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We demonstrate the importance of electron correlation effects in the hyperfine structure constants of many low-lying states in $^{210}$Fr and $^{212}$Fr. This is achieved by calculating the magnetic dipole and electric quadrupole hyperfine…

Atomic Physics · Physics 2015-05-20 B. K. Sahoo , D. K. Nandy , B. P. Das , Y. Sakemi

We have systematically investigated the ground-state hyperfine structure for alkali-metal atoms ^{87}Rb, ^{133}Cs, ^{211}Fr and alkali-metal-like ions ^{135}Ba^+, ^{225}Ra^+, which are of particular interest for parity violation studies.…

Atomic Physics · Physics 2017-12-20 J. S. M. Ginges , A. V. Volotka , S. Fritzsche

We analyze second-order $M1$-$M1$ and $M1$-$E2$ effects to the hyperfine structure (HFS) of the lowest energy $P$ states of alkali-metal atoms arising from the coupling of the two ($J=1/2,3/2$) fine-structure levels through the hyperfine…

Atomic Physics · Physics 2011-07-13 K. Beloy , A. Derevianko

The hyperfine structure constants of the lowest $s$ and $p_{1/2}$ states of superheavy elements Z=119 and Z= 120$^+$ are calculated using {\em ab initio} approach. Core polarization and dominating correlation effects are included to all…

Atomic Physics · Physics 2015-05-13 T. H. Dinh , V. A. Dzuba , V. V. Flambaum

Accurate predictions of hyperfine structure (HFS) constants are important in many areas of chemistry and physics, from the determination of nuclear electric and magnetic moments to benchmarking of new theoretical methods. We present a…

Atomic Physics · Physics 2020-07-01 Pi A. B. Haase , Ephraim Eliav , Miroslav Iliaš , Anastasia Borschevsky

We present measurements of the hyperfine structure splittings of $nS_{1/2}$ Rydberg states of $^{85}$Rb for $n$= 43, 44, 45 and 46. From the splittings, the hyperfine coupling constant, $A_{\mathrm{HFS}}$, is determined to be 15.372(80)…

Atomic Physics · Physics 2020-01-29 Andira Ramos , Ryan Cardman , Georg Raithel

The low-lying n(=3,4,5)d $^2D_{5/2}$ states alkaline earth ions are of vital importance in a number of different physical applications. The hyperfine structure constants of these states are characterized by unusually strong electron…

Atomic Physics · Physics 2015-06-26 B. K. Sahoo , C. Sur , T. Beier , B. P. Das , R. K. Chaudhuri , D. Mukherjee

We measure the hyperfine structure of $nP_{1/2}$ Rydberg states using mm-wave spectroscopy on an ensemble of laser-cooled $^{85}$Rb atoms. Systematic uncertainties in our measurement from the Zeeman splittings induced by stray magnetic…

Atomic Physics · Physics 2022-12-14 Ryan Cardman , Georg Raithel

Multiconfiguration Hartree-Fock (MCHF) and multiconfiguration Dirac-Hartree-Fock (MCDHF) calculations are performed for the $2p^{5}~^{2}P^{o}$, $2p^4(^{3}P)3s~^{4}P$, $2p^4(^{3}P)3s~^{2}P$ and $2p^4(^{3}P)3p~^{4}S^o$ states of $^{19}$F~I to…

Atomic Physics · Physics 2018-04-12 Nouria Aourir , Messaoud Nemouchi , Michel Godefroid , Per Jönsson

Using relativistic multiconfiguration Dirac-Hartree-Fock method, we calculate the hyperfine-structure properties of the $2s2p$ $^3\!P_{J}$ state in $^9$Be. The hyperfine-structure properties encompass first-order hyperfine-structure…

Atomic Physics · Physics 2024-11-21 Yu-Shan Zhang , Wei Dang , Kai Wang , Yong-Bo Tang

We report measurements of the absolute energies of the hyperfine components of the $12s \ ^2S_{1/2}$ and $13s \ ^2S_{1/2}$ levels of atomic cesium, $^{133}$Cs. Using the frequency difference between these components, we determine the…

Atomic Physics · Physics 2022-03-14 Jonah A. Quirk , Amy Damitz , Carol E. Tanner , D. S. Elliott

High-precision molecular experiments testing the Standard Model of particle physics require an accurate understanding of the molecular structure at the hyperfine level, both for the control of the molecules and for the interpretation of the…

Atomic Physics · Physics 2025-11-19 Yuly Chamorro , Felix Kogel , Tim Langen , Anastasia Borschevsky

A large-scale configuration-interaction (CI) calculation is reported for the hyperfine splitting of the 2^2S and 3^2S states of ^7Li and ^9Be^+. The CI calculation based on the Dirac-Coulomb-Breit Hamiltonian is supplemented with a separate…

Atomic Physics · Physics 2009-11-13 V. A. Yerokhin

We present calculations of the hyperfine coupling constants for all the heteronuclear alkali-metal diatomic molecules at the equilibrium geometry of the electronic ground state. These constants are important in developing methods to control…

Atomic Physics · Physics 2017-11-01 J. Aldegunde , J. M. Hutson

State-dependent quantum electrodynamic corrections are evaluated for the hyperfine splitting of nS states for arbitrary principal quantum number n. The calculations comprise both the self-energy and the vacuum-polarization correction of…

Atomic Physics · Physics 2007-05-23 Ulrich D. Jentschura , Vladimir A. Yerokhin

Advances in laser spectroscopy of superheavy ($Z>100$) elements enabled determination of the nuclear moments of the heaviest nuclei, which requires high-precision atomic calculations of the relevant hyperfine structure (HFS) constants.…

Atomic Physics · Physics 2018-12-05 S. G. Porsev , M. S. Safronova , U. I. Safronova , V. A. Dzuba , V. V. Flambaum

This work presents a first time accurate calculation of the magnetic dipole hyperfine structure constants for the ground state and some low-lying excited states of Pb$^+$. By comparing different levels of approximation with experimental…

Atomic Physics · Physics 2009-11-10 Bijaya K. Sahoo , Rajat K. Chaudhuri , B. P. Das , Holger Merlitz , Debashis Mukherjee

Accurate calculations of the fine and hyperfine splitting of the 2P state in Li and Be$^+$ isotopes using the explicitly correlated Hylleraas basis set are presented. Theoretical predictions including the mixing of $P_{1/2}$ and $P_{3/2}$…

Atomic Physics · Physics 2009-11-13 Mariusz Puchalski , Krzysztof Pachucki

Low temperature scanning tunneling spectroscopy of HfNiSn shows a V^m(m < 1) zero bias anomaly around the Fermi level. This local density of states with a fractional power law shape is well known to be a consequence of electronic…

Disordered Systems and Neural Networks · Physics 2020-12-09 Minjie Lu , Hao Chen , Glenn Agnolet

Calculations of the magnetic hyperfine structure rely on the input of nuclear properties -- nuclear magnetic moments and nuclear magnetization distributions -- as well as quantum electrodynamic (QED) radiative corrections for high-accuracy…

Atomic Physics · Physics 2018-09-19 J. S. M. Ginges , A. V. Volotka
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