinear and resonant process of two-photon ionization of atoms (He and H) in a pump-probe scheme. The pump pulse prepares the quantum system in a superposition of the ground state and an excited bound state. By varying the…
The magnetic properties and electronic structure of the ground and excited states of two recently characterized endohedral metallo-fullerenes, [Gd$_2$@C$_{78}$]$^{-}$ (1) and [Gd$_2$@C$_{80}$]$^{-}$ (2), have been studied by theoretical…
We investigate the efficacy of boosting the nonlinear-optical response by using novel systems such as those in an excited state or with a degenerate ground state. By applying the Three Level Ansatz (TLA) and using the Thomas-Reiche-Kuhn…
We have experimentally and theoretically investigated the mixed-field orientation of rotational-state-selected OCS molecules and we achieve strong degrees of alignment and orientation. The applied moderately intense nanosecond laser pulses…
The conventional picture of the light amplification by stimulated emission of radiation (laser) is broken under the ultrastrong interaction between the electromagnetic fields and matter, and distinct dynamics of the electric field and of…
We report unidirectional radiation of a magnetic dipole above planar metal surface, the radiation direction can be manipulated via changing the distance between the dipole and the surface. This phenomenon is unique for the combination of…
The swift excitation of the transparent dielectrics by intense short laser pulse produces ultra-fast re-structuring of the electronic landscape generating a wealth of material states continuously changing in space and in time in accord with…
We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…
We demonstrate polarization spectroscopy of an excited state transition in room temperature cesium vapor. An anisotropy induced by a circularly polarized pump beam on the D2 transition is observed using a weak probe on the 6P3/2 to 7S1/2…
A ballistic ring in presence of collinear dc and high-frequency electric fields is considered. A possibility is demonstrated of the system switching between two states by changing the strength of dc and/or high-frequency field. It leads to…
Ionization, excitation, and de-excitation to the ground state is studied theoretically for the first excited singlet state B $^1\Sigma_u^+$ of H$_2$ exposed to intense laser fields with photon energies in between about 3 eV and 13 eV. A…
The magnetic ground state phase diagram of the disordered Hubbard model at half-filling is computed in dynamical mean-field theory supplemented with the spin resolved, typical local density of states. The competition between many-body…
Studying the excited states of doublets is challenging for their typically multiconfigurational character. We employ light-scanning-tunneling microscopy (light-STM) to investigate photon-induced currents on a single open-shell PTCDA anion…
Atom-surface forces using excited states have a host of compelling applications, including repulsive and lateral forces. However, such states can be fragile and difficult to prepare. Here we report an explicit normal-mode based calculation…