Related papers: High-Harmonic generation from spin-polarised defec…
High-harmonic generation by a highly non-linear interaction of infrared laser fields with matter allows for the generation of attosecond pulses in the XUV spectral regime. This process, well established for atoms, has been recently extended…
We study the high harmonic generation with vortex beams beyond the dipole approximation. To do so we employ the full minimal coupling approach to account for multipolar coupling without truncation and describe the full spatio-temporal…
High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…
Rigorous electrodynamical simulations based on the nonlinear Drude model are performed to investigate the influence of strong coupling on high harmonic generation by periodic metal gratings. It is shown that a thin dispersive material with…
The creation of light-matter hybrid states, polaritons, in a cavity offers new intriguing opportunities to manipulate the electronic structure and electron dynamics of atoms and molecules. Here, we investigate the effect of electronic…
Paramagnetic defects in diamond and hexagonal boron nitride possess a unique combination of spin and optical properties that make them prototypical solid-state qubits. Despite the coherence of these spin qubits being critically limited by…
Optically addressable spin defects in hexagonal boron nitride hold promise for room-temperature quantum technologies, but their microscopic identities remain largely unknown. Using first principles calculations, we show that coupled spin…
Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…
We propose and experimentally demonstrate a scheme allowing to reach noncollinear phase-matching of high harmonic generation in solids, which may potentially lead to an enhancement of the generation efficiency. The principle is based on…
High harmonics have emerged as a powerful ultrafast probe of phonon dynamics and electron-phonon interactions in solids, with most studies focusing on odd harmonics. Here, in a pump-probe setup with variable delay, we theoretically…
The objective of this article is to investigate the profound nonlinear optical response exhibited by inversion symmetric fullerene molecules under the influence of different types of disorders described by the Anderson model. Our aim is to…
Plasmon resonances are known to amplify the electromagnetic fields near metallic nanostructures. Therefore, they are considered to provide a promising scheme to generate extreme-ultraviolet harmonics, using low power drivings. During…
Acting as a highly nonlinear response to the strong laser field, high harmonic generation (HHG) naturally contains the fingerprints of atomic and electronic properties of materials. Electronic properties of a solid such as band structure…
We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…
In the framework of time-dependent density functional theory, we obtain high-order harmonics of photon energies up to 10 Up from bilayer crystals with an interlayer spacing d = 70 {\AA}. At grazing incidence, a clear double-plateau…
Hexagonal boron nitride (hBN) hosts luminescent defects possessing spin qualities compatible with quantum sensing protocols at room temperature. Vacancies, in particular, are readily obtained via exposure to high-energy ion beams. While the…
Mechanically isolated defect centers in hexagonal boron nitride are promising coherent quantum emitters, yet spectral instabilities persist, and their spin-related nature remains unclear. Here we investigate a single mechanically isolated…
High harmonic generation (HHG) in solids reflects the underlying nonperturbative nonlinear dynamics of electrons in a strong light field and is a powerful tool for ultrafast spectroscopy of electronic structures. Photo-carrier doping allows…
High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…
Optically active spin defects in van der Waals materials are promising platforms for modern quantum technologies. Here we investigate the coherent dynamics of strongly interacting ensembles of negatively charged boron-vacancy…