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We propose a framework for describing the dynamics associated with the adsorption of small molecules to liquid-vapor interfaces, using an intermediate resolution between traditional continuum theories that are bereft of molecular detail and…

Chemical Physics · Physics 2024-01-25 Kritanjan Polley , Kevin R. Wilson , David T. Limmer

We propose a theoretical investigation of the physical adsorption of neutral comb-polymers with an adsorbing skeleton and non-adsorbing side-chains on a flat surface. Such polymers are particularly interesting as "dynamic coating" matrices…

Soft Condensed Matter · Physics 2009-11-11 Anna Sartori , Albert Johner , Jean-Louis Viovy , Jean-Francois Joanny

Many experimental studies of protein deposition on solid surfaces involve alternating adsorption/desorption steps. In this paper, we investigate the effect of a desorption step (separating two adsorption steps) on the kinetics, the…

Statistical Mechanics · Physics 2009-10-31 Paul R. Van Tassel , Pascal Viot , Gilles Tarjus , Jeremy J. Ramsden , Julian Talbot

We study the adsorption of homogeneous or heterogeneous polymers onto heterogeneous planar surfaces with exponentially decaying site-site correlations, using a variational reference system approach. As a main result, we derive simple…

Soft Condensed Matter · Physics 2009-11-11 Alexey Polotsky , Friederike Schmid , Andreas Degenhard

An analytical theory is presented for the damping of low-frequency adsorbate vibrations via resonant coupling to the substrate phonons. The system is treated classically, with the substrate modeled as a semi-infinite elastic continuum and…

Materials Science · Physics 2009-10-30 Steven P. Lewis , M. V. Pykhtin , E. J. Mele , Andrew M. Rappe

We present a theoretical study of the phase diagram and the structure of a fluid adsorbed in high-porosity aerogels by means of an integral-equation approach combined with the replica formalism. To simulate a realistic gel environment, we…

Disordered Systems and Neural Networks · Physics 2009-11-07 V. Krakoviack , E. Kierlik , M. -L. Rosinberg , G. Tarjus

Ultrasonic guided waves offer a convenient and practical approach to structural health monitoring and non-destructive evaluation. A key property of guided waves is the fully-defined relationship between central frequency and propagation…

We present an experimental approach to detect the saturated absorption spectroscopy different from conventional scheme. Using this approach, crossovers are removed to avoid their overlap with other peaks in the spectrum and sensitivity of…

Atomic Physics · Physics 2015-03-17 Jun Duan , Xianghui Qi , Xiaoji Zhou , Xuzong Chen

Since its foundations, more than one hundred years ago, the field of structural biology has strived to understand and analyze the properties of molecules and their interactions by studying the structure that they take in 3D space. However,…

Biomolecules · Quantitative Biology 2023-02-27 Gabriele Corso

The inference of the absorption configuration of an existing room solely using acoustic signals can be challenging. This research presents two methods for estimating the room dimensions and frequency-dependent absorption coefficients using…

Sound · Computer Science 2023-04-26 Yuanxin Xia , Cheol-Ho Jeong

We analyze the qualitative features in the transition spectra of a model superconductor with multiple energy gaps, using a simple extension of the Mattis-Bardeen expression for probes with case I and case II coherence factors. At…

Superconductivity · Physics 2009-11-07 Sergey V. Barabash , David Stroud

A simple multiscale approach to the diffusion-driven adsorption from a solution to a solid surface is presented. The model combines two important features of the adsorption process: (i) the kinetics of the chemical reaction between…

Chemical Physics · Physics 2009-11-13 Radek Erban , S. Jonathan Chapman

We study the problem of phase separation in systems with a positive definite order parameter, and in particular, in systems with absorbing states. Owing to the presence of a single minimum in the free energy driving the relaxation kinetics,…

Condensed Matter · Physics 2009-10-31 M. A. Munoz , U. Marini Bettolo Marconi , R. Cafiero

A generalized dispersion equation is derived featuring coupled mode theory, parity-time symmetry, and leaky wave antennas of arbitrary periodic modulation. It can be specialized to each of these cases individually or can describe a…

Optics · Physics 2024-08-07 Afshin Abbaszadeh , Jordan Budhu

Recent machine learning models to accurately obtain gas adsorption isotherms focus on polymers or metal-organic frameworks (MOFs) separately. The difficulty in creating a unified model that can predict the adsorption trends in both types of…

Soft Condensed Matter · Physics 2024-07-01 Subhadeep Dasgupta , Amal R S , Prabal K. Maiti

Lying-standing transitions in the first molecular monolayer at organic-inorganic interfaces strongly influence interface dipoles, energy-level alignment, and growth modes, yet their collective kinetics remain difficult to predict. Here, we…

Computational Physics · Physics 2026-02-26 Anna Werkovits , Simon B. Hollweger , Oliver T. Hofmann

A multiscale QM/classical approach is presented, that is able to model the optical properties of complex nanostructures composed of a molecular system adsorbed on metal nanoparticles. The latter are described by a combined…

Chemical Physics · Physics 2024-10-29 Pablo Grobas Illobre , Piero Lafiosca , Luca Bonatti , Tommaso Giovannini , Chiara Cappelli

Describing particle transport at the macroscopic or mesoscopic level in non-ideal environments poses fundamental theoretical challenges in domains ranging from inter and intra-cellular transport in biology to diffusion in porous media. Yet,…

Statistical Mechanics · Physics 2013-09-11 Marta Galanti , Duccio Fanelli , Francesco Piazza

Adsorption on a boundary line confining a monolayer of particles self-assembling into clusters is studied by MC simulations. We focus on a system of particles interacting via competing interaction potential in which effectively short-range…

Soft Condensed Matter · Physics 2020-01-22 E. Bildanau , J. Pȩkalski , V. Vikhrenko , A. Ciach

The time dependency of the diffusion coefficient of particles in porous media is an efficient probe of their geometry. The analysis of this quantity, measured e.g. by nuclear magnetic resonance (PGSE-NMR), can provide rich information…

Soft Condensed Matter · Physics 2013-02-13 Maximilien Levesque , Olivier Bénichou , Benjamin Rotenberg