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As a step toward the full \emph{ab-initio} description of two-photon double ionization processes, we present a finite-pulse version of the virtual-sequential model for polyelectronic atoms. The model relies on the \emph{ab initio}…

Atomic Physics · Physics 2023-08-02 Siddhartha Chattopadhyay , Carlos Marante , Barry Schneider , Luca Argenti

We discuss the final stages of the simultaneous ionization of two or more electrons due to a strong laser pulse. An analysis of the classical dynamics suggests that the dominant pathway for non-sequential escape has the electrons escaping…

Quantum Physics · Physics 2009-11-06 Bruno Eckhardt , Krzysztof Sacha

We show that scattering amplitudes between initial wave packet states and certain coherent final states can be computed in a systematic weak coupling expansion about classical solutions satisfying initial value conditions. The initial value…

High Energy Physics - Phenomenology · Physics 2009-10-28 Thomas M. Gould , Stephen D. H. Hsu , Erich R. Poppitz

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the…

Atomic Physics · Physics 2009-02-14 Denys I. Bondar , Wing-Ki Liu , Misha Yu. Ivanov

Starting from the Schr\"odinger-equation of a composite system, we derive unified dynamics of a classical harmonic system coupled to an arbitrary quantized system. The classical subsystem is described by random phase-space coordinates…

Quantum Physics · Physics 2007-05-23 Lajos Diosi

I discuss a formalism for computing quantum scattering amplitudes using a semiclassical expansion of a functional integral representation for the S-matrix. The classical background for the expansion is determined by solving the equations of…

High Energy Physics - Phenomenology · Physics 2007-05-23 Stephen D. H. Hsu

The development of emerging technologies in quantum optics demands accurate models that faithfully capture genuine quantum effects. Mature semiclassical approaches reach their limits when confronted with quantized electromagnetic fields,…

An ab initio quantum-classical mixed scheme for the time evolution of electrode-device-electrode systems is introduced to study nuclear dynamics in quantum transport. Two model systems are discussed to illustrate the method. Our results…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Claudio Verdozzi , Gianluca Stefanucci , Carl-Olof Almbladh

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu

We study the quantum-classical correspondence of an experimentally accessible system of interacting bosons in a tilted triple-well potential. With the semiclassical analysis, we get a better understanding of the different phases of the…

Quantum Physics · Physics 2021-10-20 E. R. Castro , Jorge Chavez-Carlos , I. Roditi , Lea F. Santos , Jorge G. Hirsch

Analytical expressions for the semiclassical dressed states and corresponding quasienergies are obtained for a two-level quantum system driven by a nonresonant and/or strong laser field in a coherent state. These expressions are of first…

Quantum Physics · Physics 2010-07-01 A. Santana , J. M. Gomez Llorente , V. Delgado

The interaction of a single-photon wave packet with an initially excited two-level atom in free space is studied in semiclassical and quantum approaches. It is shown that the final state of the field does not contain doubly occupied modes.…

Quantum Physics · Physics 2013-05-30 P. V. Elyutin

We present a novel mixed quantum-classical approach to the coupled electron-nuclear dynamics based on the exact factorization of the electron-nuclear wave function, recently proposed in [A. Abedi, N. T. Maitra, and E. K. U. Gross, Phys.…

Chemical Physics · Physics 2015-06-18 Ali Abedi , Federica Agostini , E. K. U. Gross

We study the exact solutions of the cascade three-level atom interacting with a single mode classical and quantized field with different initial conditions of the atom. For the semiclassical model, it is found that if the atom is initially…

Quantum Physics · Physics 2007-11-27 Mihir Ranjan Nath , Surajit Sen , Gautam Gangopadhyay

We study double ionization in a one-dimensional model of a three-electron atom exposed to strong short laser fields. The corresponding ab initio simulations reveal a characteristic ``knee'' in the ionization yield at lower field intensities…

Atomic Physics · Physics 2025-06-30 Dmitry Efimov

Semiclassical electrodynamics is an appealing approach for studying light-matter interactions, especially for realistic molecular systems. However, there is no unique semiclassical scheme. On the one hand, intermolecular interactions can be…

Chemical Physics · Physics 2019-12-16 Tao E. Li , Hsing-Ta Chen , Abraham Nitzan , Joseph E. Subotnik

Building on insights about the classical pathways to double ionization in strong laser fields we here propose a 1+1-dimensional model that captures essentials of the 3-d potential landscape and allows efficient studies of the process in…

Atomic Physics · Physics 2009-11-11 Bruno Eckhardt , Krzysztof Sacha

A theoretical framework for studying strong-field ionization of aligned molecules is presented, and alignment-dependent ionization yields are computed for CO2. Our calculations are in unprecedented agreement with recent experiments. We find…

Atomic Physics · Physics 2009-06-17 M. Abu-samha , L. B. Madsen

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

Quantum stochastic differential equations have been used to describe the dynamics of an atom interacting with the electromagnetic field via absorption/emission processes. Here, by using the full quantum stochastic Schroedinger equation…

Quantum Physics · Physics 2009-10-31 Alberto Barchielli , Giancarlo Lupieri