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We propose a scheme to eliminate the effect of non-nearest-neighbor qubits in preparing cluster state with double-dot molecules. As the interaction Hamiltonians between qubits are Ising-model and mutually commute, we can get positive and…

Quantum Physics · Physics 2008-04-24 Guo-Ping Guo , Xiao-Jie Hao , Tao Tu , Zhi-Cheng Zhu , Guang-Can Guo

The iterative quantum phase estimation algorithm, applied to calculating the ground state energies of quantum chemical systems, is theoretically appealing in its wide scope of being able to handle both weakly and strongly correlated…

Quantum Physics · Physics 2021-11-11 Dipanjali Halder , Srinivasa Prasannaa V. , Valay Agarawal , Rahul Maitra

Quantum computing (QC) provides a promising avenue toward enabling quantum chemistry calculations, which are classically impossible due to a computational complexity that increases exponentially with system size. As fully fault-tolerant…

Utilizing quantum computer to investigate quantum chemistry is an important research field nowadays. In addition to the ground-state problems that have been widely studied, the determination of excited-states plays a crucial role in the…

Quantum computing is emerging as a new computational paradigm with the potential to transform several research fields, including quantum chemistry. However, current hardware limitations (including limited coherence times, gate infidelities,…

We introduce a quantum Monte Carlo inspired reweighting scheme to accurately compute energies from optimally short quantum circuits. This effectively hybrid quantum-classical approach features both entanglement provided by a short quantum…

Quantum Physics · Physics 2019-10-07 Guglielmo Mazzola , Pauline Ollitrault , Panagiotis Barkoutsos , Ivano Tavernelli

Determining the energy gap in a quantum many-body system is critical to understanding its behavior and is important in quantum chemistry and condensed matter physics. The challenge of determining the energy gap requires identifying both the…

Quantum Physics · Physics 2026-03-04 Mengzhen Ren , Yu-Cheng Chen , Ching-Jui Lai , Min-Hsiu Hsieh , Alice Hu

A recent work [1] proposed a type of cluster entangled coherent states and its generation. Here we present an alternative experimental arrangement for its generation in bimodal QED cavities. The scheme employs a single two-level atom that…

Quantum Physics · Physics 2009-11-13 E. M. Becerra-Castro , W. B. Cardoso , A. T. Avelar , B. Baseia

We propose a relativistic unitary coupled cluster (UCC) expectation value approach for computing first-order properties of heavy-element systems. Both perturbative (UCC3) and non-perturbative (qUCC) commutator-based formulations are applied…

Chemical Physics · Physics 2026-02-03 Kamal Majee , Somesh Chamoli , Malaya K. Nayak , Achintya Kumar Dutta

In this work, we aim to solve a practical use-case of unsupervised clustering which has applications in predictive maintenance in the energy operations sector using quantum computers. Using only cloud access to quantum computers, we…

Quantum Physics · Physics 2022-09-13 Stephen DiAdamo , Corey O'Meara , Giorgio Cortiana , Juan Bernabé-Moreno

We present a novel method for improving the quantum simulation of the ground state energy of molecules. We perform a pre-processing step classically, which reduces the dimensionality of the problem by generating a custom mapping which…

Quantum Physics · Physics 2023-03-03 Kaur Kristjuhan , Mark Nicholas Jones

This article is a short introduction to and review of the cluster-state model of quantum computation, in which coherent quantum information processing is accomplished via a sequence of single-qubit measurements applied to a fixed quantum…

Quantum Physics · Physics 2009-11-11 Michael A. Nielsen

In truncated coupled-cluster (CC) theories, non-variational and/or generally complex ground-state energies can occur. This is due to the non-Hermitian nature of the similarity transformed Hamiltonian matrix in combination with CC…

Chemical Physics · Physics 2023-09-22 Tanner Culpitt , Erik I. Tellgren , Fabijan Pavosevic

Current quantum devices have unutilized high-level quantum resources. More and more attention has been paid to the qudit quantum systems with larger than two dimensions to maximize the potential computing power of quantum computation. Then,…

Quantum Physics · Physics 2025-04-18 Shuai Yang , Lihao Xu , Guojing Tian , Xiaoming Sun

The unitary coupled cluster (UCC) approximation is one of the more promising wave-function ans\"atze for electronic structure calculations on quantum computers via the variational quantum eigensolver algorithm. However, for large systems…

Quantum Physics · Physics 2021-09-30 Jia Chen , Hai-Ping Cheng , James K. Freericks

A practical fault-tolerant quantum computer is worth looking forward to as it provides applications that outperform their known classical counterparts. However, millions of interacting qubits with stringent criteria are required, which is…

Quantum Physics · Physics 2021-05-31 Keren Li

The development of a quadratic unitary coupled-cluster singles and doubles (qUCCSD) based self-consistent polarization propagator method is reported. We present a simple strategy for truncating the commutator expansion of the UCC…

Chemical Physics · Physics 2024-06-19 Junzi Liu , Lan Cheng

Rapid progress in noisy intermediate-scale quantum (NISQ) computing technology has led to the development of novel resource-efficient hybrid quantum-classical algorithms, such as the variational quantum eigensolver (VQE), that can address…

Strongly Correlated Electrons · Physics 2021-03-01 Yongxin Yao , Feng Zhang , Cai-Zhuang Wang , Kai-Ming Ho , Peter P. Orth

In this paper, we study a conjugate gradient method for electronic structure calculations. We propose a Hessian based step size strategy, which together with three orthogonality approaches yields three algorithms for computing the ground…

Numerical Analysis · Mathematics 2017-08-30 Xiaoying Dai , Zhuang Liu , Liwei Zhang , Aihui Zhou

Hybrid quantum-classical algorithms provide ways to use noisy intermediate-scale quantum computers for practical applications. Expanding the portfolio of such techniques, we propose a quantum circuit learning algorithm that can be used to…