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The infrared range optical absorption mechanism of Carbon-Copper composite thin layer coated on the Diamond-Like Carbon (DLC) buffer layer has been investigated. By consideration of weak interactions between copper nanoparticles in their…

We present an efficient implementation of ab initio many-body quantum embedding and local correlation methods for infinite periodic systems through translational symmetry adapted interpolative separable density fitting, an approach which…

Strongly Correlated Electrons · Physics 2026-01-26 Junjie Yang , Ning Zhang , Shunyue Yuan , Jincheng Yu , Hong-Zhou Ye , Garnet Chan

A novel finite-element method for calculating the illumination-dependence of absorption in three-dimensional nanostructures is presented based on the RF module of the COMSOL software package. This method is capable of numerically…

Optics · Physics 2015-05-28 Mária Csete , Áron Sipos , Faraz Najafi , Xiaolong Hu , Karl K. Berggren

State specific orbital optimized density functional theory (OO-DFT) methods like restricted open-shell Kohn-Sham (ROKS) can attain semiquantitative accuracy for predicting X-ray absorption spectra of closed-shell molecules. OO-DFT methods…

Chemical Physics · Physics 2022-06-15 Diptarka Hait , Katherine J. Oosterbaan , Kevin Carter-Fenk , Martin Head-Gordon

Optical absorption imaging has become a common technique for detecting the density distribution of ultracold atoms. The defocus effect generally produces artificial spatial structures in the obtained images, which confuses our understanding…

Atomic Physics · Physics 2019-03-27 Tianyou Gao , Dongfang Zhang , Lingran Kong , Ruizong Li , Kaijun Jiang

We present a systematic investigation of the role and importance of excitonic effects on the optical properties of transitions metal oxide perovskites. A representative set of fourteen compounds has been selected, including 3$d$ (SrTiO$_3$,…

We study the phase diagram of the asymmetric Hubbard model (AHM), which is characterized by different values of the hopping for the two spin projections of a fermion or equivalently, two different orbitals. This model is expected to provide…

Quantum Gases · Physics 2015-06-12 E. A. Winograd , R. Chitra , M. J. Rozenberg

We propose a fast and non-destructive spectroscopic method for single molecular ions that implements quantum logic schemes between an atomic ion and the molecular ion of interest. Our proposal relies on a hybrid coherent manipulation of the…

Inspired by recent advances in atomic homo and heterostructures, we consider the vertical stacking of plasmonic lattices as a new degree of freedom to create a coupled system showing a modified optical response concerning the monolayer. The…

Optics · Physics 2021-08-10 D. Becerril , G. Pirruccio , Cecilia Noguez

We extend our recently developed sparse-stochastic fragmented exchange formalism for ground-state hybrid DFT (ngH-DFT) to calculate absorption spectra within linear-response time-dependent Generalized Kohn-Sham DFT (LR-GKS-TDDFT), for…

Chemical Physics · Physics 2025-03-11 Mykola Sereda , Tucker Allen , Nadine C. Bradbury , Khaled Z. Ibrahim , Daniel Neuhauser

This study presents band-ensemble Spectral Proper Orthogonal Decomposition (bSPOD). The approach is inspired by frequency smoothing, a method used to reduce estimator variance in power spectral density estimates, and is here extended to…

We present an efficient algorithm for one- and two-component relativistic exact-decoupling calculations. Spin-orbit coupling is thus taken into account for the evaluation of relativistically transformed (one-electron) Hamiltonian. As the…

Chemical Physics · Physics 2013-05-10 Daoling Peng , Nils Middendorf , Florian Weigend , Markus Reiher

The linear optical absorption spectra of three isomers of planar boron cluster B$_{13}$ are calculated using time-dependent spin-polarized density functional approach. The geometries of these cluster are optimized at the B3LYP/6-311+G*…

Atomic and Molecular Clusters · Physics 2013-02-12 Ravindra Shinde , Meenakshi Tayade

In the development of highly efficient photovoltaic cells, solid perovskite systems have demonstrated unprecedented promise, with the figure of merit exceeding nineteen percent of efficiency. In this paper, we investigate the optical and…

Materials Science · Physics 2015-02-05 Towfiq Ahmed , C. La-O-Vorakiat , T. Salim , Y. M. Lam , Elbert E. M. Chia , Jian-Xin Zhu

We propose a new approach to constructing a phase diagram using the effective Hamiltonian derived only from a single real-space image produced by scanning tunneling microscopy (STM). Currently, there have been two main methods to construct…

Materials Science · Physics 2017-09-07 Kazuhito Takeuchi , Koretaka Yuge , Shinya Tabata , Hiroki Saito , Shu Kurokawa , Akira Sakai

The integration of density functional theory (DFT) with machine learning enables efficient \textit{ab initio} electronic structure calculations for ultra-large systems. In this work, we develop a transfer learning framework tailored for…

Materials Science · Physics 2025-01-23 Ting Bao , Ning Mao , Wenhui Duan , Yong Xu , Adrian Del Maestro , Yang Zhang

In this paper, we develop a robust fast method for mobile-immobile variable-order (VO) time-fractional diffusion equations (tFDEs), superiorly handling the cases of small or vanishing lower bound of the VO function. The valid fast…

Numerical Analysis · Mathematics 2022-06-22 Jia-Li Zhang , Zhi-Wei Fang , Hai-Wei Sun

In this work, the benefits of the phase fitting technique are embedded in high order discrete Lagrangian integrators. The proposed methodology creates integrators with zero phase lag in a test Lagrangian in a similar way used in phase…

Instrumentation and Methods for Astrophysics · Physics 2009-04-02 O. T. Kosmas , D. S. Vlachos

We present a first-principles method for relaxing a material's geometry in an optically excited state. This method, based on the Bethe-Salpeter equation, consists of solving coupled equations for exciton wavefunctions and atomic…

Computational Physics · Physics 2022-12-29 Mao Yang , Claudia Draxl

An efficient direct solver for solving the Lippmann-Schwinger integral equation modeling acoustic scattering in the plane is presented. For a problem with $N$ degrees of freedom, the solver constructs an approximate inverse in…

Numerical Analysis · Mathematics 2020-07-28 Abinand Gopal , Per-Gunnar Martinsson