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Silicon telluride (Si2Te3) is a two-dimensional semiconductor with unique structural properties due to the size contrast between Si and Te atoms. A recent experiment shows that the material turns metallic under hydrostatic pressure, while…

Materials Science · Physics 2021-01-11 Romakanta Bhattarai , Xiao Shen

Using molecular dynamics simulations and integral equations (Rogers-Young, Percus-Yevick and hypernetted chain closures) we investigate the thermodynamic of particles interacting with continuous core-softened intermolecular potential.…

Soft Condensed Matter · Physics 2007-05-23 Alan B. de Oliveira , Paulo A. Netz , Thiago Colla , Marcia C. Barbosa

By using the diffusion Monte Carlo method, we obtained the full phase diagram of $^3$He on top of graphite preplated with a solid layer of $^4$He. All the $^4$He atoms of the substrate were explicitly considered and allowed to move during…

Other Condensed Matter · Physics 2016-11-23 M. C. Gordillo , J. Boronat

We study structure and fluid-phase behaviour of a binary mixture of hard spheres (HSs) and hard spherocylinders (HSCs) in isotropic and nematic states using the $NP_nAT$ ensemble Monte Carlo (MC) method in which a normal pressure tensor…

Soft Condensed Matter · Physics 2015-08-18 Liang Wu , Alexandr Malijevský , George Jackson , Erich A. Müller , Carlos Avendaño

We predict a new candidate high-temperature high-pressure structure of FeSiO$_3$ with space-group symmetry Cmmm by applying an evolutionary algorithm within DFT+U that we call post-perovskite II (PPv-II). An exhaustive search found no other…

Hydrogen-rich ternary hydrides are promising candidates for high-Tc superconductivity at megabar pressures, yet their chemical space is vast and largely unexplored. Combining evolutionary structure searches with first-principles…

The structure of La$_{1-x}$Ca$_{x}$MnO$_{3}$ solid solutions (x=0, 0.25, 0.50, 0.67, 1) under high pressure (up to 40-45 GPa) has been investigated by synchrotron X-ray powder diffraction (XRD) in order to characterize their volume…

Strongly Correlated Electrons · Physics 2007-05-23 A. Sani , C. Meneghini , S. Mobilio , Sugata Ray , D. D. Sarma , J. A. Alonso

Vanadium sesquioxide, V2O3, is a prototypical metal-to-insulator system where, in temperature-dependent studies, the transition always coincides with a corundum-to-monoclinic structural transition. As a function of pressure, V2O3 follows…

Recent heat-capacity experiments show quite unambiguously the existence of a liquid $^3$He phase adsorbed on graphite. This liquid is stable at an extremely low density, possibly one of the lowest found in Nature. Previous theoretical…

Other Condensed Matter · Physics 2016-04-20 M. C. Gordillo , J. Boronat

We study the structural phase transition, originally associated with the highest superconducting critical temperature $T_c$ measured in high-pressure sulfur hydride. A quantitative description of its pressure dependence has been elusive for…

Strongly Correlated Electrons · Physics 2023-12-27 Romain Taureau , Marco Cherubini , Tommaso Morresi , Michele Casula

Hard-sphere fluids confined between parallel plates a distance $D$ apart are studied for a wide range of packing fractions, including also the onset of crystallization, applying Monte Carlo simulation techniques and density functional…

Statistical Mechanics · Physics 2011-10-10 Debabrata Deb , Alexander Winkler , Mohammad Hossein Yamani , Martin Oettel , Peter Virnau , Kurt Binder

A method is proposed for determining the line tension, which is the main physical characteristic of a three-phase contact region, by Monte-Carlo (MC) simulations. The key idea of the proposed method is that if a three-phase equilibrium…

Statistical Mechanics · Physics 2009-11-10 Yuri Djikaev

Pair potentials that are bounded at the origin provide an accurate description of the effective interaction for many systems of dissolved soft macromolecules (e.g., flexible dendrimers). Using numerical free-energy calculations, we…

Soft Condensed Matter · Physics 2014-10-29 C. Speranza , S. Prestipino , G. Malescio , P. V. Giaquinta

We present results of Diffusion Monte Carlo calculations for a system of solid ortho-D_2 at different densities, for pressure ranging from 0 up to 350MPa. We compare the equation of state obtained using two of the most used effective…

Other Condensed Matter · Physics 2009-11-11 Francesco Operetto , Francesco Pederiva

The internal energy of high-density hydrogen plasmas in the temperature range $T = 10,000 ... 50,000 K$ is calculated by two different analytical approximation schemes (method of effective ion-ion interaction potential - EIIP and Pad\'e…

Plasma Physics · Physics 2007-07-29 S. A. Trigger , W. Ebeling , V. S. Filinov , V. E. Fortov , M. Bonitz

We investigate the atomic hydrogen adsorption on Mg(0001) by using density-functional theory within the generalized gradient approximation and a supercell approach. The coverage dependence of the adsorption structures and energetics is…

Materials Science · Physics 2009-04-29 Yanfang Li , Ping Zhang , Bo Sun , Yu Yang , Yinghui Wei

We present and evaluate an efficient method for simulating Raman spectra from molecular dynamics (MD) calculations {\it without} defining normal modes. We apply the method to high pressure hydrogen in the high-temperature "Phase IV": a…

Materials Science · Physics 2014-08-19 G. J. Ackland , I. B. Magdau

High quality reference data from diffusion Monte Carlo calculations are presented for bulk sI methane hydrate, a complex crystal exhibiting both hydrogen-bond and dispersion dominated interactions. The performance of some commonly used…

Materials Science · Physics 2014-05-13 Stephen J. Cox , Michael D. Towler , Dario Alfè , Angelos Michaelides

Confinement of superfluid $^3$He on length scales comparable to the radial size of the p-wave Cooper pairs can greatly alter the phase diagram by stabilizing broken symmetry phases not observed in bulk $^3$He. We consider superfluid $^3$He…

Superconductivity · Physics 2015-11-09 J. J. Wiman , J. A. Sauls

Crystal structure prediction methods and first-principles calculations have been used to explore low-energy structures of carbon monoxide (CO). Contrary to the standard wisdom, the most stable structure of CO at ambient pressure was found…

Materials Science · Physics 2017-04-06 Kang Xia , Jian Sun , Chris J. Pickard , Dennis D. Klug , Richard J. Needs