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Recent elastic and inelastic neutron scattering studies of the highly frustrated pyrochlore antiferromagnet Tb2Ti2O7 have shown some very intriguing features that cannot be modeled by the local <111> classical Ising model, naively expected…

Disordered Systems and Neural Networks · Physics 2007-05-23 Ying-Jer Kao , Matthew Enjalran , Adrian Del Maestro , Hamid R. Molavian , Michel J. P. Gingras

A quantum spin liquid state has long been predicted to arise in spin-1/2 Heisenberg square-lattice antiferromagnets at the boundary region between N\'eel (nearest-neighbor interaction dominates) and columnar (next-nearest-neighbor…

A novel macroscopically degenerate state called kagome ice, which was recently found in a spin ice compound Dy2Ti2O7 in a magnetic field applied along the [111] direction of the cubic unit cell, is studied by specific heat measurements. The…

Materials Science · Physics 2009-11-07 Z. Hiroi , K. Matsuhira , S. Takagi , T. Tayama , T. Sakakibara

Inelastic neutron scattering reveals a broad continuum of excitations in Pr$_2$Zr$_2$O$_7$, the temperature and magnetic field dependence of which indicate a continuous distribution of quenched transverse fields ($\Delta$) acting on the…

The magnetic ground state of oxynitride pyrochlore Lu$_2$Mo$_2$O$_{5-y}$N$_2$, a candidate compound for the quantum spin liquid ($S=1/2$, Mo$^{5+}$), was studied by muon spin rotation/relaxation experiment. In contrast to Lu$_2$Mo$_2$O$_7$…

Strongly Correlated Electrons · Physics 2023-01-11 S. K. Dey , K. Ishida , H. Okabe , M. Hiraishi , A. Koda , T. Honda , J. Yamaura , H. Kageyama , R. Kadono

The ground state of the quantum spin ice candidate magnet Yb2Ti2O7 is known to be sensitive to weak disorder at the 1 percent level which occurs in single crystals grown from the melt. Powders produced by solid state synthesis tend to be…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , K. A. Ross , E. Kermarrec , N. P. Butch , G. Ehlers , H. A. Dabkowska , B. D. Gaulin

We study spin correlations for the highly frustrated classical pyrochlore lattice antiferromagnets with O(N) symmetry in the limit T->0. We conjecture that a local constraint obeyed by the extensively degenerate ground states dictates a…

Disordered Systems and Neural Networks · Physics 2016-08-31 S. V. Isakov , K. Gregor , R. Moessner , S. L. Sondhi

Nd2Hf2O7, belonging to the family of geometrically frustrated cubic rare earth pyrochlore oxides, was recently identified to order antiferromagnetically below T_N = 0.55 K with an all-in/all-out arrangement of Nd3+ moments, however with a…

Strongly Correlated Electrons · Physics 2017-12-15 V. K. Anand , D. L. Abernathy , D. T. Adroja , A. D. Hillier , P. K. Biswas , B. Lake

Spin freezing in the $A$-site spinel FeAl$_2$O$_4$ which is a spin liquid candidate is studied using remnant magnetization and nonlinear magnetic susceptibility and isofield cooling and heating protocols. The remnant magnetization behavior…

Disordered Systems and Neural Networks · Physics 2015-06-23 Harikrishnan S. Nair , Ramesh Kumar K. , Andre M. Strydom

Weak bond disorder disrupts the expected spin-liquid ground-state of the ideal $S$ = 1/2 Heisenberg pyrochlore antiferromagnet. Here we introduce a single crystal study of the structural and magnetic properties of the bond-disordered…

Strongly Correlated Electrons · Physics 2023-07-12 Andrej Kancko , Gerald Giester , Ross H. Colman

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

MuSR experiments have been performed on powder sample of the "ordered spin ice" Tb$_2$Sn$_2$O$_7$ pyrochlore compound. At base temperature (T=35mK) the muon relaxation is found to be of dynamical nature which demonstrates that strong…

Strongly Correlated Electrons · Physics 2009-11-11 F. Bert , P. Mendels , A. Olariu , N. Blanchard , G. Collin , A. Amato , C. Baines , A. D. Hillier

Muon spin relaxation on Nd$_2$Ti$_2$O$_7$ (NTO) and NdLaTi$_2$O$_7$ (NLTO) compounds are presented. The time spectra for both compounds are as expected for the paramagnetic state at high temperatures, but deviate from the exponential…

Strongly Correlated Electrons · Physics 2014-10-21 Hanjie Guo , Hui Xing , Jun Tong , Qian Tao , Isao Watanabe , Zhu-an Xu

The origin of the lowest-temperature anomaly reported several years ago using a polycrystalline sample of the spin ice compound Dy2Ti2O7 had remained unresolved. Here we finally clarify its origin by susceptibility measurements down to 65…

Strongly Correlated Electrons · Physics 2009-11-11 Ryuji Higashinaka , Yoshiteru Maeno

The charge ordered structure of ions and vacancies characterizing rare-earth pyrochlore oxides serves as a model for the study of geometrically frustrated magnetism. The organization of magnetic ions into networks of corner-sharing…

Spin correlations in the pyrochlore antiferromagnet Y_2Ru_2O_7 with Curie-Weiss temperature $\Theta_{CW}=-1100$ K and critical temperature T_N=77 K were examined through neutron scattering. For $T_N<T<\Theta_{CW}/3$ the data show spin…

Strongly Correlated Electrons · Physics 2014-07-03 J. van Duijn , N. Hur , J. W. Taylor , Y. Qiu , Q. Z. Huang , S. -W. Cheong , C. Broholm , T. G. Perring

In this work, we show that the zero field excitation spectra in the quantum spin ice candidate pyrochlore compound \ybti\ is a continuum characterized by a very broad and almost flat dynamical response which extends up to $1-1.5$ meV,…

Strongly Correlated Electrons · Physics 2015-09-30 J. Robert , E. Lhotel , G. Remenyi , S. Sahling , I. Mirebeau , C. Decorse , B. Canals , S. Petit

The results of dc and ac magnetization, heat-capacity, 57Fe Moessbauer spectroscopy, dielectric, pyroelectric current and isothermal magneto-capacitance measurements on a recently reported lithium-based oxide, Li3FeRuO6, related to…

Strongly Correlated Electrons · Physics 2016-09-21 Sanjay Kumar Upadhyay , P. L. Paulose , Kartik K Iyer , E. V. Sampathkumaran

We document the coexistence of ferro- and anti-ferromagnetism in pyrochlore $\rm Yb_2Ti_2O_7$ using three neutron scattering techniques on stoichiometric crystals: elastic neutron scattering shows a canted ferromagnetic ground state,…

Strongly Correlated Electrons · Physics 2020-10-27 A. Scheie , J. Kindervater , S. Zhang , H. J. Changlani , G. Sala , G. Ehlers , A. Heinemann , G. S. Tucker , S. M. Koohpayeh , C. Broholm

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

Strongly Correlated Electrons · Physics 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa